Insight into the effect of bromine on facet-dependent surface oxygen vacancies construction and stabilization of Bi2MoO6 for efficient photocatalytic NO removal
Benefiting from the Br− selectively induced the OVs on {001} facets of Bi2MoO6, an extended light-absorption until near-infrared region and enhanced the molecular oxygen activation were achieved, thus endowing the OVs concentration optimized Bi2MoO6 with superior activity and selectivity of NO remov...
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| Published in | Applied catalysis. B, Environmental Vol. 265; p. 118585 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.05.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Benefiting from the Br− selectively induced the OVs on {001} facets of Bi2MoO6, an extended light-absorption until near-infrared region and enhanced the molecular oxygen activation were achieved, thus endowing the OVs concentration optimized Bi2MoO6 with superior activity and selectivity of NO removal in a flow reaction.
[Display omitted]
•Br− boost the construction and stabilization of OVs on {001} facets of Bi2MoO6.•Br− induced OVs facilitate NO removal of BMO-001-Br even in near-infrared region.•NO oxidative removal with high selectivity of 93.6% is achieved on BMO-001-Br.•Mechanism for highly efficient NO removal (62.9%) over BMO-001-Br is proposed.
Surface oxygen vacancies (OVs) are believed as active sites for photocatalytic NO removal. The construction and stabilization of OVs on materials, especially from the point of view of exogenous ions towards different facets is vital for OVs-mediated photocatalysis. Herein, the impact of bromide ions (Br−) on OVs construction on different facets of Bi2MoO6 was systematically investigated. Theoretical calculations and characterizations demonstrated that Br− can boost and stabilize the OVs on {001} facets of Bi2MoO6, while hardly affect that on {010} facets. The Br- induced OVs on Bi2MoO6 caused a light-absorption until near-infrared region and enhanced the molecular oxygen activation, thus endowing the OVs concentration optimized Bi2MoO6 (BMO-001-Br) with superior activity on NO removal (62.9%) and selectivity of NO complete oxidation (93.61%) in a flow reaction. This work provides new insight into understanding the exogenous ions on construction and stabilization of OVs and the roles of OVs in photocatalytic NO removal. |
|---|---|
| AbstractList | Benefiting from the Br− selectively induced the OVs on {001} facets of Bi2MoO6, an extended light-absorption until near-infrared region and enhanced the molecular oxygen activation were achieved, thus endowing the OVs concentration optimized Bi2MoO6 with superior activity and selectivity of NO removal in a flow reaction.
[Display omitted]
•Br− boost the construction and stabilization of OVs on {001} facets of Bi2MoO6.•Br− induced OVs facilitate NO removal of BMO-001-Br even in near-infrared region.•NO oxidative removal with high selectivity of 93.6% is achieved on BMO-001-Br.•Mechanism for highly efficient NO removal (62.9%) over BMO-001-Br is proposed.
Surface oxygen vacancies (OVs) are believed as active sites for photocatalytic NO removal. The construction and stabilization of OVs on materials, especially from the point of view of exogenous ions towards different facets is vital for OVs-mediated photocatalysis. Herein, the impact of bromide ions (Br−) on OVs construction on different facets of Bi2MoO6 was systematically investigated. Theoretical calculations and characterizations demonstrated that Br− can boost and stabilize the OVs on {001} facets of Bi2MoO6, while hardly affect that on {010} facets. The Br- induced OVs on Bi2MoO6 caused a light-absorption until near-infrared region and enhanced the molecular oxygen activation, thus endowing the OVs concentration optimized Bi2MoO6 (BMO-001-Br) with superior activity on NO removal (62.9%) and selectivity of NO complete oxidation (93.61%) in a flow reaction. This work provides new insight into understanding the exogenous ions on construction and stabilization of OVs and the roles of OVs in photocatalytic NO removal. Surface oxygen vacancies (OVs) are believed as active sites for photocatalytic NO removal. The construction and stabilization of OVs on materials, especially from the point of view of exogenous ions towards different facets is vital for OVs-mediated photocatalysis. Herein, the impact of bromide ions (Br−) on OVs construction on different facets of Bi2MoO6 was systematically investigated. Theoretical calculations and characterizations demonstrated that Br− can boost and stabilize the OVs on {001} facets of Bi2MoO6, while hardly affect that on {010} facets. The Br- induced OVs on Bi2MoO6 caused a light-absorption until near-infrared region and enhanced the molecular oxygen activation, thus endowing the OVs concentration optimized Bi2MoO6 (BMO-001-Br) with superior activity on NO removal (62.9%) and selectivity of NO complete oxidation (93.61%) in a flow reaction. This work provides new insight into understanding the exogenous ions on construction and stabilization of OVs and the roles of OVs in photocatalytic NO removal. |
| ArticleNumber | 118585 |
| Author | Zhang, Lizhi Ding, Xing Wang, Shengyao Zhan, Guangming Dong, Guohui Chen, Hao Yang, Nan Zhang, Xuehao |
| Author_xml | – sequence: 1 givenname: Shengyao surname: Wang fullname: Wang, Shengyao email: wangshengyao@mail.hzau.edu.cn organization: College of Science, Huazhong Agricultural University, Wuhan, 430070, PR China – sequence: 2 givenname: Xing surname: Ding fullname: Ding, Xing organization: College of Science, Huazhong Agricultural University, Wuhan, 430070, PR China – sequence: 3 givenname: Nan surname: Yang fullname: Yang, Nan organization: College of Science, Huazhong Agricultural University, Wuhan, 430070, PR China – sequence: 4 givenname: Guangming surname: Zhan fullname: Zhan, Guangming organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental Chemistry, College of Chemistry, Central China Normal University, Wuhan, 430079, PR China – sequence: 5 givenname: Xuehao surname: Zhang fullname: Zhang, Xuehao organization: College of Science, Huazhong Agricultural University, Wuhan, 430070, PR China – sequence: 6 givenname: Guohui surname: Dong fullname: Dong, Guohui organization: School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xian, 710021, PR China – sequence: 7 givenname: Lizhi orcidid: 0000-0002-6842-9167 surname: Zhang fullname: Zhang, Lizhi organization: Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental Chemistry, College of Chemistry, Central China Normal University, Wuhan, 430079, PR China – sequence: 8 givenname: Hao orcidid: 0000-0002-3958-3456 surname: Chen fullname: Chen, Hao email: hchenhao@mail.hzau.edu.cn organization: College of Science, Huazhong Agricultural University, Wuhan, 430070, PR China |
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| Snippet | Benefiting from the Br− selectively induced the OVs on {001} facets of Bi2MoO6, an extended light-absorption until near-infrared region and enhanced the... Surface oxygen vacancies (OVs) are believed as active sites for photocatalytic NO removal. The construction and stabilization of OVs on materials, especially... |
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| SourceType | Aggregation Database Enrichment Source Index Database Publisher |
| StartPage | 118585 |
| SubjectTerms | Bi2MoO6 Bromine Electromagnetic absorption Facet Ions Near infrared radiation NO removal Oxidation Oxygen Oxygen vacancy Photocatalysis Selectivity Stabilization Vacancies |
| Title | Insight into the effect of bromine on facet-dependent surface oxygen vacancies construction and stabilization of Bi2MoO6 for efficient photocatalytic NO removal |
| URI | https://dx.doi.org/10.1016/j.apcatb.2019.118585 https://www.proquest.com/docview/2362965348 |
| Volume | 265 |
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