Recent advanced strategies for bimetallenes toward electrocatalytic energy conversion reactions
Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bime...
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| Published in | Chemical communications (Cambridge, England) Vol. 6; no. 23; pp. 3129 - 3137 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
14.03.2024
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bimetallenes present unsaturated surface coordination, high specific surface area and high conductivity, which are all indispensable features for heterogeneous electrochemical reactions. However, the intrinsic activity and stability of bimetallenes needs to be improved further for bimetallene electrocatalysts, due to the higher demands of practical applications. Recently, many strategies have been developed to optimize the chemical or electronic structure to accommodate transfer of reactants, adsorption or desorption of intermediates, and dissociation of products. Considering that most such work focuses on adjusting the structure, this review offers in-depth insight into recent representative strategies for optimizing bimetallene electrocatalysts, mainly including alloying, strain effects, ligand effects, defects and heteroatom doping. Moreover, by summarizing the performance of bimetallenes optimized using various strategies, we provide a means to understand structure-property relationships. In addition, future prospects and challenges are discussed for further development of bimetallene electrocatalysts.
Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. |
|---|---|
| AbstractList | Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bimetallenes present unsaturated surface coordination, high specific surface area and high conductivity, which are all indispensable features for heterogeneous electrochemical reactions. However, the intrinsic activity and stability of bimetallenes needs to be improved further for bimetallene electrocatalysts, due to the higher demands of practical applications. Recently, many strategies have been developed to optimize the chemical or electronic structure to accommodate transfer of reactants, adsorption or desorption of intermediates, and dissociation of products. Considering that most such work focuses on adjusting the structure, this review offers in-depth insight into recent representative strategies for optimizing bimetallene electrocatalysts, mainly including alloying, strain effects, ligand effects, defects and heteroatom doping. Moreover, by summarizing the performance of bimetallenes optimized using various strategies, we provide a means to understand structure-property relationships. In addition, future prospects and challenges are discussed for further development of bimetallene electrocatalysts. Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bimetallenes present unsaturated surface coordination, high specific surface area and high conductivity, which are all indispensable features for heterogeneous electrochemical reactions. However, the intrinsic activity and stability of bimetallenes needs to be improved further for bimetallene electrocatalysts, due to the higher demands of practical applications. Recently, many strategies have been developed to optimize the chemical or electronic structure to accommodate transfer of reactants, adsorption or desorption of intermediates, and dissociation of products. Considering that most such work focuses on adjusting the structure, this review offers in-depth insight into recent representative strategies for optimizing bimetallene electrocatalysts, mainly including alloying, strain effects, ligand effects, defects and heteroatom doping. Moreover, by summarizing the performance of bimetallenes optimized using various strategies, we provide a means to understand structure-property relationships. In addition, future prospects and challenges are discussed for further development of bimetallene electrocatalysts. Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bimetallenes present unsaturated surface coordination, high specific surface area and high conductivity, which are all indispensable features for heterogeneous electrochemical reactions. However, the intrinsic activity and stability of bimetallenes needs to be improved further for bimetallene electrocatalysts, due to the higher demands of practical applications. Recently, many strategies have been developed to optimize the chemical or electronic structure to accommodate transfer of reactants, adsorption or desorption of intermediates, and dissociation of products. Considering that most such work focuses on adjusting the structure, this review offers in-depth insight into recent representative strategies for optimizing bimetallene electrocatalysts, mainly including alloying, strain effects, ligand effects, defects and heteroatom doping. Moreover, by summarizing the performance of bimetallenes optimized using various strategies, we provide a means to understand structure-property relationships. In addition, future prospects and challenges are discussed for further development of bimetallene electrocatalysts.Designing low-dimensional nanomaterials is vital to address the energy and environmental crisis by means of electrocatalytic conversion reactions. Bimetallenes, as an emerging class of 2D materials, present promise for electrocatalytic conversion reactions. By leveraging atomically thin layers, bimetallenes present unsaturated surface coordination, high specific surface area and high conductivity, which are all indispensable features for heterogeneous electrochemical reactions. However, the intrinsic activity and stability of bimetallenes needs to be improved further for bimetallene electrocatalysts, due to the higher demands of practical applications. Recently, many strategies have been developed to optimize the chemical or electronic structure to accommodate transfer of reactants, adsorption or desorption of intermediates, and dissociation of products. Considering that most such work focuses on adjusting the structure, this review offers in-depth insight into recent representative strategies for optimizing bimetallene electrocatalysts, mainly including alloying, strain effects, ligand effects, defects and heteroatom doping. Moreover, by summarizing the performance of bimetallenes optimized using various strategies, we provide a means to understand structure-property relationships. In addition, future prospects and challenges are discussed for further development of bimetallene electrocatalysts. |
| Author | Sanati, Soheila Wang, Qiyou Abazari, Reza Liu, Min |
| AuthorAffiliation | Department of Chemistry Central South University Hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics University of Maragheh Faculty of Science State Key Laboratory of Powder Metallurgy |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/38404151$$D View this record in MEDLINE/PubMed |
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| Notes | Reza Abazari is a senior professor of Chemistry at University of Maragheh, Iran. He obtained his MSc in Inorganic Chemistry from K. N. Toosi University of Technology (Iran) in 2012 and his PhD degree from Tarbiat Modares University in 2019. His research interests include the design and synthesis of nanostructured materials based on crystalline porous frameworks for electrochemical energy storage and photocatalytic applications. Soheila Sanati obtained her PhD degree in Inorganic Chemistry at Azarbaijan Shahid Madani University (Iran) in February 2019. She is currently a postdoctoral fellow at Tarbiat Modares University (Iran). Her research interests mainly focus on the design, synthesis, and applications of advanced materials for energy storage and conversion. 2 Min Liu received his PhD (2010) from the Chinese Academy of Sciences. In 2010-2015, he joined University of Tokyo as a research fellow with Prof. Kazuhito Hashimoto and Prof. Kazunari Domen, separately. In 2015-2017, he joined University of Toronto as a postdoctoral fellow with Prof. Edward Sargent. In 2017, he joined Central South University as a professor. His research focuses on electrocatalytic energy conversion, photo/electrocatalytic CO reduction and the resource utilization of perfluorocarbon. Qiyou Wang received his MS in 2020 from Hunan University. Presently, he is a PhD student under the guidance of Prof. Liu at Central South University. His research interests are mainly design of flow cell electrolysis and study of in situ Raman spectroscopy, FTIR spectroscopy, and XAFS spectra during electrochemical conversion reactions. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 ObjectType-Review-3 content type line 23 |
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