Insights into high-efficient removal of tetracycline by a codoped mesoporous carbon adsorbent
[Display omitted] Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants. Herein, a carbon nanoplate codoped by Co and N elements with abundant ordered mesoporous (Co/N-MCs) was applied as an adsorbent for tetracycline remo...
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| Published in | Chinese journal of chemical engineering Vol. 44; no. 4; pp. 148 - 156 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.04.2022
College of Food Science and Engineering,Northwest A&F University,Yangling 712100,China%Qinghai Provincial Key Laboratory of Qinghai-Tibet Plateau Biological Resources,Northwest Institute of Plateau Biology,Chinese Academy of Sciences,Xining 810008,China |
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| Online Access | Get full text |
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| Abstract | [Display omitted]
Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants. Herein, a carbon nanoplate codoped by Co and N elements with abundant ordered mesoporous (Co/N-MCs) was applied as an adsorbent for tetracycline removal. Taking integrated advantages of ordered mesopores on carbon-based structures and N-doping inducing the strengthened π–π dispersion and generation of pyridinic N, as well as cobaltic nanoparticles embedded in carbon nanoplates, the Co/N-MCs was tailored for high efficiently absorbing tetracycline via π-π interaction, Lewis acid-base interaction, metal complexation and electrostatic attraction. The Co/N-MCs had the advantages of high surface area, porous structure, plenty adsorption sites, and easy separation. As such, the as-prepared Co/N-MCs adsorbents significantly enhanced tetracycline removal performance with a maximum adsorption capacity of 344.83 mg·g−1 at pH 6 and good reusability, which was finally applied to removal tetracycline from tap water sample. Furthermore, the adsorption process towards tetracycline hydrochloride could be well attributed to the pseudo-second-order kinetic and Langmuir isotherm models. Compared with traditional carbon-based adsorbents, it owns a simpler synthesis method and a higher adsorption capacity, as well as it is a promising candidate for water purification. |
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| AbstractList | Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants.Herein,a carbon nanoplate codoped by Co and N elements with abun-dant ordered mesoporous(Co/N-MCs)was applied as an adsorbent for tetracycline removal.Taking inte-grated advantages of ordered mesopores on carbon-based structures and N-doping inducing the strengthened π-π dispersion and generation of pyridinic N,as well as cobaltic nanoparticles embedded in carbon nanoplates,the Co/N-MCs was tailored for high efficiently absorbing tetracycline via π-π inter-action,Lewis acid-base interaction,metal complexation and electrostatic attraction.The Co/N-MCs had the advantages of high surface area,porous structure,plenty adsorption sites,and easy separation.As such,the as-prepared Co/N-MCs adsorbents significantly enhanced tetracycline removal performance with a maximum adsorption capacity of 344.83 mg·g-1 at pH 6 and good reusability,which was finally applied to removal tetracycline from tap water sample.Furthermore,the adsorption process towards tetracycline hydrochloride could be well attributed to the pseudo-second-order kinetic and Langmuir iso-therm models.Compared with traditional carbon-based adsorbents,it owns a simpler synthesis method and a higher adsorption capacity,as well as it is a promising candidate for water purification. [Display omitted] Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants. Herein, a carbon nanoplate codoped by Co and N elements with abundant ordered mesoporous (Co/N-MCs) was applied as an adsorbent for tetracycline removal. Taking integrated advantages of ordered mesopores on carbon-based structures and N-doping inducing the strengthened π–π dispersion and generation of pyridinic N, as well as cobaltic nanoparticles embedded in carbon nanoplates, the Co/N-MCs was tailored for high efficiently absorbing tetracycline via π-π interaction, Lewis acid-base interaction, metal complexation and electrostatic attraction. The Co/N-MCs had the advantages of high surface area, porous structure, plenty adsorption sites, and easy separation. As such, the as-prepared Co/N-MCs adsorbents significantly enhanced tetracycline removal performance with a maximum adsorption capacity of 344.83 mg·g−1 at pH 6 and good reusability, which was finally applied to removal tetracycline from tap water sample. Furthermore, the adsorption process towards tetracycline hydrochloride could be well attributed to the pseudo-second-order kinetic and Langmuir isotherm models. Compared with traditional carbon-based adsorbents, it owns a simpler synthesis method and a higher adsorption capacity, as well as it is a promising candidate for water purification. |
| Author | Li, Min Nian, Ying Yue, Tianli Wang, Jianlong Han, Ximei Sun, Jing Zhang, Wentao Chen, Xinyu Shi, Shuo |
| AuthorAffiliation | College of Food Science and Engineering,Northwest A&F University,Yangling 712100,China%Qinghai Provincial Key Laboratory of Qinghai-Tibet Plateau Biological Resources,Northwest Institute of Plateau Biology,Chinese Academy of Sciences,Xining 810008,China |
| AuthorAffiliation_xml | – name: College of Food Science and Engineering,Northwest A&F University,Yangling 712100,China%Qinghai Provincial Key Laboratory of Qinghai-Tibet Plateau Biological Resources,Northwest Institute of Plateau Biology,Chinese Academy of Sciences,Xining 810008,China |
| Author_xml | – sequence: 1 givenname: Xinyu surname: Chen fullname: Chen, Xinyu organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 2 givenname: Shuo surname: Shi fullname: Shi, Shuo organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 3 givenname: Ximei surname: Han fullname: Han, Ximei organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 4 givenname: Min surname: Li fullname: Li, Min organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 5 givenname: Ying surname: Nian fullname: Nian, Ying organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 6 givenname: Jing surname: Sun fullname: Sun, Jing organization: Qinghai Provincial Key Laboratory of Qinghai-Tibet Plateau Biological Resources, Northwest Institute of Plateau Biology, Chinese Academy of Sciences, Xining 810008, China – sequence: 7 givenname: Wentao surname: Zhang fullname: Zhang, Wentao email: zhangwt@nwsuaf.edu.cn organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 8 givenname: Tianli surname: Yue fullname: Yue, Tianli organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China – sequence: 9 givenname: Jianlong surname: Wang fullname: Wang, Jianlong organization: College of Food Science and Engineering, Northwest A&F University, Yangling 712100, China |
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| Copyright | 2021 The Chemical Industry and Engineering Society of China, and Chemical Industry Press Co., Ltd. Copyright © Wanfang Data Co. Ltd. All Rights Reserved. |
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| Keywords | Cobalt/nitrogen codoping Adsorption Carbon Mechanism Tetracycline |
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Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants. Herein,... Adsorbents with simple preparation and high surface area have become increasingly prevalent for the removal of organic contaminants.Herein,a carbon nanoplate... |
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| SubjectTerms | Adsorption Carbon Cobalt/nitrogen codoping Mechanism Tetracycline |
| Title | Insights into high-efficient removal of tetracycline by a codoped mesoporous carbon adsorbent |
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