Visible light promoted Fe3S4 Fenton oxidation of atrazine
[Display omitted] •Visible light could promote Fe3S4 Fenton oxidation of atrazine by 4.9 times.•The promoted activity was attributed to the efficient surface iron redox cycle.•The efficient surface iron redox cycle was triggered by visible light.•The formation of FeOOH accounted for poor Fenton acti...
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| Published in | Applied catalysis. B, Environmental Vol. 277; p. 119229 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.11.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Visible light could promote Fe3S4 Fenton oxidation of atrazine by 4.9 times.•The promoted activity was attributed to the efficient surface iron redox cycle.•The efficient surface iron redox cycle was triggered by visible light.•The formation of FeOOH accounted for poor Fenton activity of Fe3S4 in dark.•Visible light excited Fe3S4 to produce photo-generated electrons and O2−.
We demonstrate that visible light irradiation can promote Fe3S4 Fenton oxidation of atrazine. The visible light irradiation could increase the atrazine Fenton degradation rate by 4.9 times. The enhanced atrazine degradation activity under visible light was attributed to the higher surficial Fe(II)/Fe(III) ratio of Fe3S4 and the efficient surface iron redox cycle triggered by visible light. Experimental results revealed that the operando formation of FeOOH on the Fe3S4 surface blocked the iron redox cycle and inhibited the H2O2 decomposition, accounting for the largely decreased Fenton activity of Fe3S4 in dark, while these problems were successfully solved by the introduction of visible light irradiation, which excite Fe3S4 to produce abundant photo-generated electrons and O2− for efficient regeneration of active Fe(II) species of Fe3S4 and in-situ formed FeOOH. |
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| AbstractList | We demonstrate that visible light irradiation can promote Fe3S4 Fenton oxidation of atrazine. The visible light irradiation could increase the atrazine Fenton degradation rate by 4.9 times. The enhanced atrazine degradation activity under visible light was attributed to the higher surficial Fe(II)/Fe(III) ratio of Fe3S4 and the efficient surface iron redox cycle triggered by visible light. Experimental results revealed that the operando formation of FeOOH on the Fe3S4 surface blocked the iron redox cycle and inhibited the H2O2 decomposition, accounting for the largely decreased Fenton activity of Fe3S4 in dark, while these problems were successfully solved by the introduction of visible light irradiation, which excite Fe3S4 to produce abundant photo-generated electrons and ·O2− for efficient regeneration of active Fe(II) species of Fe3S4 and in-situ formed FeOOH. [Display omitted] •Visible light could promote Fe3S4 Fenton oxidation of atrazine by 4.9 times.•The promoted activity was attributed to the efficient surface iron redox cycle.•The efficient surface iron redox cycle was triggered by visible light.•The formation of FeOOH accounted for poor Fenton activity of Fe3S4 in dark.•Visible light excited Fe3S4 to produce photo-generated electrons and O2−. We demonstrate that visible light irradiation can promote Fe3S4 Fenton oxidation of atrazine. The visible light irradiation could increase the atrazine Fenton degradation rate by 4.9 times. The enhanced atrazine degradation activity under visible light was attributed to the higher surficial Fe(II)/Fe(III) ratio of Fe3S4 and the efficient surface iron redox cycle triggered by visible light. Experimental results revealed that the operando formation of FeOOH on the Fe3S4 surface blocked the iron redox cycle and inhibited the H2O2 decomposition, accounting for the largely decreased Fenton activity of Fe3S4 in dark, while these problems were successfully solved by the introduction of visible light irradiation, which excite Fe3S4 to produce abundant photo-generated electrons and O2− for efficient regeneration of active Fe(II) species of Fe3S4 and in-situ formed FeOOH. |
| ArticleNumber | 119229 |
| Author | Ling, Cancan Zhang, Lizhi Shen, Wenjuan Liu, Xiufan Shi, Yanbiao Wang, Xiaobing |
| Author_xml | – sequence: 1 givenname: Yanbiao surname: Shi fullname: Shi, Yanbiao organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China – sequence: 2 givenname: Xiaobing surname: Wang fullname: Wang, Xiaobing organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China – sequence: 3 givenname: Xiufan surname: Liu fullname: Liu, Xiufan organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China – sequence: 4 givenname: Cancan surname: Ling fullname: Ling, Cancan organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China – sequence: 5 givenname: Wenjuan surname: Shen fullname: Shen, Wenjuan organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China – sequence: 6 givenname: Lizhi orcidid: 0000-0002-6842-9167 surname: Zhang fullname: Zhang, Lizhi email: zhanglz@mail.ccnu.edu.cn organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, Central China Normal University, Wuhan 430079, PR China |
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•Visible light could promote Fe3S4 Fenton oxidation of atrazine by 4.9 times.•The promoted activity was attributed to the efficient surface... We demonstrate that visible light irradiation can promote Fe3S4 Fenton oxidation of atrazine. The visible light irradiation could increase the atrazine Fenton... |
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| SubjectTerms | Atrazine Atrazine degradation Degradation Herbicides Heterogeneous Fenton reaction Hydrogen peroxide Iron Iron sulfides Irradiation Light Light irradiation Oxidation Radiation Regeneration Reusability Surface iron redox cycle Visible light irradiation |
| Title | Visible light promoted Fe3S4 Fenton oxidation of atrazine |
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