The increase of europium-based OLED luminance through reducing the excited state lifetime by mixed-ligand complex formation

An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1 H and 19 F NMR spectrosco...

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Published inPhysical chemistry chemical physics : PCCP Vol. 25; no. 29; pp. 242 - 248
Main Authors Kozlov, Makarii I, Vashchenko, Andrey A, Pavlov, Alexander A, Goloveshkin, Alexander S, Latipov, Egor V, Kuzmina, Natalia P, Utochnikova, Valentina V
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 26.07.2023
Subjects
Complex formation
Europium
Excitation
Ligands
Luminance
NMR spectroscopy
X ray powder diffraction
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Abstract An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1 H and 19 F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes. Mixed-ligand europium complex formation resulted in a significant luminance increase due to the reduction of the lifetime of the excited state.
AbstractList An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, H and F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes.
An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1 H and 19 F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes. Mixed-ligand europium complex formation resulted in a significant luminance increase due to the reduction of the lifetime of the excited state.
An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1H and 19F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes.An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1H and 19F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes.
An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1H and 19F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes.
An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse anionic ligands around one europium ion forming a mixed-ligand complex is confirmed by powder X-ray diffraction, 1 H and 19 F NMR spectroscopy, MALDI MS spectroscopy, and luminescence spectroscopy. A decrease in the symmetry of the coordination environment leads to a 50% reduction of the lifetime of the excited state. The obtained OLEDs based on mixed ligand europium complexes are significantly superior in luminance to OLEDs based on individual complexes.
Author Kozlov, Makarii I
Goloveshkin, Alexander S
Kuzmina, Natalia P
Vashchenko, Andrey A
Pavlov, Alexander A
Utochnikova, Valentina V
Latipov, Egor V
AuthorAffiliation M. V. Lomonosov Moscow State University
BMSTU Center of National Technological Initiative "Digital Material Science: New Material and Substances"
Institute of Nanotechnology of Microelectronics of the Russian Academy of Sciences
P. N. Lebedev Physical Institute
A. N. Nesmeyanov Institute of Organoelement Compounds
Bauman Moscow State Technical University
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Snippet An approach to the luminance increase of the europium-based OLED is proposed through the formation of the mixed-ligand complex. The introduction of two diverse...
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SubjectTerms Complex formation
Europium
Excitation
Ligands
Luminance
NMR spectroscopy
X ray powder diffraction
Title The increase of europium-based OLED luminance through reducing the excited state lifetime by mixed-ligand complex formation
URI https://www.ncbi.nlm.nih.gov/pubmed/37462080
https://www.proquest.com/docview/2841902617
https://www.proquest.com/docview/2839250601
Volume 25
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linkProvider Royal Society of Chemistry
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