A palladium-catalyzed sequential Heck coupling/C-C bond activation approach to oxindoles with all-carbon-quaternary centers
Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. Herein, we report a palladium-catalyzed sequential Heck coupling/C-C bond activation of aryl halide-tethered alkenes with benzocyclobutenols affording a series of...
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Published in | Organic & biomolecular chemistry Vol. 2; no. 8; pp. 1642 - 1646 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
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Royal Soc Chemistry
23.02.2022
Royal Society of Chemistry |
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Abstract | Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. Herein, we report a palladium-catalyzed sequential Heck coupling/C-C bond activation of aryl halide-tethered alkenes with benzocyclobutenols affording a series of oxindole-derived compounds in good to excellent yields, as well as the preliminary enantioselectivity results.
Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. |
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AbstractList | Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. Herein, we report a palladium-catalyzed sequential Heck coupling/C–C bond activation of aryl halide-tethered alkenes with benzocyclobutenols affording a series of oxindole-derived compounds in good to excellent yields, as well as the preliminary enantioselectivity results. Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. Herein, we report a palladium-catalyzed sequential Heck coupling/C-C bond activation of aryl halide-tethered alkenes with benzocyclobutenols affording a series of oxindole-derived compounds in good to excellent yields, as well as the preliminary enantioselectivity results. Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. |
Author | Gao, Yuan-Yuan Mao, Guoliang Liu, Lantao Wu, Wenbo Meng, Chenxiang Cheng, Fangyuan Li, Gao-Wei |
AuthorAffiliation | College of Chemistry Provincial Key Laboratory of Oil and Gas Chemical Technology Henan Engineering Laboratory of Green Synthesis for Pharmaceuticals Shangqiu Normal University College of Chemistry and Chemical Engineering Northeast Petroleum University Zhengzhou University |
AuthorAffiliation_xml | – name: Provincial Key Laboratory of Oil and Gas Chemical Technology – name: Zhengzhou University – name: College of Chemistry and Chemical Engineering – name: Northeast Petroleum University – name: Henan Engineering Laboratory of Green Synthesis for Pharmaceuticals – name: College of Chemistry – name: Shangqiu Normal University |
Author_xml | – sequence: 1 givenname: Guoliang surname: Mao fullname: Mao, Guoliang – sequence: 2 givenname: Chenxiang surname: Meng fullname: Meng, Chenxiang – sequence: 3 givenname: Fangyuan surname: Cheng fullname: Cheng, Fangyuan – sequence: 4 givenname: Wenbo surname: Wu fullname: Wu, Wenbo – sequence: 5 givenname: Yuan-Yuan surname: Gao fullname: Gao, Yuan-Yuan – sequence: 6 givenname: Gao-Wei surname: Li fullname: Li, Gao-Wei – sequence: 7 givenname: Lantao surname: Liu fullname: Liu, Lantao |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35108719$$D View this record in MEDLINE/PubMed |
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Keywords | FUNCTIONALIZATION INSERTION ASYMMETRIC-SYNTHESIS RING-FUSED BENZOCYCLOBUTENOLS CONSTRUCTION SITE-SELECTIVITY PHYSOSTIGMINE CLEAVAGE ENANTIOMER H ACTIVATION |
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Snippet | Catalytic construction of oxindoles bearing all-carbon-quaternary centers attracts wide attention from the synthetic chemistry community. Herein, we report a... |
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SubjectTerms | Alkenes Carbon Chemistry Chemistry, Organic Coupling Covalent bonds Enantiomers Palladium Physical Sciences Science & Technology |
Title | A palladium-catalyzed sequential Heck coupling/C-C bond activation approach to oxindoles with all-carbon-quaternary centers |
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