An investigation on gas hydrate formation and slurry viscosity in the presence of wax crystals
Clarifying the interaction effect between hydrate and wax is of great significance to guarantee operation safety in deep water petroleum fields. Experiments in a high‐pressure hydrate slurry rheological measurement system were carried out to investigate hydrate formation and slurry viscosity in the...
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| Published in | AIChE journal Vol. 64; no. 9; pp. 3502 - 3518 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
American Institute of Chemical Engineers
01.09.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Clarifying the interaction effect between hydrate and wax is of great significance to guarantee operation safety in deep water petroleum fields. Experiments in a high‐pressure hydrate slurry rheological measurement system were carried out to investigate hydrate formation and slurry viscosity in the presence of wax crystals. Results indicate that the presence of wax crystals can prolong hydrate nucleation induction time, and its influence on hydrate growth depends on multiple factors. Higher stirring rate can obviously promote hydrate growth rate, while its influence on hydrate nucleation induction time is complicated. Higher initial pressure will promote hydrate formation. Gas hydrate slurry shows a shear‐thinning behavior, and slurry viscosity increases with the increase of wax content and initial pressure. A semiempirical viscosity model showing a well‐fitting is established for hydrate slurry with wax crystals by considering the aggregation and breakage of hydrate particles, wax crystals, and water droplets. © 2018 American Institute of Chemical Engineers AIChE J, 64: 3502–3518, 2018 |
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| AbstractList | Clarifying the interaction effect between hydrate and wax is of great significance to guarantee operation safety in deep water petroleum fields. Experiments in a high‐pressure hydrate slurry rheological measurement system were carried out to investigate hydrate formation and slurry viscosity in the presence of wax crystals. Results indicate that the presence of wax crystals can prolong hydrate nucleation induction time, and its influence on hydrate growth depends on multiple factors. Higher stirring rate can obviously promote hydrate growth rate, while its influence on hydrate nucleation induction time is complicated. Higher initial pressure will promote hydrate formation. Gas hydrate slurry shows a shear‐thinning behavior, and slurry viscosity increases with the increase of wax content and initial pressure. A semiempirical viscosity model showing a well‐fitting is established for hydrate slurry with wax crystals by considering the aggregation and breakage of hydrate particles, wax crystals, and water droplets. © 2018 American Institute of Chemical Engineers AIChE J, 64: 3502–3518, 2018 Clarifying the interaction effect between hydrate and wax is of great significance to guarantee operation safety in deep water petroleum fields. Experiments in a high‐pressure hydrate slurry rheological measurement system were carried out to investigate hydrate formation and slurry viscosity in the presence of wax crystals. Results indicate that the presence of wax crystals can prolong hydrate nucleation induction time, and its influence on hydrate growth depends on multiple factors. Higher stirring rate can obviously promote hydrate growth rate, while its influence on hydrate nucleation induction time is complicated. Higher initial pressure will promote hydrate formation. Gas hydrate slurry shows a shear‐thinning behavior, and slurry viscosity increases with the increase of wax content and initial pressure. A semiempirical viscosity model showing a well‐fitting is established for hydrate slurry with wax crystals by considering the aggregation and breakage of hydrate particles, wax crystals, and water droplets. © 2018 American Institute of Chemical Engineers AIChE J , 64: 3502–3518, 2018 |
| Author | Wu, Hai‐Hao Wang, Wei Gong, Jing Chen, Yu‐Chuan Shi, Bo‐Hui Yao, Hai‐Yuan Ding, Lin Liu, Yang Song, Shang‐Fei Chai, Shuai |
| Author_xml | – sequence: 1 givenname: Bo‐Hui orcidid: 0000-0003-2683-6984 surname: Shi fullname: Shi, Bo‐Hui email: bh.shi@cup.edu.cn organization: China University of Petroleum‐Beijing – sequence: 2 givenname: Shuai surname: Chai fullname: Chai, Shuai organization: Sinopec Engineering Incorporation – sequence: 3 givenname: Lin surname: Ding fullname: Ding, Lin organization: China University of Petroleum‐Beijing – sequence: 4 givenname: Yu‐Chuan surname: Chen fullname: Chen, Yu‐Chuan organization: China University of Petroleum‐Beijing – sequence: 5 givenname: Yang surname: Liu fullname: Liu, Yang organization: China University of Petroleum‐Beijing – sequence: 6 givenname: Shang‐Fei surname: Song fullname: Song, Shang‐Fei organization: China University of Petroleum‐Beijing – sequence: 7 givenname: Hai‐Yuan surname: Yao fullname: Yao, Hai‐Yuan organization: CNOOC Research Institute Co. Ltd – sequence: 8 givenname: Hai‐Hao surname: Wu fullname: Wu, Hai‐Hao organization: China University of Petroleum‐Beijing – sequence: 9 givenname: Wei surname: Wang fullname: Wang, Wei organization: China University of Petroleum‐Beijing – sequence: 10 givenname: Jing orcidid: 0000-0002-2970-7988 surname: Gong fullname: Gong, Jing email: ydgj@cup.edu.cn organization: China University of Petroleum‐Beijing |
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| Snippet | Clarifying the interaction effect between hydrate and wax is of great significance to guarantee operation safety in deep water petroleum fields. Experiments in... |
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| SubjectTerms | Breakage Crystals Deep water hydrate formation hydrate slurry viscosity hydrates induction time Initial pressure Nucleation Organic chemistry Pressure Rheological properties Sedimentation & deposition Slurries Viscosity Water drops wax crystals Waxes |
| Title | An investigation on gas hydrate formation and slurry viscosity in the presence of wax crystals |
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