Functional separator with lower resistance toward lithium ion transport for enhancing the electrochemical performance of lithium ion batteries
[Display omitted] •Hydrophilicity is imparted into PE separator by chemical treatment with benzoyl peroxide (BPO).•BPO-PE separator exhibits superior wettability toward polar organic liquid electrolyte of LIBs.•The cell with the BPO-PE separator displays remarkable rate capability (86.7%) compared t...
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| Published in | Journal of industrial and engineering chemistry (Seoul, Korea) Vol. 71; pp. 228 - 233 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.03.2019
한국공업화학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1226-086X 1876-794X |
| DOI | 10.1016/j.jiec.2018.11.029 |
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| Abstract | [Display omitted]
•Hydrophilicity is imparted into PE separator by chemical treatment with benzoyl peroxide (BPO).•BPO-PE separator exhibits superior wettability toward polar organic liquid electrolyte of LIBs.•The cell with the BPO-PE separator displays remarkable rate capability (86.7%) compared to the PE separator (78.6%) at a current rate of 3.0C.
By chemical treatment with benzoyl peroxide, oxygen-containing functional groups can be successfully introduced to the surface and interior of the PE separator, resulting in improved wettability and high electrolyte uptake without sacrificing mechanical and physicochemical properties. Hence, lithium ion transport across the PE separator treated by benzoyl peroxide is effectively facilitated by the formation of oxygen functional groups, leading to improved ionic conductivity. The LiB cells assembled with the PE separator treated by BPO exhibit remarkable rate capability and outstanding capacity retention (98.1%) after 70 cycles. |
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| AbstractList | By chemical treatment with benzoyl peroxide, oxygen-containing functional groups can be successfullyintroduced to the surface and interior of the PE separator, resulting in improved wettability and highelectrolyte uptake without sacrificing mechanical and physicochemical properties. Hence, lithium iontransport across the PE separator treated by benzoyl peroxide is effectively facilitated by the formation ofoxygen functional groups, leading to improved ionic conductivity. The LiB cells assembled with the PEseparator treated by BPO exhibit remarkable rate capability and outstanding capacity retention (98.1%)after 70 cycles. KCI Citation Count: 1 [Display omitted] •Hydrophilicity is imparted into PE separator by chemical treatment with benzoyl peroxide (BPO).•BPO-PE separator exhibits superior wettability toward polar organic liquid electrolyte of LIBs.•The cell with the BPO-PE separator displays remarkable rate capability (86.7%) compared to the PE separator (78.6%) at a current rate of 3.0C. By chemical treatment with benzoyl peroxide, oxygen-containing functional groups can be successfully introduced to the surface and interior of the PE separator, resulting in improved wettability and high electrolyte uptake without sacrificing mechanical and physicochemical properties. Hence, lithium ion transport across the PE separator treated by benzoyl peroxide is effectively facilitated by the formation of oxygen functional groups, leading to improved ionic conductivity. The LiB cells assembled with the PE separator treated by BPO exhibit remarkable rate capability and outstanding capacity retention (98.1%) after 70 cycles. |
| Author | Choi, Wonchang Yim, Taeeun Kwon, Yong Kab Kim, Ki Jae |
| Author_xml | – sequence: 1 givenname: Ki Jae surname: Kim fullname: Kim, Ki Jae organization: Department of Energy Engineering, Konkuk University, Neungdong-ro 120, Gwangjin-gu, Seoul, Republic of Korea – sequence: 2 givenname: Yong Kab surname: Kwon fullname: Kwon, Yong Kab organization: Department of Energy Engineering, Konkuk University, Neungdong-ro 120, Gwangjin-gu, Seoul, Republic of Korea – sequence: 3 givenname: Taeeun orcidid: 0000-0002-7057-9308 surname: Yim fullname: Yim, Taeeun organization: Department of Chemistry, Incheon National University, Academy-ro 119, Songdo-dong, Yeonsu-gu, Incheon, 460-772, Republic of Korea – sequence: 4 givenname: Wonchang orcidid: 0000-0002-8463-1517 surname: Choi fullname: Choi, Wonchang email: wonchangchoi@kist.re.kr organization: Center for Energy Convergence, Korea Institute of Science and Technology, 39-1 Hawolgok-dong, Seongbuk-gu, Seoul, 136-791, Republic of Korea |
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| CitedBy_id | crossref_primary_10_1016_j_jpowsour_2020_228812 crossref_primary_10_3390_polym15183690 crossref_primary_10_1016_j_carbpol_2020_115907 crossref_primary_10_59400_esc1631 crossref_primary_10_1016_j_jpowsour_2021_229933 crossref_primary_10_1016_j_jiec_2019_04_008 crossref_primary_10_3390_coatings13050916 crossref_primary_10_1002_er_7256 crossref_primary_10_1016_j_cej_2022_136801 crossref_primary_10_1007_s10924_024_03320_7 crossref_primary_10_1016_j_est_2021_103668 crossref_primary_10_1016_j_etran_2024_100330 crossref_primary_10_1016_j_mtener_2020_100485 crossref_primary_10_1016_j_jiec_2025_03_032 crossref_primary_10_1021_acsnano_2c09526 crossref_primary_10_1002_er_5401 crossref_primary_10_3390_batteries9110556 |
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| SubjectTerms | Hydrophilicity Lithium ion battery Lithium ion transfer Separator Surface treatment Wettability 화학공학 |
| Title | Functional separator with lower resistance toward lithium ion transport for enhancing the electrochemical performance of lithium ion batteries |
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