Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design
•The brightest solution-processed terbium-based OLED was obtained.•The approach towards emitter hole mobility increase by the ligand design was developed.•Recently studied material PO4 was used as a host able to both increase electron mobility and sensitize terbium luminescence.•The role of charge c...
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| Published in | Journal of alloys and compounds Vol. 887; p. 161319 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
20.12.2021
Elsevier BV |
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| Abstract | •The brightest solution-processed terbium-based OLED was obtained.•The approach towards emitter hole mobility increase by the ligand design was developed.•Recently studied material PO4 was used as a host able to both increase electron mobility and sensitize terbium luminescence.•The role of charge carrier mobility was directly demonstrated.
The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes. |
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| AbstractList | •The brightest solution-processed terbium-based OLED was obtained.•The approach towards emitter hole mobility increase by the ligand design was developed.•Recently studied material PO4 was used as a host able to both increase electron mobility and sensitize terbium luminescence.•The role of charge carrier mobility was directly demonstrated.
The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes. The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes. |
| ArticleNumber | 161319 |
| Author | Aslandukov, Andrey N. Medved'ko, Aleksei V. Goloveshkin, Alexander S. Tameev, Alexey R. Vashchenko, Andrey A. Latipov, Egor V. Aleksandrov, Alexey E. Kozlov, Makarii I. Utochnikova, Valentina V. Lypenko, Dmitri A. |
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| Cites_doi | 10.1016/j.jlumin.2007.10.008 10.1107/S0021889802019878 10.1103/PhysRev.127.131 10.1039/C8DT02911C 10.1002/adfm.201603719 10.1016/j.orgel.2011.11.024 10.1016/j.tsf.2013.11.035 10.1146/annurev.biophys.093008.131321 10.1016/j.ccr.2015.02.018 10.1002/aenm.201300954 10.1016/j.ccr.2016.09.012 10.1016/bs.hpcre.2021.05.001 10.3390/molecules24071412 10.1016/j.optmat.2017.02.052 10.1016/j.dyepig.2019.107604 10.1002/ejic.201403071 10.1016/j.orgel.2017.01.026 10.1002/adom.201801536 10.1016/j.jlumin.2018.09.027 10.1016/j.mencom.2019.03.035 10.1002/adma.202004072 10.2116/analsci.7.543 10.1002/adma.19970090308 10.1016/j.mser.2010.01.001 10.1016/j.jlumin.2016.04.017 10.1016/j.jlumin.2018.05.022 10.1002/bio.3423 10.1039/C9DT03823J |
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| Keywords | Thin films Solution-processed OLED Rare earth compounds Aromatic carboxylates Luminescence Charge carrier mobility |
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| Snippet | •The brightest solution-processed terbium-based OLED was obtained.•The approach towards emitter hole mobility increase by the ligand design was... The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore,... |
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| SubjectTerms | Aromatic carboxylates Charge carrier mobility Electroluminescence Electron transport Emitters Hole mobility Ligands Luminescence Rare earth compounds Solution-processed OLED Terbium Thin films Transport properties |
| Title | Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design |
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