Study on mass transfer of ethyl acetate in polymer adsorbent by experimental and theoretical breakthrough curves
A new polymeric adsorbent with highly hypercrosslinked structure was developed for the removal of VOCs from polluted air. The purpose of this work is to obtain the intraparticle mass transfer coefficient of the adsorbent particles. Adsorption experiments for obtaining breakthrough curves were carrie...
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| Published in | Chinese journal of chemical engineering Vol. 28; no. 1; pp. 84 - 89 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.01.2020
State Key Laboratory of Multiphase Complex Systems,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China Sino-Danish College,University of Chinese Academy of Sciences,Beijing 100190,China%State Key Laboratory of Multiphase Complex Systems,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China |
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| Abstract | A new polymeric adsorbent with highly hypercrosslinked structure was developed for the removal of VOCs from polluted air. The purpose of this work is to obtain the intraparticle mass transfer coefficient of the adsorbent particles. Adsorption experiments for obtaining breakthrough curves were carried out with a fixed bed system. A dynamic mathematical model for the fixed bed adsorption system was developed. By model fitting, the overall mass transfer coefficient was determined when the deviation error was minimum. Then, the intraparticle mass transfer coefficient of the adsorbent was determined when the external mass transfer resistance was eliminated at higher velocities. Furthermore, a linear relationship of the intraparticle mass transfer coefficient and equilibrium coefficient at lower inlet gas concentrations range was correlated. Moreover, an equation for predicting external mass transfer coefficient at low Reynolds number range at room temperature was obtained. |
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| AbstractList | A new polymeric adsorbent with highly hypercrosslinked structure was developed for the removal of VOCs from polluted air. The purpose of this work is to obtain the intraparticle mass transfer coefficient of the adsorbent particles. Adsorption experiments for obtaining breakthrough curves were carried out with a fixed bed system. A dynamic mathematical model for the fixed bed adsorption system was developed. By model fitting, the overall mass transfer coefficient was determined when the deviation error was minimum. Then, the intraparticle mass transfer coefficient of the adsorbent was determined when the external mass transfer resistance was eliminated at higher velocities. Furthermore, a linear relationship of the intraparticle mass transfer coefficient and equilibrium coefficient at lower inlet gas concentrations range was correlated. Moreover, an equation for predicting external mass transfer coefficient at low Reynolds number range at room temperature was obtained. |
| Author | Li, Songgeng Song, Wenli Wang, Lina Du, Lin Zheng, Jiale |
| AuthorAffiliation | State Key Laboratory of Multiphase Complex Systems,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China;Sino-Danish College,University of Chinese Academy of Sciences,Beijing 100190,China%State Key Laboratory of Multiphase Complex Systems,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China |
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| Cites_doi | 10.1021/ie50677a007 10.1080/00986448008912520 10.1080/19443994.2013.862869 10.1080/09593330.2014.904445 10.1016/0009-2509(68)87056-3 10.1021/es010017x 10.1021/i160026a016 10.30955/gnj.002368 10.1021/i160017a002 10.1016/S0950-4230(00)00007-3 10.1021/i160006a007 |
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Fundam. doi: 10.1021/i160006a007 |
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| Title | Study on mass transfer of ethyl acetate in polymer adsorbent by experimental and theoretical breakthrough curves |
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