Particle‐resolved simulations of methane steam reforming in multilayered packed beds
Particle‐resolved CFD simulations of multilayered packed beds containing 30 particles of different particle shapes (trilobe, daisy, hollow cylinder, cylcut, and 7‐hole cylinder) with a tube to particle diameter ratio of 5, were performed to understand the effect of particle shape on pressure drop (Δ...
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| Published in | AIChE journal Vol. 64; no. 11; pp. 4162 - 4176 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken, USA
John Wiley & Sons, Inc
01.11.2018
American Institute of Chemical Engineers |
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| Online Access | Get full text |
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| Abstract | Particle‐resolved CFD simulations of multilayered packed beds containing 30 particles of different particle shapes (trilobe, daisy, hollow cylinder, cylcut, and 7‐hole cylinder) with a tube to particle diameter ratio of 5, were performed to understand the effect of particle shape on pressure drop (ΔP), dispersion, CH4 conversion and effectiveness factors for methane steam reforming reactions. The effect of different boundary conditions and particle modeling approaches were analyzed in detail. The empirical correlations (Ergun and Zhavoronkov et al.) over‐predicted the ΔP and a modified correlation was developed to predict ΔP for the particles with different shapes. Overall, the externally shaped particles (trilobe and daisy) offered lower ΔP and higher dispersion because of the lower surface area and higher back flow regions, whereas the internally shaped particles (cylcut, hollow, and 7‐hole cylinder) offered higher CH4 conversion and effectiveness factors because of the better access for the reactants. The cylcut‐shape offered the highest CH4 conversion/ΔP. © 2018 American Institute of Chemical Engineers AIChE J, 64: 4162–4176, 2018 |
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| AbstractList | Particle‐resolved CFD simulations of multilayered packed beds containing 30 particles of different particle shapes (trilobe, daisy, hollow cylinder, cylcut, and 7‐hole cylinder) with a tube to particle diameter ratio of 5, were performed to understand the effect of particle shape on pressure drop (ΔP), dispersion, CH4 conversion and effectiveness factors for methane steam reforming reactions. The effect of different boundary conditions and particle modeling approaches were analyzed in detail. The empirical correlations (Ergun and Zhavoronkov et al.) over‐predicted the ΔP and a modified correlation was developed to predict ΔP for the particles with different shapes. Overall, the externally shaped particles (trilobe and daisy) offered lower ΔP and higher dispersion because of the lower surface area and higher back flow regions, whereas the internally shaped particles (cylcut, hollow, and 7‐hole cylinder) offered higher CH4 conversion and effectiveness factors because of the better access for the reactants. The cylcut‐shape offered the highest CH4 conversion/ΔP. © 2018 American Institute of Chemical Engineers AIChE J, 64: 4162–4176, 2018 Particle‐resolved CFD simulations of multilayered packed beds containing 30 particles of different particle shapes (trilobe, daisy, hollow cylinder, cylcut, and 7‐hole cylinder) with a tube to particle diameter ratio of 5, were performed to understand the effect of particle shape on pressure drop ( ΔP ), dispersion, CH 4 conversion and effectiveness factors for methane steam reforming reactions. The effect of different boundary conditions and particle modeling approaches were analyzed in detail. The empirical correlations (Ergun and Zhavoronkov et al.) over‐predicted the ΔP and a modified correlation was developed to predict ΔP for the particles with different shapes. Overall, the externally shaped particles (trilobe and daisy) offered lower ΔP and higher dispersion because of the lower surface area and higher back flow regions, whereas the internally shaped particles (cylcut, hollow, and 7‐hole cylinder) offered higher CH 4 conversion and effectiveness factors because of the better access for the reactants. The cylcut‐shape offered the highest CH 4 conversion/ ΔP . © 2018 American Institute of Chemical Engineers AIChE J , 64: 4162–4176, 2018 |
| Author | Buwa, Vivek V. G. M., Karthik |
| Author_xml | – sequence: 1 givenname: Karthik surname: G. M. fullname: G. M., Karthik organization: Indian Institute of Technology Delhi – sequence: 2 givenname: Vivek V. orcidid: 0000-0003-2335-6379 surname: Buwa fullname: Buwa, Vivek V. email: vvbuwa@iitd.ac.in organization: Indian Institute of Technology Delhi |
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| SubjectTerms | Boundary conditions catalyst shape CFD simulation Computer simulation Conversion Correlation analysis Cylinders effectiveness factor Empirical analysis Methane methane steam reforming Organic chemistry packed bed Packed beds Particle shape Particle size Pressure drop Reforming Shape effects |
| Title | Particle‐resolved simulations of methane steam reforming in multilayered packed beds |
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