Resistivity, thermopower, and thermal conductivity of nickel doped compounds Cr1−xNixSb2 at low temperatures
▶ Thermoelectric properties of Cr1−xNixSb2 were improved due to the decrease in resistivity and thermal conductivity. ▶ The decrease in resistivity and thermopower of Cr1−xNixSb2 may be due to an increase in electron concentration due to Ni substitution for Cr. ▶ The decrease in thermal conductivity...
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Published in | Journal of alloys and compounds Vol. 509; no. 8; pp. 3677 - 3681 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
24.02.2011
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Abstract | ▶ Thermoelectric properties of Cr1−xNixSb2 were improved due to the decrease in resistivity and thermal conductivity. ▶ The decrease in resistivity and thermopower of Cr1−xNixSb2 may be due to an increase in electron concentration due to Ni substitution for Cr. ▶ The decrease in thermal conductivity of Cr1−xNixSb2 with increasing Ti content could be due to an enhancement of phonon scattering by increased number of Ti atoms. ▶ The Neel temperature of Cr1−xNixSb2 decreased from 273K for CrSb2 to 195K for Cr0.9Ni0.1Sb2, which may be caused by the substitution of the low spin state Ni (3d6) for high spin state Cr (3d2), weakening the effective moment of doping compounds.
Substitutional compounds Cr1−xNixSb2 (0≤x≤0.1) were synthesized, and the effect of Ni substitution on transport and thermoelectric properties of Cr1−xNixSb2 were investigated at the temperatures from 7 to 310K. The results indicated that the magnitudes of the resistivity and thermopower of Cr1−xNixSb2 decreased greatly with increasing Ni content at low temperatures, owing to an increase in electron concentration caused by Ni substitution for Cr. Experiments also showed that the low-temperature lattice thermal conductivity of Cr1−xNixSb2 decreased substantially with increasing Ni content due to an enhancement of phonon scattering by the increased number of Ni atoms. As a result, the figure of merit, ZT, of lightly doped Cr0.99Ni0.01Sb2 was improved at T>∼230K. Specifically, the ZT of Cr0.99Ni0.01Sb2 at 310K was approximately ∼29% larger than that of CrSb2, indicating that thermoelectric properties of CrSb2 can be improved by an appropriate substitution of Ni for Cr. |
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AbstractList | ▶ Thermoelectric properties of Cr1−xNixSb2 were improved due to the decrease in resistivity and thermal conductivity. ▶ The decrease in resistivity and thermopower of Cr1−xNixSb2 may be due to an increase in electron concentration due to Ni substitution for Cr. ▶ The decrease in thermal conductivity of Cr1−xNixSb2 with increasing Ti content could be due to an enhancement of phonon scattering by increased number of Ti atoms. ▶ The Neel temperature of Cr1−xNixSb2 decreased from 273K for CrSb2 to 195K for Cr0.9Ni0.1Sb2, which may be caused by the substitution of the low spin state Ni (3d6) for high spin state Cr (3d2), weakening the effective moment of doping compounds.
Substitutional compounds Cr1−xNixSb2 (0≤x≤0.1) were synthesized, and the effect of Ni substitution on transport and thermoelectric properties of Cr1−xNixSb2 were investigated at the temperatures from 7 to 310K. The results indicated that the magnitudes of the resistivity and thermopower of Cr1−xNixSb2 decreased greatly with increasing Ni content at low temperatures, owing to an increase in electron concentration caused by Ni substitution for Cr. Experiments also showed that the low-temperature lattice thermal conductivity of Cr1−xNixSb2 decreased substantially with increasing Ni content due to an enhancement of phonon scattering by the increased number of Ni atoms. As a result, the figure of merit, ZT, of lightly doped Cr0.99Ni0.01Sb2 was improved at T>∼230K. Specifically, the ZT of Cr0.99Ni0.01Sb2 at 310K was approximately ∼29% larger than that of CrSb2, indicating that thermoelectric properties of CrSb2 can be improved by an appropriate substitution of Ni for Cr. |
Author | Qin, Xiao Ying Li, Di Li, Hai Jin Hu, Jin Lian Liu, Yi |
Author_xml | – sequence: 1 givenname: Hai Jin surname: Li fullname: Li, Hai Jin organization: School of Mathematics and Physics, Anhui University of Technology, Ma’anhan 243002, PR China – sequence: 2 givenname: Xiao Ying surname: Qin fullname: Qin, Xiao Ying email: xyqin@issp.ac.cn organization: Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Science, Hefei 230031, PR China – sequence: 3 givenname: Yi surname: Liu fullname: Liu, Yi organization: School of Mathematics and Physics, Anhui University of Technology, Ma’anhan 243002, PR China – sequence: 4 givenname: Di surname: Li fullname: Li, Di organization: Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Science, Hefei 230031, PR China – sequence: 5 givenname: Jin Lian surname: Hu fullname: Hu, Jin Lian organization: School of Materials Science and Engineering, and Anhui Key Laboratory of Metal Materials and Processing, Anhui University of Technology, Ma’anhan 243002, PR China |
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CitedBy_id | crossref_primary_10_1016_j_eurpolymj_2020_110238 crossref_primary_10_1016_j_jallcom_2011_10_058 crossref_primary_10_1016_j_jssc_2012_06_046 crossref_primary_10_1016_j_physe_2016_04_029 crossref_primary_10_4028_www_scientific_net_AMR_1039_210 |
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Keywords | Thermal conductivity Thermopower Electrical resistivity Cr1−xNixSb2 Temperature dependence Electrical conductivity Transport properties Phonon-phonon interactions Doping Nickel additions Thermoelectric properties Cr Sb Thermoelectric power Electric resistivity Nickel compounds Transport processes Ni Phonon scattering Carrier density Figure of merit Lattice thermal conductivity |
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Snippet | ▶ Thermoelectric properties of Cr1−xNixSb2 were improved due to the decrease in resistivity and thermal conductivity. ▶ The decrease in resistivity and... |
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SubjectTerms | Condensed matter: electronic structure, electrical, magnetic, and optical properties Conductivity of specific materials Cr1−xNixSb2 Electrical resistivity Electronic transport in condensed matter Exact sciences and technology Iii-v and ii-vi semiconductors Physics Thermal conductivity Thermopower |
Title | Resistivity, thermopower, and thermal conductivity of nickel doped compounds Cr1−xNixSb2 at low temperatures |
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