Vertical recrystallization for highly efficient and stable formamidinium-based inverted-structure perovskite solar cells
Formamidinium (FA)-based perovskite materials show an extended absorption spectrum to 840 nm, which enables high power conversion efficiencies of over 20% compared with normal-structure perovskite solar cells (PSCs). However, it is rarely possible to obtain high performance in inverted-structure PSC...
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| Published in | Energy & environmental science Vol. 10; no. 9; pp. 1942 - 1949 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
2017
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| Online Access | Get full text |
| ISSN | 1754-5692 1754-5706 |
| DOI | 10.1039/C7EE01675A |
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| Abstract | Formamidinium (FA)-based perovskite materials show an extended absorption spectrum to 840 nm, which enables high power conversion efficiencies of over 20% compared with normal-structure perovskite solar cells (PSCs). However, it is rarely possible to obtain high performance in inverted-structure PSCs owing to the unbalanced electron–hole transport properties. To achieve desirable electronic qualities in a FA perovskite film, it is necessary to substantially improve the crystallinity of the perovskite films. A new perovskite growth method is presented here using methylammonium chloride (MACl) to assist vertical recrystallization in a formamidinium perovskite film. The obtained film consists of highly crystallized vertically-orientated grains, which minimize the vertical grain boundary and trap site in the films, and later contribute to a power conversion efficiency above 20% in inverted-structure PSCs. Most importantly, the highly crystalline, phase-pure morphology and low MA content in formamidinium perovskite films can contribute to the light-soaking stability and thermal stability up to 500 h in solar-cell devices. |
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| AbstractList | Formamidinium (FA)-based perovskite materials show an extended absorption spectrum to 840 nm, which enables high power conversion efficiencies of over 20% compared with normal-structure perovskite solar cells (PSCs). However, it is rarely possible to obtain high performance in inverted-structure PSCs owing to the unbalanced electron–hole transport properties. To achieve desirable electronic qualities in a FA perovskite film, it is necessary to substantially improve the crystallinity of the perovskite films. A new perovskite growth method is presented here using methylammonium chloride (MACl) to assist vertical recrystallization in a formamidinium perovskite film. The obtained film consists of highly crystallized vertically-orientated grains, which minimize the vertical grain boundary and trap site in the films, and later contribute to a power conversion efficiency above 20% in inverted-structure PSCs. Most importantly, the highly crystalline, phase-pure morphology and low MA content in formamidinium perovskite films can contribute to the light-soaking stability and thermal stability up to 500 h in solar-cell devices. |
| Author | Wu, Yongzhen Cai, Molang Yang, Xudong Xie, Fengxian Li, Xing Chen, Chun-Chao Han, Liyuan Liu, Xiao |
| Author_xml | – sequence: 1 givenname: Fengxian orcidid: 0000-0002-6274-9290 surname: Xie fullname: Xie, Fengxian organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan – sequence: 2 givenname: Chun-Chao surname: Chen fullname: Chen, Chun-Chao organization: State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, 800 Dong Chuan RD, Shanghai 200240, China – sequence: 3 givenname: Yongzhen surname: Wu fullname: Wu, Yongzhen organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan – sequence: 4 givenname: Xing surname: Li fullname: Li, Xing organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan – sequence: 5 givenname: Molang surname: Cai fullname: Cai, Molang organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan – sequence: 6 givenname: Xiao surname: Liu fullname: Liu, Xiao organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan – sequence: 7 givenname: Xudong orcidid: 0000-0002-7398-4229 surname: Yang fullname: Yang, Xudong organization: State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, 800 Dong Chuan RD, Shanghai 200240, China – sequence: 8 givenname: Liyuan orcidid: 0000-0001-9766-9015 surname: Han fullname: Han, Liyuan organization: Research Network and Facility Services Division, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan |
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