Induced-charge electrokinetics in rotating electric fields: A linear asymptotic analysis
Concerning the electroconvective analyte manipulation in microfluidics, we describe the basic physics of fluid flow driven by rotating induced-charge electro-osmosis (ROT-ICEO), which occurs on the planar surface of a single floating electrode in an external rotating electric field. First, based on...
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| Published in | Physics of fluids (1994) Vol. 30; no. 6 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.06.2018
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| Online Access | Get full text |
| ISSN | 1070-6631 1089-7666 |
| DOI | 10.1063/1.5030579 |
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| Abstract | Concerning the electroconvective analyte manipulation in microfluidics, we
describe the basic physics of fluid flow driven by rotating induced-charge
electro-osmosis (ROT-ICEO), which occurs on the planar surface of a single
floating electrode in an external rotating electric field. First, based on a
linear asymptotic analysis, the dynamic flow stagnation line in ROT-ICEO induced
on the bipolar electrode from a rotary Debye screening charge
revolves synchronously with the applied rotating fields. A net hydrodynamic
torque is then generated that acts on any fluid or particle sample to produce
either a synchronous or asynchronous co-field rotation depending on the
frequency of the ac signal. Next, from the synergy between the hydrodynamic and
electrochemical ion relaxations, an analytical solution of the sample rotation
rate subject to ROT-ICEO slipping on an ideally polarizable surface is obtained
for different frequency ranges and determined by the transient nature of the
rotating electro-osmotic flow oscillating at twice the field frequency. To
visualize the flow field in ROT-ICEO, experiments were performed with
fluorescent tracer nanoparticles; they exhibited concentric rotational behavior
at the polarized phase interface. Formed like the arms of a nebula disk, the
four twisted tails of nanoparticles can be arbitrarily directed under
voltage-phase rectification. These experimental results are in good agreement
with our mathematical simulations using the Debye–Hückel
approximation on ROT-ICEO. |
|---|---|
| AbstractList | Concerning the electroconvective analyte manipulation in microfluidics, we describe the basic physics of fluid flow driven by rotating induced-charge electro-osmosis (ROT-ICEO), which occurs on the planar surface of a single floating electrode in an external rotating electric field. First, based on a linear asymptotic analysis, the dynamic flow stagnation line in ROT-ICEO induced on the bipolar electrode from a rotary Debye screening charge revolves synchronously with the applied rotating fields. A net hydrodynamic torque is then generated that acts on any fluid or particle sample to produce either a synchronous or asynchronous co-field rotation depending on the frequency of the ac signal. Next, from the synergy between the hydrodynamic and electrochemical ion relaxations, an analytical solution of the sample rotation rate subject to ROT-ICEO slipping on an ideally polarizable surface is obtained for different frequency ranges and determined by the transient nature of the rotating electro-osmotic flow oscillating at twice the field frequency. To visualize the flow field in ROT-ICEO, experiments were performed with fluorescent tracer nanoparticles; they exhibited concentric rotational behavior at the polarized phase interface. Formed like the arms of a nebula disk, the four twisted tails of nanoparticles can be arbitrarily directed under voltage-phase rectification. These experimental results are in good agreement with our mathematical simulations using the Debye–Hückel approximation on ROT-ICEO. Concerning the electroconvective analyte manipulation in microfluidics, we describe the basic physics of fluid flow driven by rotating induced-charge electro-osmosis (ROT-ICEO), which occurs on the planar surface of a single floating electrode in an external rotating electric field. First, based on a linear asymptotic analysis, the dynamic flow stagnation line in ROT-ICEO induced on the bipolar electrode from a rotary Debye screening charge revolves synchronously with the applied rotating fields. A net hydrodynamic torque is then generated that acts on any fluid or particle sample to produce either a synchronous or asynchronous co-field rotation depending on the frequency of the ac signal. Next, from the synergy between the hydrodynamic and electrochemical ion relaxations, an analytical solution of the sample rotation rate subject to ROT-ICEO slipping on an ideally polarizable surface is obtained for different frequency ranges and determined by the transient nature of the rotating electro-osmotic flow oscillating at twice the field frequency. To visualize the flow field in ROT-ICEO, experiments were performed with fluorescent tracer nanoparticles; they exhibited concentric rotational behavior at the polarized phase interface. Formed like the arms of a nebula disk, the four twisted tails of nanoparticles can be arbitrarily directed under voltage-phase rectification. These experimental results are in good agreement with our mathematical simulations using the Debye–Hückel approximation on ROT-ICEO. |
| Author | Tao, Ye Ren, Yukun Wang, Zhijie Liu, Weiyu |
| Author_xml | – sequence: 1 givenname: Yukun surname: Ren fullname: Ren, Yukun organization: State Key Laboratory of Robotics and System, Harbin Institute of Technology – sequence: 2 givenname: Weiyu surname: Liu fullname: Liu, Weiyu organization: School of Electronics and Control Engineering, Chang’an University – sequence: 3 givenname: Zhijie surname: Wang fullname: Wang, Zhijie organization: State Key Laboratory of Robotics and System, Harbin Institute of Technology – sequence: 4 givenname: Ye surname: Tao fullname: Tao, Ye organization: State Key Laboratory of Robotics and System, Harbin Institute of Technology |
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| Snippet | Concerning the electroconvective analyte manipulation in microfluidics, we
describe the basic physics of fluid flow driven by rotating induced-charge... Concerning the electroconvective analyte manipulation in microfluidics, we describe the basic physics of fluid flow driven by rotating induced-charge... |
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