Stable green light-emission from poly[9,9-bis(4′- n-octyloxyphenyl)fluorenyl-2,7-vinylene] synthesized via the Gilch polymerization route
A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch polymerization route and its light-emission properties were characterized and compared with those of poly(9,9-di- n-octylfluorenyl-2,7-vinylene) (...
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| Published in | Current applied physics Vol. 9; no. 2; pp. 441 - 447 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.03.2009
한국물리학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1567-1739 1878-1675 |
| DOI | 10.1016/j.cap.2008.04.002 |
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| Abstract | A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch polymerization route and its light-emission properties were characterized and compared with those of poly(9,9-di-
n-octylfluorenyl-2,7-vinylene) (PFV). As is the case for poly(alkylfluorene)s, PFV exhibits a long-wavelength emission that is additional to its emission in the blue-green region after thermal annealing or the passage of current. We have successfully suppressed this long-wavelength emission by introducing an octyloxyphenyl group at the 9-position of the fluorene group. PBOPFV produces PL emission maxima at 478 and 510
nm and no significant changes were found in its PL emission spectrum even after thermal annealing at 150
°C for 2
h. Light-emitting devices were fabricated with ITO/PEDOT:PSS/polymer/LiF/Al configurations. The EL spectrum of the device constructed using PFV was found to undergo significant changes during device operation, whereas the EL spectrum of the device constructed using PBOPFV was found to be stable. |
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| AbstractList | A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch polymerization route and its light-emission properties were characterized and compared with those of poly(9,9-di-
n-octylfluorenyl-2,7-vinylene) (PFV). As is the case for poly(alkylfluorene)s, PFV exhibits a long-wavelength emission that is additional to its emission in the blue-green region after thermal annealing or the passage of current. We have successfully suppressed this long-wavelength emission by introducing an octyloxyphenyl group at the 9-position of the fluorene group. PBOPFV produces PL emission maxima at 478 and 510
nm and no significant changes were found in its PL emission spectrum even after thermal annealing at 150
°C for 2
h. Light-emitting devices were fabricated with ITO/PEDOT:PSS/polymer/LiF/Al configurations. The EL spectrum of the device constructed using PFV was found to undergo significant changes during device operation, whereas the EL spectrum of the device constructed using PBOPFV was found to be stable. A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch polymerization route and its light-emission properties were characterized and compared with those of poly(9,9-di-n-octylfluorenyl-2,7-vinylene) (PFV). As is the case for poly(alkylfluorene)s, PFV exhibits a long-wavelength emission that is additional to its emission in the blue-green region after thermal annealing or the passage of current. We have successfully suppressed this long-wavelength emission by introducing an octyloxyphenyl group at the 9-position of the fluorene group. PBOPFV produces PL emission maxima at 478 and 510 nm and no significant changes were found in its PL emission spectrum even after thermal annealing at 150 ℃ for 2 h. Light-emitting devices were fabricated with ITO/PEDOT:PSS/polymer/LiF/Al configurations. The EL spectrum of the device constructed using PFV was found to undergo significant changes during device operation, whereas the EL spectrum of the device constructed using PBOPFV was found to be stable. KCI Citation Count: 3 |
| Author | Kang, Jong-Min Chu, Hye-Yong Eom, Jae-Hoon Shim, Hong-Ku Cho, Hoon-Je Lee, Jeong-Ik Hwang, Do-Hoon Lee, Changhee Park, Moo-Jin Jin, Sung-Ho |
| Author_xml | – sequence: 1 givenname: Do-Hoon surname: Hwang fullname: Hwang, Do-Hoon email: dhhwang@kumoh.ac.kr organization: Department of Applied Chemistry, Kumoh National Institute of Technology, Kumi 730-701, Republic of Korea – sequence: 2 givenname: Jong-Min surname: Kang fullname: Kang, Jong-Min organization: Department of Applied Chemistry, Kumoh National Institute of Technology, Kumi 730-701, Republic of Korea – sequence: 3 givenname: Jae-Hoon surname: Eom fullname: Eom, Jae-Hoon organization: Department of Applied Chemistry, Kumoh National Institute of Technology, Kumi 730-701, Republic of Korea – sequence: 4 givenname: Moo-Jin surname: Park fullname: Park, Moo-Jin organization: Polymer Science and Engineering Program, Korea Advanced Institute of Science and Technology, Daejeon 305-701, Republic of Korea – sequence: 5 givenname: Hoon-Je surname: Cho fullname: Cho, Hoon-Je organization: Department of Chemistry and School of Molecular Science (BK21), Korea Advanced Institute of Science and Technology, Daejeon 305-701, Republic of Korea – sequence: 6 givenname: Jeong-Ik surname: Lee fullname: Lee, Jeong-Ik organization: IT Convergence and Components Laboratory, Electronics and Telecommunications Research Institute, Daejeon 305-350, Republic of Korea – sequence: 7 givenname: Hye-Yong surname: Chu fullname: Chu, Hye-Yong organization: IT Convergence and Components Laboratory, Electronics and Telecommunications Research Institute, Daejeon 305-350, Republic of Korea – sequence: 8 givenname: Changhee surname: Lee fullname: Lee, Changhee organization: School of Electrical Engineering and Computer Science, Seoul National University, Seoul 151-744, Republic of Korea – sequence: 9 givenname: Sung-Ho surname: Jin fullname: Jin, Sung-Ho organization: Department of Chemistry Education, Pusan National University, Pusan 609-735, Republic of Korea – sequence: 10 givenname: Hong-Ku surname: Shim fullname: Shim, Hong-Ku organization: Department of Chemistry and School of Molecular Science (BK21), Korea Advanced Institute of Science and Technology, Daejeon 305-701, Republic of Korea |
| BackLink | https://www.kci.go.kr/kciportal/ci/sereArticleSearch/ciSereArtiView.kci?sereArticleSearchBean.artiId=ART001326433$$DAccess content in National Research Foundation of Korea (NRF) |
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| CitedBy_id | crossref_primary_10_1016_j_matchemphys_2011_06_029 crossref_primary_10_1016_j_cplett_2010_08_036 crossref_primary_10_1039_c1gc15136c |
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| Keywords | Electroluminescence 72.80.Le Poly(arylenevinylene) derivative Light-emitting diode Photoluminescence |
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| Snippet | A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch... A new fluorene-containing poly(arylenevinylene) derivative, poly[9,9-bis(4-octyloxyphenyl)fluorenyl-2,7-vinylene] (PBOPFV), was synthesized via the Gilch... |
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| StartPage | 441 |
| SubjectTerms | Electroluminescence Light-emitting diode Photoluminescence Poly(arylenevinylene) derivative 물리학 |
| Title | Stable green light-emission from poly[9,9-bis(4′- n-octyloxyphenyl)fluorenyl-2,7-vinylene] synthesized via the Gilch polymerization route |
| URI | https://dx.doi.org/10.1016/j.cap.2008.04.002 https://www.kci.go.kr/kciportal/ci/sereArticleSearch/ciSereArtiView.kci?sereArticleSearchBean.artiId=ART001326433 |
| Volume | 9 |
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| ispartofPNX | Current Applied Physics, 2009, 9(3), , pp.441-447 |
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