Luminescence of trivalent samarium ions in silver and tin co-doped aluminophosphate glass
► Influence of silver and tin on Sm 3+ luminescence in glass. ► Energy transfer mechanism elucidation and connection with glass structure. ► Effect of Ag nanoparticles on material optical properties. This work presents the spectroscopic properties of trivalent samarium ions in a melt-quenched alumin...
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Published in | Optical materials Vol. 33; no. 8; pp. 1215 - 1220 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
Published |
Elsevier B.V
01.06.2011
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Abstract | ► Influence of silver and tin on Sm
3+ luminescence in glass. ► Energy transfer mechanism elucidation and connection with glass structure. ► Effect of Ag nanoparticles on material optical properties.
This work presents the spectroscopic properties of trivalent samarium ions in a melt-quenched aluminophosphate glass containing silver and tin. Addition of 4
mol% of each Ag
2O and SnO into the glass system with 2
mol% Sm
2O
3 results in Sm
3+ ions luminescence under non-resonant UV excitation owing to energy transfer from single silver ions and/or twofold-coordinated Sn centers. Assessment of luminescence spectra and decay dynamics suggest the energy transfer mechanism to be essentially of the resonant radiative type. Moreover, a connection between the luminescent and structural properties of the rare-earth doped glass system was demonstrated. Raman spectroscopy characterization revealed that no significant variation in the glass matrix is induced by Sm
3+ doping at the concentration employed. A comparison was made with a structural study performed on the Eu
3+ doped system (containing 2
mol% Eu
2O
3 along with 4
mol% of each Ag
2O and SnO) where the radiative energy transfer mechanism was previously established. The data appears consistent regarding the lack of variation in glass structure upon the Eu
3+ and Sm
3+ doping in connection with the dominance of the radiative transfer in the matrix. Thermal treatment of the material leads to precipitation of Ag nanoparticles of a broad size range inside the dielectric as observed by transmission electron microspcopy. Assessment of
4G
5/2 excited state decay in Sm
3+ ions shows no influence from the silver particles. |
---|---|
AbstractList | ► Influence of silver and tin on Sm
3+ luminescence in glass. ► Energy transfer mechanism elucidation and connection with glass structure. ► Effect of Ag nanoparticles on material optical properties.
This work presents the spectroscopic properties of trivalent samarium ions in a melt-quenched aluminophosphate glass containing silver and tin. Addition of 4
mol% of each Ag
2O and SnO into the glass system with 2
mol% Sm
2O
3 results in Sm
3+ ions luminescence under non-resonant UV excitation owing to energy transfer from single silver ions and/or twofold-coordinated Sn centers. Assessment of luminescence spectra and decay dynamics suggest the energy transfer mechanism to be essentially of the resonant radiative type. Moreover, a connection between the luminescent and structural properties of the rare-earth doped glass system was demonstrated. Raman spectroscopy characterization revealed that no significant variation in the glass matrix is induced by Sm
3+ doping at the concentration employed. A comparison was made with a structural study performed on the Eu
3+ doped system (containing 2
mol% Eu
2O
3 along with 4
mol% of each Ag
2O and SnO) where the radiative energy transfer mechanism was previously established. The data appears consistent regarding the lack of variation in glass structure upon the Eu
3+ and Sm
3+ doping in connection with the dominance of the radiative transfer in the matrix. Thermal treatment of the material leads to precipitation of Ag nanoparticles of a broad size range inside the dielectric as observed by transmission electron microspcopy. Assessment of
4G
5/2 excited state decay in Sm
3+ ions shows no influence from the silver particles. This work presents the spectroscopic properties of trivalent samarium ions in a melt-quenched aluminophosphate glass containing silver and tin. Addition of 4 mol% of each Ag sub(2)O and SnO into the glass system with 2 mol% Sm sub(2)O sub(3) results in Sm super(3+) ions luminescence under non-resonant UV excitation owing to energy transfer from single silver ions and/or twofold-coordinated Sn centers. Assessment of luminescence spectra and decay dynamics suggest the energy transfer mechanism to be essentially of the resonant radiative type. Moreover, a connection between the luminescent and structural properties of the rare-earth doped glass system was demonstrated. Raman spectroscopy characterization revealed that no significant variation in the glass matrix is induced by Sm super(3+) doping at the concentration employed. A comparison was made with a structural study performed on the Eu super(3+) doped system (containing 2 mol% Eu sub(2)O sub(3) along with 4 mol% of each Ag sub(2)O and SnO) where the radiative energy transfer mechanism was previously established. The data appears consistent regarding the lack of variation in glass structure upon the Eu super(3+) and Sm super(3+) doping in connection with the dominance of the radiative transfer in the matrix. Thermal treatment of the material leads to precipitation of Ag nanoparticles of a broad size range inside the dielectric as observed by transmission electron microspcopy. Assessment of super(4)G sub(5)/2 excited state decay in Sm super(3+) ions shows no influence from the silver particles. |
Author | Jiménez, José A. Lysenko, Sergiy Sendova, Mariana Liu, Huimin |
Author_xml | – sequence: 1 givenname: José A. surname: Jiménez fullname: Jiménez, José A. email: jjimenez@ncf.edu organization: Division of Natural Sciences, New College of Florida, Sarasota, FL 34243, USA – sequence: 2 givenname: Sergiy surname: Lysenko fullname: Lysenko, Sergiy organization: Department of Physics, University of Puerto Rico, Mayagüez, PR 00681, USA – sequence: 3 givenname: Huimin surname: Liu fullname: Liu, Huimin organization: Department of Physics, University of Puerto Rico, Mayagüez, PR 00681, USA – sequence: 4 givenname: Mariana surname: Sendova fullname: Sendova, Mariana organization: Division of Natural Sciences, New College of Florida, Sarasota, FL 34243, USA |
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Snippet | ► Influence of silver and tin on Sm
3+ luminescence in glass. ► Energy transfer mechanism elucidation and connection with glass structure. ► Effect of Ag... This work presents the spectroscopic properties of trivalent samarium ions in a melt-quenched aluminophosphate glass containing silver and tin. Addition of 4... |
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SubjectTerms | Assessments Dynamics Energy transfer Glass Luminescence Nanoparticles Non-crystalline solids Optical absorption Photoluminescence Rare earth metals Silver Tin |
Title | Luminescence of trivalent samarium ions in silver and tin co-doped aluminophosphate glass |
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