Polyacrylonitrile@TiO2 nanofibrous membrane decorated by MOF for efficient filtration and green degradation of PM2.5
[Display omitted] A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid membrane. The hybrid membrane was prepared by electrospinning technique and in situ Metal-organic frameworks (MOFs) synthesi...
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| Published in | Journal of colloid and interface science Vol. 635; pp. 598 - 610 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Inc
01.04.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid membrane. The hybrid membrane was prepared by electrospinning technique and in situ Metal-organic frameworks (MOFs) synthesis. The optimized membrane maintained a good PM2.5 capture efficiency (greater than 99%) and a pressure drop of 34 Pa. The larger specific surface area and higher pore structure enhance the filter interception effect and electrostatic interaction, which can have high applications for the filtering of PM2.5. In addition, zeolitic imidazolate framework-8 (ZIF-8) is uniformly coated on the surface of polyacrylonitrile @ TiO2 (PT) nanofiber to form N-Ti-O bonds, thus reducing the reorganization of electron-hole pairs and improving the efficiency of photodegradation. Compared with PT, the hybrid structure formed by PTZ has a higher degradation efficiency for PM2.5 (increased from 66% to 85%). The produced PTZ membrane exhibits a promising future in the collection and green degradation of PM2.5. |
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| AbstractList | [Display omitted]
A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid membrane. The hybrid membrane was prepared by electrospinning technique and in situ Metal-organic frameworks (MOFs) synthesis. The optimized membrane maintained a good PM2.5 capture efficiency (greater than 99%) and a pressure drop of 34 Pa. The larger specific surface area and higher pore structure enhance the filter interception effect and electrostatic interaction, which can have high applications for the filtering of PM2.5. In addition, zeolitic imidazolate framework-8 (ZIF-8) is uniformly coated on the surface of polyacrylonitrile @ TiO2 (PT) nanofiber to form N-Ti-O bonds, thus reducing the reorganization of electron-hole pairs and improving the efficiency of photodegradation. Compared with PT, the hybrid structure formed by PTZ has a higher degradation efficiency for PM2.5 (increased from 66% to 85%). The produced PTZ membrane exhibits a promising future in the collection and green degradation of PM2.5. A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid membrane. The hybrid membrane was prepared by electrospinning technique and in situ Metal-organic frameworks (MOFs) synthesis. The optimized membrane maintained a good PM2.5 capture efficiency (greater than 99%) and a pressure drop of 34 Pa. The larger specific surface area and higher pore structure enhance the filter interception effect and electrostatic interaction, which can have high applications for the filtering of PM2.5. In addition, zeolitic imidazolate framework-8 (ZIF-8) is uniformly coated on the surface of polyacrylonitrile @ TiO2 (PT) nanofiber to form N-Ti-O bonds, thus reducing the reorganization of electron-hole pairs and improving the efficiency of photodegradation. Compared with PT, the hybrid structure formed by PTZ has a higher degradation efficiency for PM2.5 (increased from 66% to 85%). The produced PTZ membrane exhibits a promising future in the collection and green degradation of PM2.5.A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid membrane. The hybrid membrane was prepared by electrospinning technique and in situ Metal-organic frameworks (MOFs) synthesis. The optimized membrane maintained a good PM2.5 capture efficiency (greater than 99%) and a pressure drop of 34 Pa. The larger specific surface area and higher pore structure enhance the filter interception effect and electrostatic interaction, which can have high applications for the filtering of PM2.5. In addition, zeolitic imidazolate framework-8 (ZIF-8) is uniformly coated on the surface of polyacrylonitrile @ TiO2 (PT) nanofiber to form N-Ti-O bonds, thus reducing the reorganization of electron-hole pairs and improving the efficiency of photodegradation. Compared with PT, the hybrid structure formed by PTZ has a higher degradation efficiency for PM2.5 (increased from 66% to 85%). The produced PTZ membrane exhibits a promising future in the collection and green degradation of PM2.5. |
| Author | Yang, Zhengren Feng, Yao Zhen, Yuhua Qin, Zheng Jiang, Xiaolin Yang, Wenjie Qie, Yuanyue |
| Author_xml | – sequence: 1 givenname: Zhengren surname: Yang fullname: Yang, Zhengren – sequence: 2 givenname: Yuhua surname: Zhen fullname: Zhen, Yuhua – sequence: 3 givenname: Yao surname: Feng fullname: Feng, Yao – sequence: 4 givenname: Xiaolin surname: Jiang fullname: Jiang, Xiaolin – sequence: 5 givenname: Zheng surname: Qin fullname: Qin, Zheng – sequence: 6 givenname: Wenjie surname: Yang fullname: Yang, Wenjie – sequence: 7 givenname: Yuanyue surname: Qie fullname: Qie, Yuanyue |
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A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate... A systematic study was performed on PM2.5 filtration and photodegradation performance of polyacrylonitrile @TiO2/ zeolitic imidazolate framework-8（PTZ）hybrid... |
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| Title | Polyacrylonitrile@TiO2 nanofibrous membrane decorated by MOF for efficient filtration and green degradation of PM2.5 |
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