Kelp-inspired N–I-doped ZnO photocatalysts with highly efficient catalytic activity
Efficient N–I-doped ZnO photocatalysts with hierarchical structures are fabricated with kelp as the template. Abundant nitrogen and iodine are successfully simultaneously introduced into the bulk ZnO crystals though calcination under high temperature (600°C). The morphology, structure, composition,...
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| Published in | Materials science in semiconductor processing Vol. 43; pp. 25 - 33 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.03.2016
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| Abstract | Efficient N–I-doped ZnO photocatalysts with hierarchical structures are fabricated with kelp as the template. Abundant nitrogen and iodine are successfully simultaneously introduced into the bulk ZnO crystals though calcination under high temperature (600°C). The morphology, structure, composition, and optical absorption properties of the kelp-templated ZnO are characterized by X-ray diffraction (XRD), field-emission scanning microscopy (FESEM), transmission electron microscopy (TEM), and diffuse reflectance spectra (DRS), respectively. The band gap of the kelp-templated ZnO is narrowed by the N–I coping. The photocatalytic activity under UV-irradiation of the kelp-templated ZnO is about 23.1 times and 1.1 times that of common ZnO and P25, respectively. In addition, no obvious activity of the kelp-templated ZnO is decreased, during five cycle runs. The efficient photocatalytic activity of the kelp-templated ZnO is attributed to the sufficient UV-light utilization and efficient separation of electron–hole pairs. |
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| AbstractList | Efficient N–I-doped ZnO photocatalysts with hierarchical structures are fabricated with kelp as the template. Abundant nitrogen and iodine are successfully simultaneously introduced into the bulk ZnO crystals though calcination under high temperature (600°C). The morphology, structure, composition, and optical absorption properties of the kelp-templated ZnO are characterized by X-ray diffraction (XRD), field-emission scanning microscopy (FESEM), transmission electron microscopy (TEM), and diffuse reflectance spectra (DRS), respectively. The band gap of the kelp-templated ZnO is narrowed by the N–I coping. The photocatalytic activity under UV-irradiation of the kelp-templated ZnO is about 23.1 times and 1.1 times that of common ZnO and P25, respectively. In addition, no obvious activity of the kelp-templated ZnO is decreased, during five cycle runs. The efficient photocatalytic activity of the kelp-templated ZnO is attributed to the sufficient UV-light utilization and efficient separation of electron–hole pairs. Efficient N-I-doped ZnO photocatalysts with hierarchical structures are fabricated with kelp as the template. Abundant nitrogen and iodine are successfully simultaneously introduced into the bulk ZnO crystals though calcination under high temperature (600 degree C). The morphology, structure, composition, and optical absorption properties of the kelp-templated ZnO are characterized by X-ray diffraction (XRD), field-emission scanning microscopy (FESEM), transmission electron microscopy (TEM), and diffuse reflectance spectra (DRS), respectively. The band gap of the kelp-templated ZnO is narrowed by the N-I coping. The photocatalytic activity under UV-irradiation of the kelp-templated ZnO is about 23.1 times and 1.1 times that of common ZnO and P25, respectively. In addition, no obvious activity of the kelp-templated ZnO is decreased, during five cycle runs. The efficient photocatalytic activity of the kelp-templated ZnO is attributed to the sufficient UV-light utilization and efficient separation of electron-hole pairs. |
| Author | Cai, Aijun Du, Liqiang Wang, Xiuping Wang, Qian Chang, Yongfang Guo, Xuemin |
| Author_xml | – sequence: 1 givenname: Aijun surname: Cai fullname: Cai, Aijun organization: College of Life Science and Technology, Hebei Normal University of Science & Technology, Qinhuangdao 066600, PR China – sequence: 2 givenname: Liqiang surname: Du fullname: Du, Liqiang organization: College of Life Science and Technology, Hebei Normal University of Science & Technology, Qinhuangdao 066600, PR China – sequence: 3 givenname: Qian surname: Wang fullname: Wang, Qian organization: Beijing University of Chinese Medicine Dongfang College, Langfang 065001, PR China – sequence: 4 givenname: Yongfang surname: Chang fullname: Chang, Yongfang email: changyongfang@126.com organization: College of Chemical Technology, Shijiazhuang University, Shijianzhuang 050035, PR China – sequence: 5 givenname: Xiuping surname: Wang fullname: Wang, Xiuping email: wangxiuping0721@163.com organization: College of Life Science and Technology, Hebei Normal University of Science & Technology, Qinhuangdao 066600, PR China – sequence: 6 givenname: Xuemin surname: Guo fullname: Guo, Xuemin organization: College of Life Science and Technology, Hebei Normal University of Science & Technology, Qinhuangdao 066600, PR China |
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| SubjectTerms | Catalytic activity Kelp Materials science N–I doping Photocatalysis Photocatalysts Photocatalytic activity Reflectance Semiconductors Template Transmission electron microscopy Zinc oxide ZnO |
| Title | Kelp-inspired N–I-doped ZnO photocatalysts with highly efficient catalytic activity |
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