High-performance CH3NH3PbI3 inverted planar perovskite solar cells via ammonium halide additives
[Display omitted] Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate for use as light-absorbing materials in high-efficiency, low-cost and solution-processable photovoltaic devices owing to their excellent optoelectronic properties. Here, we fabrica...
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| Published in | Journal of industrial and engineering chemistry (Seoul, Korea) Vol. 80; pp. 265 - 272 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.12.2019
한국공업화학회 |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate for use as light-absorbing materials in high-efficiency, low-cost and solution-processable photovoltaic devices owing to their excellent optoelectronic properties. Here, we fabricated inverted planar perovskite solar cells by incorporating small amounts of ammonium halide NH4X (X=F, Cl, Br, I) additives into a CH3NH3PbI3 (MAPbI3) perovskite solution. A compact and uniform perovskite absorber layer with large perovskite crystalline grains is realized by simply incorporating small amounts of additives and by using an anti-solvent engineering technique to control the nucleation and crystal growth of perovskite. The enlarged perovskite grain size with a reduced density of the grain boundaries and improved crystallinity results in fewer charge carrier recombinations and a reduced defect density, leading to enhanced device efficiency (NH4F: 14.88±0.33%, NH4Cl: 16.63±0.21%, NH4Br: 16.64±0.35%, and NH4I: 17.28±0.15%) compared to that of a reference MAPbI3 device (Ref.: 12.95±0.48%) and greater device stability. This simple technique involving the introduction of small amounts of ammonium halide additives to regulate the nucleation and crystal growth of perovskite films translates into highly reproducible enhanced device performance. |
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| AbstractList | Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate foruse as light-absorbing materials in high-efficiency, low-cost and solution-processable photovoltaicdevices owing to their excellent optoelectronic properties. Here, we fabricated inverted planar perovskitesolar cells by incorporating small amounts of ammonium halide NH4X (X = F, Cl, Br, I) additives into aCH3NH3PbI3 (MAPbI3) perovskite solution. A compact and uniform perovskite absorber layer with largeperovskite crystalline grains is realized by simply incorporating small amounts of additives and by usingan anti-solvent engineering technique to control the nucleation and crystal growth of perovskite. Theenlarged perovskite grain size with a reduced density of the grain boundaries and improved crystallinityresults in fewer charge carrier recombinations and a reduced defect density, leading to enhanced deviceefficiency (NH4F: 14.88
0.33%, NH4Cl: 16.63
0.21%, NH4Br: 16.64
0.35%, and NH4I: 17.28
0.15%)compared to that of a reference MAPbI3 device (Ref.: 12.95
0.48%) and greater device stability. Thissimple technique involving the introduction of small amounts of ammonium halide additives to regulatethe nucleation and crystal growth of perovskitefilms translates into highly reproducible enhanced deviceperformance. KCI Citation Count: 2 [Display omitted] Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate for use as light-absorbing materials in high-efficiency, low-cost and solution-processable photovoltaic devices owing to their excellent optoelectronic properties. Here, we fabricated inverted planar perovskite solar cells by incorporating small amounts of ammonium halide NH4X (X=F, Cl, Br, I) additives into a CH3NH3PbI3 (MAPbI3) perovskite solution. A compact and uniform perovskite absorber layer with large perovskite crystalline grains is realized by simply incorporating small amounts of additives and by using an anti-solvent engineering technique to control the nucleation and crystal growth of perovskite. The enlarged perovskite grain size with a reduced density of the grain boundaries and improved crystallinity results in fewer charge carrier recombinations and a reduced defect density, leading to enhanced device efficiency (NH4F: 14.88±0.33%, NH4Cl: 16.63±0.21%, NH4Br: 16.64±0.35%, and NH4I: 17.28±0.15%) compared to that of a reference MAPbI3 device (Ref.: 12.95±0.48%) and greater device stability. This simple technique involving the introduction of small amounts of ammonium halide additives to regulate the nucleation and crystal growth of perovskite films translates into highly reproducible enhanced device performance. |
| Author | Khan, Nasir Shin, Won Suk Lee, Hang Ken Lee, Jong-Cheol Song, Chang Eun Jahankhan, Muhammad Jahandar, Muhammad Lee, Sang Kyu Moon, Sang-Jin Im, Sang Hyuk |
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| CitedBy_id | crossref_primary_10_1016_j_jiec_2022_11_013 crossref_primary_10_1016_j_mtener_2021_100847 crossref_primary_10_1002_eem2_12582 crossref_primary_10_1039_D3RA05857C crossref_primary_10_1016_j_mtener_2021_100837 crossref_primary_10_3390_cryst11070814 crossref_primary_10_1038_s41598_023_39189_0 crossref_primary_10_1080_10667857_2023_2254137 crossref_primary_10_1021_acsami_1c19546 crossref_primary_10_1016_j_jiec_2020_11_010 crossref_primary_10_1016_j_solener_2019_11_098 crossref_primary_10_1016_j_jiec_2020_06_006 crossref_primary_10_1016_j_dib_2019_104817 crossref_primary_10_1002_solr_202200631 crossref_primary_10_1515_ntrev_2022_0547 crossref_primary_10_1016_j_orgel_2022_106549 crossref_primary_10_1007_s12034_021_02625_w crossref_primary_10_1016_j_jiec_2021_05_001 crossref_primary_10_1016_j_jallcom_2020_157320 |
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| Keywords | Ammonium halide additives CH3NH3PbI3perovskite Inverted planar structure Anti-Solvent engineering Perovskite grain size |
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Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate for use as light-absorbing materials in... Organic-inorganic hybrid perovskites have recently attracted substantial attention as a top candidate foruse as light-absorbing materials in high-efficiency,... |
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| SubjectTerms | Ammonium halide additives Anti-Solvent engineering CH3NH3PbI3perovskite Inverted planar structure Perovskite grain size 화학공학 |
| Title | High-performance CH3NH3PbI3 inverted planar perovskite solar cells via ammonium halide additives |
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