Multistimuli-responsive multicolor solid-state luminescence tuned by NH-dependent switchable hydrogen bonds
Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper( i ) complex [{Cu(bpmtzH)} 2 (μ-dppa) 2 ](ClO 4 ) 2 ( 1 ), and the multistimuli...
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| Published in | Dalton transactions : an international journal of inorganic chemistry Vol. 53; no. 1; pp. 339 - 345 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
19.12.2023
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 1477-9226 1477-9234 1477-9234 |
| DOI | 10.1039/d3dt03124a |
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| Abstract | Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(
i
) complex [{Cu(bpmtzH)}
2
(μ-dppa)
2
](ClO
4
)
2
(
1
), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds
1
·2CH
3
COCH
3
·2H
2
O,
1
·2DMSO·2H
2
O,
1
·4CH
3
OH, and
1
·4CH
2
Cl
2
. It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO
4
−
induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N-H ones, to construct switchable hydrogen bonds.
Stimuli-responsive multicolor solid-state luminescence is tuned by NH-dependent switchable hydrogen bonds, in which luminescence vapochromism and mechanochromism are associated with hydrogen bonding with dppa-NH and bpmtzH-NH, respectively. |
|---|---|
| AbstractList | Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(
i
) complex [{Cu(bpmtzH)}
2
(μ-dppa)
2
](ClO
4
)
2
(
1
), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds
1
·2CH
3
COCH
3
·2H
2
O,
1
·2DMSO·2H
2
O,
1
·4CH
3
OH, and
1
·4CH
2
Cl
2
. It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO
4
−
induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N-H ones, to construct switchable hydrogen bonds.
Stimuli-responsive multicolor solid-state luminescence is tuned by NH-dependent switchable hydrogen bonds, in which luminescence vapochromism and mechanochromism are associated with hydrogen bonding with dppa-NH and bpmtzH-NH, respectively. Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(I) complex [{Cu(bpmtzH)} (μ-dppa) ](ClO ) (1), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds 1·2CH COCH ·2H O, 1·2DMSO·2H O, 1·4CH OH, and 1·4CH Cl . It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N-H ones, to construct switchable hydrogen bonds. Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper( i ) complex [{Cu(bpmtzH)} 2 (μ-dppa) 2 ](ClO 4 ) 2 (1), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds 1·2CH 3 COCH 3 ·2H 2 O, 1·2DMSO·2H 2 O, 1·4CH 3 OH, and 1·4CH 2 Cl 2 . It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO 4 − induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N–H ones, to construct switchable hydrogen bonds. Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(I) complex [{Cu(bpmtzH)}2(μ-dppa)2](ClO4)2 (1), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds 1·2CH3COCH3·2H2O, 1·2DMSO·2H2O, 1·4CH3OH, and 1·4CH2Cl2. It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO4- induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N-H ones, to construct switchable hydrogen bonds.Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(I) complex [{Cu(bpmtzH)}2(μ-dppa)2](ClO4)2 (1), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds 1·2CH3COCH3·2H2O, 1·2DMSO·2H2O, 1·4CH3OH, and 1·4CH2Cl2. It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO4- induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N-H ones, to construct switchable hydrogen bonds. Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the multistimuli-responsive multicolor solid-state luminescence of a new dicopper(i) complex [{Cu(bpmtzH)}2(μ-dppa)2](ClO4)2 (1), and the multistimuli-responsive mechanism is clarified by investigating its four different solvated compounds 1·2CH3COCH3·2H2O, 1·2DMSO·2H2O, 1·4CH3OH, and 1·4CH2Cl2. It is shown that luminescence mechanochromism is associated with the breakage of the hydrogen bonds of bmptzH-NH with counter-ions such as ClO4− induced by grinding, while luminescence vapochromism is attributable to the breaking and forming of hydrogen bonds of dppa-NH with solvents, such as acetone, dimethylsulfoxide, and methanol, caused by heating and vapor fuming. In addition, those results might provide new insights into the design and synthesis of multistimuli-responsive multicolor luminescent materials by using various structure-sensitive functional groups, such as distinct N–H ones, to construct switchable hydrogen bonds. |
| Author | Chen, Jing-Lin He, Li-Hua Zhao, Feng Zhang, Rui Liu, Sui-Jun Liao, Jin-Sheng Wen, He-Rui |
| AuthorAffiliation | State Key Laboratory of Structural Chemistry Jiangxi Science and Technology Normal University Jiangxi Provincial Key Laboratory of Functional Molecular Materials Chemistry Chinese Academy of Sciences Jiangxi University of Science and Technology Fujian Institute of Research on the Structure of Matter School of Chemistry and Chemical Engineering |
| AuthorAffiliation_xml | – sequence: 0 name: State Key Laboratory of Structural Chemistry – sequence: 0 name: Jiangxi Science and Technology Normal University – sequence: 0 name: School of Chemistry and Chemical Engineering – sequence: 0 name: Chinese Academy of Sciences – sequence: 0 name: Jiangxi Provincial Key Laboratory of Functional Molecular Materials Chemistry – sequence: 0 name: Fujian Institute of Research on the Structure of Matter – sequence: 0 name: Jiangxi University of Science and Technology |
| Author_xml | – sequence: 1 givenname: Rui surname: Zhang fullname: Zhang, Rui – sequence: 2 givenname: Li-Hua surname: He fullname: He, Li-Hua – sequence: 3 givenname: Sui-Jun surname: Liu fullname: Liu, Sui-Jun – sequence: 4 givenname: Jin-Sheng surname: Liao fullname: Liao, Jin-Sheng – sequence: 5 givenname: He-Rui surname: Wen fullname: Wen, He-Rui – sequence: 6 givenname: Jing-Lin surname: Chen fullname: Chen, Jing-Lin – sequence: 7 givenname: Feng surname: Zhao fullname: Zhao, Feng |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/38050406$$D View this record in MEDLINE/PubMed |
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| CitedBy_id | crossref_primary_10_1002_asia_202400413 crossref_primary_10_1016_j_dyepig_2024_112346 |
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| Snippet | Revealing the stimuli-responsive mechanism is the key to the accurate design of stimuli-responsive luminescent materials. We report herein the... |
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| SubjectTerms | Functional groups Hydrogen bonds Luminescence Solid state Stimuli |
| Title | Multistimuli-responsive multicolor solid-state luminescence tuned by NH-dependent switchable hydrogen bonds |
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