Hybrid photoanode films based on sparse ZnO rod array-TiO2 nanoparticles in dye-sensitized solar cells
ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles. A special surface-coating technique was developed to deposit a thin TiO2 layer on the surface of ZnO rods. Microstructure, optical and photo...
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Published in | Science China. Physics, mechanics & astronomy Vol. 55; no. 7; pp. 1183 - 1188 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
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SP Science China Press
01.07.2012
Springer Nature B.V |
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Abstract | ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles. A special surface-coating technique was developed to deposit a thin TiO2 layer on the surface of ZnO rods. Microstructure, optical and photoelectrochemical performance of the hybrid photoanodes were investi- gated. The denser ZnO array exhibited bad filling behavior of nanoparticles in the interspace of ZnO rods, strong scattering and low conversion efficiency (0.27%). The sparser array showed a much better integrated microstructure, improved transmittance and high conversion efficiency (2.68%). The surface modification of ZnO rods by the TiO2 thin layer was found useful in im- proving the interfacial microstructure between the ZnO rod and the TiO2 bulk film, and the total conversion efficiency of 3.01% was achieved, higher than that of the pure TiO2 nanoparticle cell (2.93%). The increased scattering effects on the inci- dent light, the enhanced electron transportation at TiO2/dye/electrolyte interface, and the inhabited recombination were respon- sible for this improvement. |
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AbstractList | ZnO-TiO
2
hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO
2
nanoparticles. A special surface-coating technique was developed to deposit a thin TiO
2
layer on the surface of ZnO rods. Microstructure, optical and photoelectrochemical performance of the hybrid photoanodes were investigated. The denser ZnO array exhibited bad filling behavior of nanoparticles in the interspace of ZnO rods, strong scattering and low conversion efficiency (0.27%). The sparser array showed a much better integrated microstructure, improved transmittance and high conversion efficiency (2.68%). The surface modification of ZnO rods by the TiO
2
thin layer was found useful in improving the interfacial microstructure between the ZnO rod and the TiO
2
bulk film, and the total conversion efficiency of 3.01% was achieved, higher than that of the pure TiO
2
nanoparticle cell (2.93%). The increased scattering effects on the incident light, the enhanced electron transportation at TiO
2
/dye/electrolyte interface, and the inhabited recombination were responsible for this improvement. ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles. A special surface-coating technique was developed to deposit a thin TiO2 layer on the surface of ZnO rods. Microstructure, optical and photoelectrochemical performance of the hybrid photoanodes were investigated. The denser ZnO array exhibited bad filling behavior of nanoparticles in the interspace of ZnO rods, strong scattering and low conversion efficiency (0.27%). The sparser array showed a much better integrated microstructure, improved transmittance and high conversion efficiency (2.68%). The surface modification of ZnO rods by the TiO2 thin layer was found useful in improving the interfacial microstructure between the ZnO rod and the TiO2 bulk film, and the total conversion efficiency of 3.01% was achieved, higher than that of the pure TiO2 nanoparticle cell (2.93%). The increased scattering effects on the incident light, the enhanced electron transportation at TiO2/dye/electrolyte interface, and the inhabited recombination were responsible for this improvement. ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles. A special surface-coating technique was developed to deposit a thin TiO2 layer on the surface of ZnO rods. Microstructure, optical and photoelectrochemical performance of the hybrid photoanodes were investi- gated. The denser ZnO array exhibited bad filling behavior of nanoparticles in the interspace of ZnO rods, strong scattering and low conversion efficiency (0.27%). The sparser array showed a much better integrated microstructure, improved transmittance and high conversion efficiency (2.68%). The surface modification of ZnO rods by the TiO2 thin layer was found useful in im- proving the interfacial microstructure between the ZnO rod and the TiO2 bulk film, and the total conversion efficiency of 3.01% was achieved, higher than that of the pure TiO2 nanoparticle cell (2.93%). The increased scattering effects on the inci- dent light, the enhanced electron transportation at TiO2/dye/electrolyte interface, and the inhabited recombination were respon- sible for this improvement. |
