Morphology of self-assembled merocyanine J-aggregates in films studied by scanning near-field optical microscope
Morphology of 6-methyl merocyanine J-aggregates self-assembled in polyvinyl alcohol (PVA) films by a spin-coating method has been investigated by means of scanning near-field optical microscope and confocal laser scanning microscope. Photoluminescence image measurements show that J-aggregates form d...
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| Published in | Chemical physics letters Vol. 378; no. 1; pp. 47 - 54 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
29.08.2003
Elsevier Science |
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| Abstract | Morphology of 6-methyl merocyanine
J-aggregates self-assembled in polyvinyl alcohol (PVA) films by a spin-coating method has been investigated by means of scanning near-field optical microscope and confocal laser scanning microscope. Photoluminescence image measurements show that
J-aggregates form different domain structures with a grain-shape and a fiber-shape depending on the concentrations of merocyanine and arachidic acid in the PVA film. From the polarization-dependent measurements, we have found that the 6-methyl merocyanine molecules construct a hierarchical structure of
J-aggregates in which a
J-aggregate domain is composed of coherent aggregates with the same transition dipole orientation. |
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| AbstractList | Morphology of 6-methyl merocyanine
J-aggregates self-assembled in polyvinyl alcohol (PVA) films by a spin-coating method has been investigated by means of scanning near-field optical microscope and confocal laser scanning microscope. Photoluminescence image measurements show that
J-aggregates form different domain structures with a grain-shape and a fiber-shape depending on the concentrations of merocyanine and arachidic acid in the PVA film. From the polarization-dependent measurements, we have found that the 6-methyl merocyanine molecules construct a hierarchical structure of
J-aggregates in which a
J-aggregate domain is composed of coherent aggregates with the same transition dipole orientation. |
| Author | Kawasaki, O. Nakamura, A. Yamauchi, T. Hamanaka, Y. |
| Author_xml | – sequence: 1 givenname: Y. surname: Hamanaka fullname: Hamanaka, Y. email: hamanaka@nuap.nagoya-u.ac.jp organization: Department of Applied Physics, Graduate School of Engineering, Nagoya University, Chikusa-ku, Nagoya 464-8603, Japan – sequence: 2 givenname: O. surname: Kawasaki fullname: Kawasaki, O. organization: Department of Applied Physics, Graduate School of Engineering, Nagoya University, Chikusa-ku, Nagoya 464-8603, Japan – sequence: 3 givenname: T. surname: Yamauchi fullname: Yamauchi, T. organization: Core Research for Evolutional Science and Technology (CREST), Japan Science and Technology Corporation (JST), Shibuya-ku, Tokyo 150-0002, Japan – sequence: 4 givenname: A. surname: Nakamura fullname: Nakamura, A. email: nakamura@nuap.nagoya-u.ac.jp organization: Department of Applied Physics, Graduate School of Engineering, Nagoya University, Chikusa-ku, Nagoya 464-8603, Japan |
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| CitedBy_id | crossref_primary_10_1038_nnano_2009_227 crossref_primary_10_1016_j_colsurfa_2005_10_055 crossref_primary_10_1021_jp507791q crossref_primary_10_1021_nl050469y crossref_primary_10_1016_j_colsurfa_2004_10_081 crossref_primary_10_1143_JJAP_44_599 crossref_primary_10_1070_RC2009v078n02ABEH003900 |
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| Keywords | Sulfur nitrogen heterocycle Self-assembly Domain structure Molecular clusters Merocyanine Photoluminescence Rigid solvent Near-field scanning optical microscopy Absorption spectra J-aggregates Experimental study Organic compounds |
| Language | English |
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| Snippet | Morphology of 6-methyl merocyanine
J-aggregates self-assembled in polyvinyl alcohol (PVA) films by a spin-coating method has been investigated by means of... |
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| SubjectTerms | Atomic and molecular clusters Atomic and molecular physics Exact sciences and technology Physics Spectroscopy and geometrical structure of clusters Studies of special atoms, molecules and their ions; clusters |
| Title | Morphology of self-assembled merocyanine J-aggregates in films studied by scanning near-field optical microscope |
| URI | https://dx.doi.org/10.1016/S0009-2614(03)01239-9 |
| Volume | 378 |
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