Design strategy for hierarchical structure of carbon black on microporous elastomer surface toward stretchable and compressive strain sensors
Flexible mechanical sensors capable of sensing both compressive and tensile strains with high sensitivity and linear piezoresistive response are of great significance for the development of wearable devices, flexible electronic skins, and robotics. However, it is still of challenge to develop simple...
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| Published in | Carbon (New York) Vol. 206; pp. 53 - 61 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
25.03.2023
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| Subjects | |
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| Abstract | Flexible mechanical sensors capable of sensing both compressive and tensile strains with high sensitivity and linear piezoresistive response are of great significance for the development of wearable devices, flexible electronic skins, and robotics. However, it is still of challenge to develop simple 3-dimensional (3D) porous polymer/carbon nanomaterial composite strain sensors capable of sensing both tensile and compressive strains with reproducible electrical signals. Herein, we report a simple and scalable morphology-engineering strategy, i.e., selective location of carbon black (CB) in polyoxyethylene (PEO)/ethylene-α-octene random copolymer (ORC) blends via phase separation, to fabricate isotropic 3D continuous porous composite strain sensors. Such a composite consists of a continuous porous ORC matrix inlaid with preferable CB distribution on ORC surface after PEO removal, enabling distinguishable detection of both compressive and tensile strains with opposite resistance changes. Specifically, the as-fabricated strain sensors exhibit linear response with a sensitivity of 16 for 0–46% compressive strain, a detection limit of 0.3% strain with 16/16 ms response/recovery time. Besides, it has a large gauge factor for tensile strain of 0–300%, a detection limit strain of 0.06% with 16/47 ms response/recovery time, and low hysteresis degree. As such, it allows for full-range body motion monitoring and Morse code communication.
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| AbstractList | Flexible mechanical sensors capable of sensing both compressive and tensile strains with high sensitivity and linear piezoresistive response are of great significance for the development of wearable devices, flexible electronic skins, and robotics. However, it is still of challenge to develop simple 3-dimensional (3D) porous polymer/carbon nanomaterial composite strain sensors capable of sensing both tensile and compressive strains with reproducible electrical signals. Herein, we report a simple and scalable morphology-engineering strategy, i.e., selective location of carbon black (CB) in polyoxyethylene (PEO)/ethylene-α-octene random copolymer (ORC) blends via phase separation, to fabricate isotropic 3D continuous porous composite strain sensors. Such a composite consists of a continuous porous ORC matrix inlaid with preferable CB distribution on ORC surface after PEO removal, enabling distinguishable detection of both compressive and tensile strains with opposite resistance changes. Specifically, the as-fabricated strain sensors exhibit linear response with a sensitivity of 16 for 0–46% compressive strain, a detection limit of 0.3% strain with 16/16 ms response/recovery time. Besides, it has a large gauge factor for tensile strain of 0–300%, a detection limit strain of 0.06% with 16/47 ms response/recovery time, and low hysteresis degree. As such, it allows for full-range body motion monitoring and Morse code communication. Flexible mechanical sensors capable of sensing both compressive and tensile strains with high sensitivity and linear piezoresistive response are of great significance for the development of wearable devices, flexible electronic skins, and robotics. However, it is still of challenge to develop simple 3-dimensional (3D) porous polymer/carbon nanomaterial composite strain sensors capable of sensing both tensile and compressive strains with reproducible electrical signals. Herein, we report a simple and scalable morphology-engineering strategy, i.e., selective location of carbon black (CB) in polyoxyethylene (PEO)/ethylene-α-octene random copolymer (ORC) blends via phase separation, to fabricate isotropic 3D continuous porous composite strain sensors. Such a composite consists of a continuous porous ORC matrix inlaid with preferable CB distribution on ORC surface after PEO removal, enabling distinguishable detection of both compressive and tensile strains with opposite resistance changes. Specifically, the as-fabricated strain sensors exhibit linear response with a sensitivity of 16 for 0–46% compressive strain, a detection limit of 0.3% strain with 16/16 ms response/recovery time. Besides, it has a large gauge factor for tensile strain of 0–300%, a detection limit strain of 0.06% with 16/47 ms response/recovery time, and low hysteresis degree. As such, it allows for full-range body motion monitoring and Morse code communication. [Display omitted] |
| Author | Sun, Xiao-Rong Gong, Tao Li, Wu-Di Bao, Rui-Ying Ke, Kai Jia, Jin Yang, Wei |
| Author_xml | – sequence: 1 givenname: Tao surname: Gong fullname: Gong, Tao – sequence: 2 givenname: Jin surname: Jia fullname: Jia, Jin – sequence: 3 givenname: Xiao-Rong surname: Sun fullname: Sun, Xiao-Rong – sequence: 4 givenname: Wu-Di surname: Li fullname: Li, Wu-Di – sequence: 5 givenname: Kai surname: Ke fullname: Ke, Kai email: kaike@scu.edu.cn – sequence: 6 givenname: Rui-Ying surname: Bao fullname: Bao, Rui-Ying – sequence: 7 givenname: Wei orcidid: 0000-0003-0198-1632 surname: Yang fullname: Yang, Wei email: weiyang@scu.edu.cn |
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| SubjectTerms | 3D continuous porous structure carbon composite polymers compression strength detection limit hysteresis Isotropic composites isotropy nanomaterials Phase separation polyethylene glycol porous media Pressure/tensile strain sensors separation soot tensile strength Wearable electronics |
| Title | Design strategy for hierarchical structure of carbon black on microporous elastomer surface toward stretchable and compressive strain sensors |
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