2D/2D Heterojunction systems for the removal of organic pollutants: A review

Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable photocatalyst. 2D materials-based heterojunction has aroused widespread concerns in photocatalysis because of its merits in more active sites, adjus...

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Published inAdvances in colloid and interface science Vol. 297; p. 102540
Main Authors Qin, Meng-Zhu, Fu, Wen-Xin, Guo, Hai, Niu, Cheng-Gang, Huang, Da-Wei, Liang, Chao, Yang, Ya-Ya, Liu, Hui-Yun, Tang, Ning, Fan, Qian-Qian
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.11.2021
Subjects
Degradation
Intimate contact interface
Photocatalysis
Synthesis
Types
Degradation
Intimate contact interface
Types
Synthesis
Photocatalysis
Online AccessGet full text
ISSN0001-8686
1873-3727
1873-3727
DOI10.1016/j.cis.2021.102540

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Abstract Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable photocatalyst. 2D materials-based heterojunction has aroused widespread concerns in photocatalysis because of its merits in more active sites, adjustable band gaps and shorter charge transfer distance. Among various 2D heterojunction systems, 2D/2D heterojunction with a face-to-face contact interface is regarded as a highly promising photocatalyst. Due to the strong coupling interface in 2D/2D heterojunction, the separation and migration of photoexcited electron-hole pairs are facilitated, which enhances the photocatalytic performance. Thus, the design of 2D/2D heterojunction can become a potential model for expanding the application of photocatalysis in the removal of organic pollutants. Herein, in this review, we first summarize the fundamental principles, classification, and strategies for elevating photocatalytic performance. Then, the synthesis and application of the 2D/2D heterojunction system for the removal of organic pollutants are discussed. Finally, the challenges and perspectives in 2D/2D heterojunction photocatalysts and their application for removing organic pollutants are presented. [Display omitted] •The fundamental principles and synthesis methods of 2D/2D heterojunction.•Type I, type II, p-n junction, Z-scheme, S-scheme and Schottky junction.•The photodegradation performance of 2D/2D heterojunction systems.•The current challenges and future development directions of 2D/2D heterojunctions.
AbstractList Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable photocatalyst. 2D materials-based heterojunction has aroused widespread concerns in photocatalysis because of its merits in more active sites, adjustable band gaps and shorter charge transfer distance. Among various 2D heterojunction systems, 2D/2D heterojunction with a face-to-face contact interface is regarded as a highly promising photocatalyst. Due to the strong coupling interface in 2D/2D heterojunction, the separation and migration of photoexcited electron-hole pairs are facilitated, which enhances the photocatalytic performance. Thus, the design of 2D/2D heterojunction can become a potential model for expanding the application of photocatalysis in the removal of organic pollutants. Herein, in this review, we first summarize the fundamental principles, classification, and strategies for elevating photocatalytic performance. Then, the synthesis and application of the 2D/2D heterojunction system for the removal of organic pollutants are discussed. Finally, the challenges and perspectives in 2D/2D heterojunction photocatalysts and their application for removing organic pollutants are presented.Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable photocatalyst. 2D materials-based heterojunction has aroused widespread concerns in photocatalysis because of its merits in more active sites, adjustable band gaps and shorter charge transfer distance. Among various 2D heterojunction systems, 2D/2D heterojunction with a face-to-face contact interface is regarded as a highly promising photocatalyst. Due to the strong coupling interface in 2D/2D heterojunction, the separation and migration of photoexcited electron-hole pairs are facilitated, which enhances the photocatalytic performance. Thus, the design of 2D/2D heterojunction can become a potential model for expanding the application of photocatalysis in the removal of organic pollutants. Herein, in this review, we first summarize the fundamental principles, classification, and strategies for elevating photocatalytic performance. Then, the synthesis and application of the 2D/2D heterojunction system for the removal of organic pollutants are discussed. Finally, the challenges and perspectives in 2D/2D heterojunction photocatalysts and their application for removing organic pollutants are presented.
Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable photocatalyst. 2D materials-based heterojunction has aroused widespread concerns in photocatalysis because of its merits in more active sites, adjustable band gaps and shorter charge transfer distance. Among various 2D heterojunction systems, 2D/2D heterojunction with a face-to-face contact interface is regarded as a highly promising photocatalyst. Due to the strong coupling interface in 2D/2D heterojunction, the separation and migration of photoexcited electron-hole pairs are facilitated, which enhances the photocatalytic performance. Thus, the design of 2D/2D heterojunction can become a potential model for expanding the application of photocatalysis in the removal of organic pollutants. Herein, in this review, we first summarize the fundamental principles, classification, and strategies for elevating photocatalytic performance. Then, the synthesis and application of the 2D/2D heterojunction system for the removal of organic pollutants are discussed. Finally, the challenges and perspectives in 2D/2D heterojunction photocatalysts and their application for removing organic pollutants are presented. [Display omitted] •The fundamental principles and synthesis methods of 2D/2D heterojunction.•Type I, type II, p-n junction, Z-scheme, S-scheme and Schottky junction.•The photodegradation performance of 2D/2D heterojunction systems.•The current challenges and future development directions of 2D/2D heterojunctions.
ArticleNumber 102540
Author Fu, Wen-Xin
Huang, Da-Wei
Fan, Qian-Qian
Guo, Hai
Liang, Chao
Tang, Ning
Liu, Hui-Yun
Niu, Cheng-Gang
Yang, Ya-Ya
Qin, Meng-Zhu
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  surname: Qin
  fullname: Qin, Meng-Zhu
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  fullname: Fu, Wen-Xin
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  givenname: Hai
  surname: Guo
  fullname: Guo, Hai
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  givenname: Cheng-Gang
  surname: Niu
  fullname: Niu, Cheng-Gang
  email: cgniu@hnu.edu.cn
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  fullname: Yang, Ya-Ya
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
– sequence: 8
  givenname: Hui-Yun
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  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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  surname: Fan
  fullname: Fan, Qian-Qian
  organization: College of Environmental Science and Engineering, Key Laboratory of Environmental Biology and Pollution Control, Ministry of Education, Hunan University, Changsha, PR China
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Snippet Photocatalysis is considered to be an effective way to remove organic pollutants, but the key to photocatalysis is finding a high-efficiency and stable...
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SubjectTerms Degradation
Intimate contact interface
Photocatalysis
Synthesis
Types
Title 2D/2D Heterojunction systems for the removal of organic pollutants: A review
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