Novel p-n heterojunction photocatalyst fabricated by flower-like BiVO4 and Ag2S nanoparticles: Simple synthesis and excellent photocatalytic performance
[Display omitted] •The degradation efficiency of TC over the 0.3-p-Ag2S/n-BiVO4 can be achieved 90.2%.•Ten intermediate products for TC degradation were verified by the GC-MS.•The enhancing photocatalysis mechanism was attributed to the facilitated charge transfer. Three-dimensional microsphere p-Ag...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 361; pp. 1173 - 1181 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.04.2019
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•The degradation efficiency of TC over the 0.3-p-Ag2S/n-BiVO4 can be achieved 90.2%.•Ten intermediate products for TC degradation were verified by the GC-MS.•The enhancing photocatalysis mechanism was attributed to the facilitated charge transfer.
Three-dimensional microsphere p-Ag2S/n-BiVO4 p-n heterojunction photocatalyst was successfully fabricated via depositing p-type Ag2S on n-type BiVO4, which showed excellent photocatalytic performance, compared with BiVO4 and Ag2S, for the photocatalytic degradation of tetracycline under visible light irradiation. The enhancing photocatalytic performance can be attributed to the facilitated charge transfer, and the increased lifetime of the charge carriers confirmed by the results of time-resolved fluorescence spectra and photoelectrochemical measures. Moreover, 10 photocatalytic degradation intermediates and products were also identified by the gas chromatography-mass spectrometer. Finally, the photocatalytic enhancement mechanism over p-Ag2S/n-BiVO4 was discussed. The strategy to form three-dimensional microspheres p-n heterojunction photocatalyst may open a new opportunity to design highly efficient photocatalyst for environmental treatment to control pollution. |
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| AbstractList | [Display omitted]
•The degradation efficiency of TC over the 0.3-p-Ag2S/n-BiVO4 can be achieved 90.2%.•Ten intermediate products for TC degradation were verified by the GC-MS.•The enhancing photocatalysis mechanism was attributed to the facilitated charge transfer.
Three-dimensional microsphere p-Ag2S/n-BiVO4 p-n heterojunction photocatalyst was successfully fabricated via depositing p-type Ag2S on n-type BiVO4, which showed excellent photocatalytic performance, compared with BiVO4 and Ag2S, for the photocatalytic degradation of tetracycline under visible light irradiation. The enhancing photocatalytic performance can be attributed to the facilitated charge transfer, and the increased lifetime of the charge carriers confirmed by the results of time-resolved fluorescence spectra and photoelectrochemical measures. Moreover, 10 photocatalytic degradation intermediates and products were also identified by the gas chromatography-mass spectrometer. Finally, the photocatalytic enhancement mechanism over p-Ag2S/n-BiVO4 was discussed. The strategy to form three-dimensional microspheres p-n heterojunction photocatalyst may open a new opportunity to design highly efficient photocatalyst for environmental treatment to control pollution. |
| Author | Wei, Zhao Yue, Feng Benlin, Dai Fengxia, Zhu Xiaomeng, Wang Jiming, Xu Lili, Zhang Ni, Sheng Xinyue, Tu |
| Author_xml | – sequence: 1 givenname: Zhao surname: Wei fullname: Wei, Zhao organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 2 givenname: Tu surname: Xinyue fullname: Xinyue, Tu organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 3 givenname: Wang surname: Xiaomeng fullname: Xiaomeng, Wang organization: School of the Environment, Nanjing University, BK20160430, Nanjing 210023, China – sequence: 4 givenname: Dai surname: Benlin fullname: Benlin, Dai organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 5 givenname: Zhang surname: Lili fullname: Lili, Zhang organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 6 givenname: Xu surname: Jiming fullname: Jiming, Xu email: 8201711050@hytc.edu.cn organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 7 givenname: Feng surname: Yue fullname: Yue, Feng organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China – sequence: 8 givenname: Sheng surname: Ni fullname: Ni, Sheng organization: Department of Decision Sciences, Macau University of Science and Technology, Avenida Wai Long, Taipa, Macau, China – sequence: 9 givenname: Zhu surname: Fengxia fullname: Fengxia, Zhu email: zhufx@hytc.cn organization: Jiangsu Key Laboratory for Biomass-based Energy and Enzyme Technology, Jiangsu Collaborative Innovation Center of Regional Modern Agriculture & Environmental Protection, School of Chemistry and Chemical Engineering, Huaiyin Normal University, Huaian, China |
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•The degradation efficiency of TC over the 0.3-p-Ag2S/n-BiVO4 can be achieved 90.2%.•Ten intermediate products for TC degradation were... |
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| Title | Novel p-n heterojunction photocatalyst fabricated by flower-like BiVO4 and Ag2S nanoparticles: Simple synthesis and excellent photocatalytic performance |
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