2D Bi2WO6/MoS2 as a new photo-activated carrier for boosting electrocatalytic methanol oxidation with visible light illumination
A kind of new 2D heterojunction of Bi2WO6/MoS2 was constructed and used as visible-light activated carrier for depositing Pt electrocatalyst. With assistance of visible light irradiation, Pt-Bi2WO6/MoS2 composite shows enhanced electrocatalytic activity and stability towards methanol oxidation than...
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| Published in | Chinese chemical letters Vol. 30; no. 12; pp. 2338 - 2342 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.12.2019
School of Environment, Jinan University, Guangzhou 510632, China School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China%School of Environment, Jinan University, Guangzhou 510632, China%School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China |
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| Abstract | A kind of new 2D heterojunction of Bi2WO6/MoS2 was constructed and used as visible-light activated carrier for depositing Pt electrocatalyst. With assistance of visible light irradiation, Pt-Bi2WO6/MoS2 composite shows enhanced electrocatalytic activity and stability towards methanol oxidation than traditional electrocatalytic process and commercial Pt/C.
[Display omitted]
In this paper, a new two-dimensional (2D)/2D composite of Bi2WO6/MoS2 was facile synthesized, and then was used as supporting material for depositing Pt nanoparticles. The as-synthesized Pt-Bi2WO6/MoS2 was extended into photo-assisted electrocatalytic oxidation of methanol, which is a model anode reaction for direct methanol fuel cell. Compare with traditional electrocatalytic process, Pt-Bi2WO6/MoS2 displays 1.5 times enhanced electrocatalytic performance on methanol oxidation with assistance of visible light irradiation and 2.2 times for commercial Pt/C. Besides, from the results of chronoamperometric and chronopotentiometry experiments, the stability of Pt-Bi2WO6/MoS2 electrode is clearly improved under visible light irradiation. The synergistic effects of photo- and electro-catalytic in the heterojunction of Pt-Bi2WO6/MoS2 in favor of the above enhancement. This research gives more insights in the fields of photo-assisted traditional electrocatalytic application by constructing of semiconductor heterojunction carrier. |
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| AbstractList | In this paper, a new two-dimensional (2D)/2D composite of Bi2WO6/MoS2 was facile synthesized, and then was used as supporting material for depositing Pt nanoparticles. The as-synthesized Pt-Bi2WO6/MoS2 was extended into photo-assisted electrocatalytic oxidation of methanol, which is a model anode reaction for direct methanol fuel cell. Compare with traditional electrocatalytic process, Pt-Bi2WO6/MoS2 displays 1.5 times enhanced electrocatalytic performance on methanol oxidation with assistance of visible light irradiation and 2.2 times for commercial Pt/C. Besides, from the results of chronoamperometric and chronopotentiometry experiments, the stability of Pt-Bi2WO6/MoS2 electrode is clearly improved under visible light irradiation. The synergistic effects of photo-and electro-catalytic in the heterojunction of Pt-Bi2WO6/MoS2 in favor of the above enhancement. This research gives more insights in the fields of photo-assisted traditional electrocatalytic application by constructing of semiconductor heterojunction carrier. A kind of new 2D heterojunction of Bi2WO6/MoS2 was constructed and used as visible-light activated carrier for depositing Pt electrocatalyst. With assistance of visible light irradiation, Pt-Bi2WO6/MoS2 composite shows enhanced electrocatalytic activity and stability towards methanol oxidation than traditional electrocatalytic process and commercial Pt/C. [Display omitted] In this paper, a new two-dimensional (2D)/2D composite of Bi2WO6/MoS2 was facile synthesized, and then was used as supporting material for depositing Pt nanoparticles. The as-synthesized Pt-Bi2WO6/MoS2 was extended into photo-assisted electrocatalytic oxidation of methanol, which is a model anode reaction for direct methanol fuel cell. Compare with traditional electrocatalytic process, Pt-Bi2WO6/MoS2 displays 1.5 times enhanced electrocatalytic performance on methanol oxidation with assistance of visible light irradiation and 2.2 times for commercial Pt/C. Besides, from the results of chronoamperometric and chronopotentiometry experiments, the stability of Pt-Bi2WO6/MoS2 electrode is clearly improved under visible light irradiation. The synergistic effects of photo- and electro-catalytic in the heterojunction of Pt-Bi2WO6/MoS2 in favor of the above enhancement. This research gives more insights in the fields of photo-assisted traditional electrocatalytic application by constructing of semiconductor heterojunction carrier. |
| Author | He, Jie Zhai, Chunyang Zhang, Hongmin Zhu, Mingshan |
| AuthorAffiliation | School of Environment, Jinan University, Guangzhou 510632, China;School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China%School of Environment, Jinan University, Guangzhou 510632, China%School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China |
| AuthorAffiliation_xml | – name: School of Environment, Jinan University, Guangzhou 510632, China;School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China%School of Environment, Jinan University, Guangzhou 510632, China%School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China |
| Author_xml | – sequence: 1 givenname: Hongmin surname: Zhang fullname: Zhang, Hongmin organization: School of Environment, Jinan University, Guangzhou 510632, China – sequence: 2 givenname: Jie surname: He fullname: He, Jie organization: School of Environment, Jinan University, Guangzhou 510632, China – sequence: 3 givenname: Chunyang surname: Zhai fullname: Zhai, Chunyang organization: School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China – sequence: 4 givenname: Mingshan surname: Zhu fullname: Zhu, Mingshan email: zhumingshan@jnu.edu.cn organization: School of Environment, Jinan University, Guangzhou 510632, China |
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| Keywords | Electrocatalysis Visible light Bi2WO6 MoS2 Methanol oxidation |
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| Publisher | Elsevier B.V School of Environment, Jinan University, Guangzhou 510632, China School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China%School of Environment, Jinan University, Guangzhou 510632, China%School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China |
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| Snippet | A kind of new 2D heterojunction of Bi2WO6/MoS2 was constructed and used as visible-light activated carrier for depositing Pt electrocatalyst. With assistance... In this paper, a new two-dimensional (2D)/2D composite of Bi2WO6/MoS2 was facile synthesized, and then was used as supporting material for depositing Pt... |
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| SubjectTerms | Bi2WO6 Electrocatalysis Methanol oxidation MoS2 Visible light |
| Title | 2D Bi2WO6/MoS2 as a new photo-activated carrier for boosting electrocatalytic methanol oxidation with visible light illumination |
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