Growth and physical properties of ZnO rod arrays that integrally match the geometries of photoresists with hole sizes larger than rods' habit diameters
Bottom-up and top-down methods can be combined to create well-designed two-dimensional rod arrays for use in optoelectronics. Toward this end, the bottom-up material growth should follow the exact input of the top-down surface patterning, for example, the growth morphologies should integrally match...
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Published in | Journal of alloys and compounds Vol. 704; pp. 131 - 140 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
15.05.2017
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Abstract | Bottom-up and top-down methods can be combined to create well-designed two-dimensional rod arrays for use in optoelectronics. Toward this end, the bottom-up material growth should follow the exact input of the top-down surface patterning, for example, the growth morphologies should integrally match to the geometries of the patterning. Through the repeated use of appropriate amounts of sodium citrate and polyethylenimine, ZnO rod arrays, in which each rod integrally matched with restriction holes in the surfaces, were formed even when the diameters of restriction holes were much larger than the original habit diameters of the ZnO rods. The diameters and lengths of the ZnO rods were varied by adjusting the diameters of photoresist holes, the concentrations of precursors in solution, and the reaction time. This method was successfully extended the diameter of integrally matching growth of ZnO rods to micrometer scale. The effects of the restriction diameters, the concentration of adjuvants, and the crystallinity of the seeds on integrally matching growth of ZnO rods are discussed. The photoluminescence spectra and crystallinities of the ZnO rods produced in different environments were characterized, revealing that a smaller photoresist aperture improved crystallization quality. The photoluminescence spectra of ZnO rods with different growth times and adjuvant concentrations were also explored. Fibrous ZnO/Cu2O heterostructures were successfully synthesized via the growth of ZnO rods. The electrical properties of ZnO/Cu2O and ZnO rods/Si heterojunctions were investigated, and the crystallinities of the ZnO rods were shown to change based on the different synthesis conditions used. This method for the integrally matching growth of ZnO using photoresist patterns was also generalized to ZnO tubes and rings, which individually match to single restriction hole.
•ZnO rods with individual geometry in micrometer scale were formed using photoresist.•Each rod integrally matched with photoresist hole on nonepitaxial substrates.•The crystalline quality of ZnO rods by photoresist was analyzed by PL spectra.•Cu2O/ZnO heterojunctions based on ZnO rods were formed and characterized.•The influence factors on integrally matching growth of ZnO rods were demonstrated. |
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AbstractList | Bottom-up and top-down methods can be combined to create well-designed two-dimensional rod arrays for use in optoelectronics. Toward this end, the bottom-up material growth should follow the exact input of the top-down surface patterning, for example, the growth morphologies should integrally match to the geometries of the patterning. Through the repeated use of appropriate amounts of sodium citrate and polyethylenimine, ZnO rod arrays, in which each rod integrally matched with restriction holes in the surfaces, were formed even when the diameters of restriction holes were much larger than the original habit diameters of the ZnO rods. The diameters and lengths of the ZnO rods were varied by adjusting the diameters of photoresist holes, the concentrations of precursors in solution, and the reaction time. This method was successfully extended the diameter of integrally matching growth of ZnO rods to micrometer scale. The effects of the restriction diameters, the concentration of adjuvants, and the crystallinity of the seeds on integrally matching growth of ZnO rods are discussed. The photoluminescence spectra and crystallinities of the ZnO rods produced in different environments were characterized, revealing that a smaller photoresist aperture improved crystallization quality. The photoluminescence spectra of ZnO rods with different growth times and adjuvant concentrations were also explored. Fibrous ZnO/Cu2O heterostructures were successfully synthesized via the growth of ZnO rods. The electrical properties of ZnO/Cu2O and ZnO rods/Si heterojunctions were investigated, and the crystallinities of the ZnO rods were shown to change based on the different synthesis conditions used. This method for the integrally matching growth of ZnO using photoresist patterns was also generalized to ZnO tubes and rings, which individually match to single restriction hole. Bottom-up and top-down methods can be combined to create well-designed two-dimensional rod arrays for use in optoelectronics. Toward this end, the bottom-up material growth should follow the exact input of the top-down surface patterning, for example, the growth morphologies should integrally match to the geometries of the patterning. Through the repeated use of appropriate amounts of sodium citrate and polyethylenimine, ZnO rod arrays, in which each rod integrally matched with restriction holes in the surfaces, were formed even when the diameters of restriction holes were much larger than the original habit diameters of the ZnO rods. The diameters and lengths of the ZnO rods were varied by adjusting the diameters of photoresist holes, the concentrations of precursors in solution, and the reaction time. This method was successfully extended the diameter of integrally matching growth of ZnO rods to micrometer scale. The effects of the restriction diameters, the concentration of adjuvants, and the crystallinity of the seeds on integrally matching growth of ZnO rods are discussed. The photoluminescence spectra and crystallinities of the ZnO rods produced in different environments were characterized, revealing that a smaller photoresist aperture improved crystallization quality. The photoluminescence spectra of ZnO rods with different growth times and adjuvant concentrations were also explored. Fibrous ZnO/Cu2O heterostructures were successfully synthesized via the growth of ZnO rods. The electrical properties of ZnO/Cu2O and ZnO rods/Si heterojunctions were investigated, and the crystallinities of the ZnO rods were shown to change based on the different synthesis conditions used. This method for the integrally matching growth of ZnO using photoresist patterns was also generalized to ZnO tubes and rings, which individually match to single restriction hole. •ZnO rods with individual geometry in micrometer scale were formed using photoresist.•Each rod integrally matched with photoresist hole on nonepitaxial substrates.•The crystalline quality of ZnO rods by photoresist was analyzed by PL spectra.•Cu2O/ZnO heterojunctions based on ZnO rods were formed and characterized.•The influence factors on integrally matching growth of ZnO rods were demonstrated. |
Author | Fu, Ming Tao, Yinglei He, Dawei Wang, Yongsheng Zhao, Haiyan Wang, Xin |
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Cites_doi | 10.1039/c3ce40734a 10.1039/c2cy00411a 10.1021/jp073806v 10.1002/adfm.201000613 10.1021/cr500002z 10.1016/j.jallcom.2013.04.039 10.1038/nnano.2010.46 10.1021/cg2002755 10.1166/jnn.2012.5195 10.1126/science.1157566 10.1088/0957-4484/18/15/155302 10.1021/am3003473 10.1002/adfm.201501411 10.1088/0957-4484/25/13/135604 10.1021/ph400038g 10.1063/1.2924282 10.1021/cg901223t 10.1063/1.2811717 10.1002/adfm.201201008 10.1021/ja806952j 10.1007/s00339-004-3114-z 10.1039/c3ee43278e 10.1021/cm802839u 10.1093/nsr/nwt002 10.1002/adma.200701203 10.1002/adma.200600257 10.1021/nl035102c 10.1039/C4RA12889C |
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Snippet | Bottom-up and top-down methods can be combined to create well-designed two-dimensional rod arrays for use in optoelectronics. Toward this end, the bottom-up... |
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SubjectTerms | Adjuvants Arrays Copper oxides Crystallization Cuprous oxide Electrical properties Heterojunctions Heterostructures Hydrothermal Integrally match Matching Optoelectronics Photoluminescence Photoresist Photoresists Physical properties Polyethyleneimine Reaction time Rods Seeds Sodium citrate Tubes Zinc oxide Zinc oxides |
Title | Growth and physical properties of ZnO rod arrays that integrally match the geometries of photoresists with hole sizes larger than rods' habit diameters |
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