Author | WANG CaiLu GAO XiangDong LI XiaoMin JIANG ZhengWu YANG ZhengHong GU ZhengYing HE Peng |
AuthorAffiliation | State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China; Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education, Tongji University, Shanghai 200092, China |
Author_xml | – sequence: 1 givenname: CaiLu surname: Wang fullname: Wang, CaiLu organization: State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences – sequence: 2 givenname: XiangDong surname: Gao fullname: Gao, XiangDong email: xdgao@mail.sic.ac.cn organization: State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences – sequence: 3 givenname: XiaoMin surname: Li fullname: Li, XiaoMin organization: State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences – sequence: 4 givenname: ZhengWu surname: Jiang fullname: Jiang, ZhengWu organization: Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education, Tongji University – sequence: 5 givenname: ZhengHong surname: Yang fullname: Yang, ZhengHong organization: Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education, Tongji University – sequence: 6 givenname: ZhengYing surname: Gu fullname: Gu, ZhengYing organization: State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences – sequence: 7 givenname: Peng surname: He fullname: He, Peng organization: State Key Lab of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences |
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CitedBy_id | crossref_primary_10_1080_15533174_2014_988806 crossref_primary_10_1080_15533174_2013_862680 crossref_primary_10_1007_s12598_014_0327_y crossref_primary_10_1007_s12598_014_0329_9 |
Cites_doi | 10.1021/nl101198b 10.1016/S0040-6090(97)00231-9 10.1126/science.1209688 10.1021/cm702286e 10.1016/j.tsf.2010.01.043 10.1016/j.solmat.2006.04.007 10.1039/c1ee01071a 10.1002/adma.200803827 10.1002/adma.201003902 10.1016/j.tsf.2007.05.090 10.1142/S1793604709000508 10.1021/cg7012599 10.1021/cr900356p 10.1038/353737a0 10.1038/nmat1387 10.1021/jp0763073 10.1021/nn901660v |
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Notes | 11-5000/N ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles. A special surface-coating technique was developed to deposit a thin TiO2 layer on the surface of ZnO rods. Microstructure, optical and photoelectrochemical performance of the hybrid photoanodes were investi- gated. The denser ZnO array exhibited bad filling behavior of nanoparticles in the interspace of ZnO rods, strong scattering and low conversion efficiency (0.27%). The sparser array showed a much better integrated microstructure, improved transmittance and high conversion efficiency (2.68%). The surface modification of ZnO rods by the TiO2 thin layer was found useful in im- proving the interfacial microstructure between the ZnO rod and the TiO2 bulk film, and the total conversion efficiency of 3.01% was achieved, higher than that of the pure TiO2 nanoparticle cell (2.93%). The increased scattering effects on the inci- dent light, the enhanced electron transportation at TiO2/dye/electrolyte interface, and the inhabited recombination were respon- sible for this improvement. hybrid photoanode, ZnO, TiO2, dye-sensitized solar cells ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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PublicationTitle | Science China. Physics, mechanics & astronomy |
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Snippet | ZnO-TiO2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO2 nanoparticles.... ZnO-TiO 2 hybrid photoanodes were fabricated via the doctor-blade method by integrating vertically-grown sparse ZnO arrays with hydrothermal TiO 2... |
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SubjectTerms | Arrays Astronomy Classical and Continuum Physics Dye-sensitized solar cells Dyes Efficiency Electrolytic cells Incident light Microstructure Nanoparticles Observations and Techniques Photoanodes Physics Physics and Astronomy Rods Scattering Solar cells TiO2纳米粒子 Titanium dioxide Zinc oxide 染料敏化太阳能电池 氧化锌 混合光 稀疏阵列 纳米TiO2 纳米二氧化钛 阳极膜 |
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Title | Hybrid photoanode films based on sparse ZnO rod array-TiO2 nanoparticles in dye-sensitized solar cells |
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