Stable high efficiency two-dimensional perovskite solar cells via cesium doping
Two-dimensional (2D) organic–inorganic perovskites have recently emerged as one of the most important thin-film solar cell materials owing to their excellent environmental stability. The remaining major pitfall is their relatively poor photovoltaic performance in contrast to 3D perovskites. In this...
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| Published in | Energy & environmental science Vol. 10; no. 10; pp. 2095 - 2102 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
2017
|
| Online Access | Get full text |
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| Abstract | Two-dimensional (2D) organic–inorganic perovskites have recently emerged as one of the most important thin-film solar cell materials owing to their excellent environmental stability. The remaining major pitfall is their relatively poor photovoltaic performance in contrast to 3D perovskites. In this work we demonstrate cesium cation (Cs
+
) doped 2D (BA)
2
(MA)
3
Pb
4
I
13
perovskite solar cells giving a power conversion efficiency (PCE) as high as 13.7%, the highest among the reported 2D devices, with excellent humidity resistance. The enhanced efficiency from 12.3% (without Cs
+
) to 13.7% (with 5% Cs
+
) is attributed to perfectly controlled crystal orientation, an increased grain size of the 2D planes, superior surface quality, reduced trap-state density, enhanced charge-carrier mobility and charge-transfer kinetics. Surprisingly, it is found that the Cs
+
doping yields superior stability for the 2D perovskite solar cells when subjected to a high humidity environment without encapsulation. The device doped using 5% Cs
+
degrades only
ca.
10% after 1400 hours of exposure in 30% relative humidity (RH), and exhibits significantly improved stability under heating and high moisture environments. Our results provide an important step toward air-stable and fully printable low dimensional perovskites as a next-generation renewable energy source. |
|---|---|
| AbstractList | Two-dimensional (2D) organic–inorganic perovskites have recently emerged as one of the most important thin-film solar cell materials owing to their excellent environmental stability. The remaining major pitfall is their relatively poor photovoltaic performance in contrast to 3D perovskites. In this work we demonstrate cesium cation (Cs
+
) doped 2D (BA)
2
(MA)
3
Pb
4
I
13
perovskite solar cells giving a power conversion efficiency (PCE) as high as 13.7%, the highest among the reported 2D devices, with excellent humidity resistance. The enhanced efficiency from 12.3% (without Cs
+
) to 13.7% (with 5% Cs
+
) is attributed to perfectly controlled crystal orientation, an increased grain size of the 2D planes, superior surface quality, reduced trap-state density, enhanced charge-carrier mobility and charge-transfer kinetics. Surprisingly, it is found that the Cs
+
doping yields superior stability for the 2D perovskite solar cells when subjected to a high humidity environment without encapsulation. The device doped using 5% Cs
+
degrades only
ca.
10% after 1400 hours of exposure in 30% relative humidity (RH), and exhibits significantly improved stability under heating and high moisture environments. Our results provide an important step toward air-stable and fully printable low dimensional perovskites as a next-generation renewable energy source. |
| Author | Munir, Rahim Zhao, Kui Liu, Shengzhong (Frank) Zhang, Xu Liu, Yucheng Yang, Dong Li, Ruipeng Wang, Xiuli Zhu, Xuejie Liu, Bin Niu, Tianqi Ren, Xiaodong Yang, Zhou Li, Jianbo Amassian, Aram Smilgies, Detlef-M. |
| Author_xml | – sequence: 1 givenname: Xu surname: Zhang fullname: Zhang, Xu organization: Dalian National Laboratory for Clean Energy, iChEM, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian – sequence: 2 givenname: Xiaodong surname: Ren fullname: Ren, Xiaodong organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 3 givenname: Bin surname: Liu fullname: Liu, Bin organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 4 givenname: Rahim orcidid: 0000-0002-6029-3760 surname: Munir fullname: Munir, Rahim organization: King Abdullah University of Science and Technology (KAUST), KAUST Solar Center (KSC) and Physical Science and Engineering Division (PSE), Thuwal 23955-6900, Saudi Arabia – sequence: 5 givenname: Xuejie surname: Zhu fullname: Zhu, Xuejie organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 6 givenname: Dong surname: Yang fullname: Yang, Dong organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 7 givenname: Jianbo surname: Li fullname: Li, Jianbo organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 8 givenname: Yucheng surname: Liu fullname: Liu, Yucheng organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 9 givenname: Detlef-M. orcidid: 0000-0001-9351-581X surname: Smilgies fullname: Smilgies, Detlef-M. organization: Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, USA – sequence: 10 givenname: Ruipeng surname: Li fullname: Li, Ruipeng organization: Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, USA – sequence: 11 givenname: Zhou surname: Yang fullname: Yang, Zhou organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 12 givenname: Tianqi surname: Niu fullname: Niu, Tianqi organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 13 givenname: Xiuli surname: Wang fullname: Wang, Xiuli organization: Dalian National Laboratory for Clean Energy, iChEM, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian – sequence: 14 givenname: Aram surname: Amassian fullname: Amassian, Aram organization: King Abdullah University of Science and Technology (KAUST), KAUST Solar Center (KSC) and Physical Science and Engineering Division (PSE), Thuwal 23955-6900, Saudi Arabia – sequence: 15 givenname: Kui orcidid: 0000-0002-9512-0405 surname: Zhao fullname: Zhao, Kui organization: Key Laboratory of Applied Surface and Colloid Chemistry, National Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering – sequence: 16 givenname: Shengzhong (Frank) orcidid: 0000-0002-6338-852X surname: Liu fullname: Liu, Shengzhong (Frank) organization: Dalian National Laboratory for Clean Energy, iChEM, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian |
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