Stabilized oxygen vacancies over heterojunction for highly efficient and exceptionally durable VOCs photocatalytic degradation
[Display omitted] •Enrichment of OVs on the BiVO4 component of R-BiVO4/WO3/TNTs composite matrix by a simple electrochemical reduction step.•Achievement of enhanced electron-hole separation and charge transport capabilities by introducing OVs in R-BiVO4/WO3/TNTs.•Improving the reaction stability of...
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| Published in | Applied catalysis. B, Environmental Vol. 273; p. 119061 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.09.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Enrichment of OVs on the BiVO4 component of R-BiVO4/WO3/TNTs composite matrix by a simple electrochemical reduction step.•Achievement of enhanced electron-hole separation and charge transport capabilities by introducing OVs in R-BiVO4/WO3/TNTs.•Improving the reaction stability of OVs by transforming active species OH into O2− during the photocatalytic process.•R-BiVO4/WO3/TNTs that exhibit 28 times higher photocurrent density and a highly efficient VOCs photocatalytic degradation.
In this study, an electrochemical reduction strategy was adopted to introduce oxygen vacancies (OVs) into BiVO4/WO3/TiO2 nanotubes composite film (R-BiVO4/WO3/TNTs), and the newly generated OVs were mainly distributed on BiVO4. Desired concentration and distribution of the OVs were achieved by optimizing the reduction potential and duration. By introducing the reduced BiVO4, the inherent reaction mechanism dominated by OH and photogenerated hole was changed into the reaction dominated by O2− and hole, thereby improving the stability of the OVs in the catalytic process. The construction of heterojunction with the stabilized OVs had a significant contribution towards charge carrier separation and transmission in the material, and especially the stability of the performance. Thus, the R-BiVO4/WO3/TNTs exhibited a 28 times higher photocurrent intensity than the pristine BiVO4/WO3/TNTs, and the one-time purification experiment further confirmed the excellent performance and persistent nature of R-BiVO4/WO3/TNTs composite film in the actual treatment of VOCs. |
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| AbstractList | In this study, an electrochemical reduction strategy was adopted to introduce oxygen vacancies (OVs) into BiVO4/WO3/TiO2 nanotubes composite film (R-BiVO4/WO3/TNTs), and the newly generated OVs were mainly distributed on BiVO4. Desired concentration and distribution of the OVs were achieved by optimizing the reduction potential and duration. By introducing the reduced BiVO4, the inherent reaction mechanism dominated by •OH and photogenerated hole was changed into the reaction dominated by •O2− and hole, thereby improving the stability of the OVs in the catalytic process. The construction of heterojunction with the stabilized OVs had a significant contribution towards charge carrier separation and transmission in the material, and especially the stability of the performance. Thus, the R-BiVO4/WO3/TNTs exhibited a 28 times higher photocurrent intensity than the pristine BiVO4/WO3/TNTs, and the one-time purification experiment further confirmed the excellent performance and persistent nature of R-BiVO4/WO3/TNTs composite film in the actual treatment of VOCs. [Display omitted] •Enrichment of OVs on the BiVO4 component of R-BiVO4/WO3/TNTs composite matrix by a simple electrochemical reduction step.•Achievement of enhanced electron-hole separation and charge transport capabilities by introducing OVs in R-BiVO4/WO3/TNTs.•Improving the reaction stability of OVs by transforming active species OH into O2− during the photocatalytic process.•R-BiVO4/WO3/TNTs that exhibit 28 times higher photocurrent density and a highly efficient VOCs photocatalytic degradation. In this study, an electrochemical reduction strategy was adopted to introduce oxygen vacancies (OVs) into BiVO4/WO3/TiO2 nanotubes composite film (R-BiVO4/WO3/TNTs), and the newly generated OVs were mainly distributed on BiVO4. Desired concentration and distribution of the OVs were achieved by optimizing the reduction potential and duration. By introducing the reduced BiVO4, the inherent reaction mechanism dominated by OH and photogenerated hole was changed into the reaction dominated by O2− and hole, thereby improving the stability of the OVs in the catalytic process. The construction of heterojunction with the stabilized OVs had a significant contribution towards charge carrier separation and transmission in the material, and especially the stability of the performance. Thus, the R-BiVO4/WO3/TNTs exhibited a 28 times higher photocurrent intensity than the pristine BiVO4/WO3/TNTs, and the one-time purification experiment further confirmed the excellent performance and persistent nature of R-BiVO4/WO3/TNTs composite film in the actual treatment of VOCs. |
| ArticleNumber | 119061 |
| Author | Wang, Xiaoguang Murugananthan, Muthu Chen, Yong Zhang, Yanrong Sun, Minghui Chen, Zhiquan |
| Author_xml | – sequence: 1 givenname: Minghui surname: Sun fullname: Sun, Minghui organization: School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, PR China – sequence: 2 givenname: Xiaoguang surname: Wang fullname: Wang, Xiaoguang organization: School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, PR China – sequence: 3 givenname: Zhiquan orcidid: 0000-0002-9518-7837 surname: Chen fullname: Chen, Zhiquan organization: Hubei Nuclear Solid Physics Key Laboratory, Department of Physics, Wuhan University, Wuhan, 430072, PR China – sequence: 4 givenname: Muthu orcidid: 0000-0003-0575-5018 surname: Murugananthan fullname: Murugananthan, Muthu organization: Department of Chemistry, PSG College of Technology, Peelamedu, Coimbatore, 641004, India – sequence: 5 givenname: Yong surname: Chen fullname: Chen, Yong organization: School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, PR China – sequence: 6 givenname: Yanrong orcidid: 0000-0002-8793-090X surname: Zhang fullname: Zhang, Yanrong email: yanrong_zhang@hust.edu.cn organization: School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, PR China |
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| Keywords | Electrochemical reduction Photodegradation of VOCs BiVO4/WO3/TiO2 nanotubes Stabilized OVs |
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•Enrichment of OVs on the BiVO4 component of R-BiVO4/WO3/TNTs composite matrix by a simple electrochemical reduction step.•Achievement of... In this study, an electrochemical reduction strategy was adopted to introduce oxygen vacancies (OVs) into BiVO4/WO3/TiO2 nanotubes composite film... |
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| StartPage | 119061 |
| SubjectTerms | Bismuth oxides BiVO4/WO3/TiO2 nanotubes Chemical reduction Current carriers Electrochemical reduction Electrochemistry Heterojunctions Nanotechnology Nanotubes Oxygen Photodegradation Photodegradation of VOCs Photoelectric effect Photoelectric emission Reaction mechanisms Stability Stabilized OVs Titanium dioxide Tungsten oxides Vacancies Vanadates |
| Title | Stabilized oxygen vacancies over heterojunction for highly efficient and exceptionally durable VOCs photocatalytic degradation |
| URI | https://dx.doi.org/10.1016/j.apcatb.2020.119061 https://www.proquest.com/docview/2440098587 |
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