Visible-light photooxidation of trichloroethylene by Cr–Al-MCM-41
In the present study, the photooxidation of gaseous trichloroethylene (TCE) was performed on Cr–Al-MCM-41 (predominantly a SiO 2 framework) under visible light and UV light. This mesoporous Cr-containing MCM-41 material is a promising photocatalyst and exhibits excellent photoactivity. Moreover, the...
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Published in | Journal of catalysis Vol. 230; no. 1; pp. 158 - 165 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Amsterdam
Elsevier Inc
15.02.2005
Elsevier |
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Abstract | In the present study, the photooxidation of gaseous trichloroethylene (TCE) was performed on Cr–Al-MCM-41 (predominantly a SiO
2 framework) under visible light and UV light. This mesoporous Cr-containing MCM-41 material is a promising photocatalyst and exhibits excellent photoactivity. Moreover, the products of photooxidation under visible light are similar to those under UV-light illumination. The photocatalysis process occurs on isolated Cr
6+ ions supported on a predominantly SiO
2 framework. A possible mechanism leading to the photooxidation of TCE together with the detection of intermediates by gas chromatography-mass spectrometry is reported here. |
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AbstractList | In the present study, the photooxidation of gaseous trichloroethylene (TCE) was performed on Cr–Al-MCM-41 (predominantly a SiO
2 framework) under visible light and UV light. This mesoporous Cr-containing MCM-41 material is a promising photocatalyst and exhibits excellent photoactivity. Moreover, the products of photooxidation under visible light are similar to those under UV-light illumination. The photocatalysis process occurs on isolated Cr
6+ ions supported on a predominantly SiO
2 framework. A possible mechanism leading to the photooxidation of TCE together with the detection of intermediates by gas chromatography-mass spectrometry is reported here. |
Author | Martyanov, Igor N. Ranjit, Koodali T. Klabunde, K.J. Uma, S. Rodrigues, Shalini |
Author_xml | – sequence: 1 givenname: Shalini surname: Rodrigues fullname: Rodrigues, Shalini – sequence: 2 givenname: Koodali T. surname: Ranjit fullname: Ranjit, Koodali T. – sequence: 3 givenname: S. surname: Uma fullname: Uma, S. – sequence: 4 givenname: Igor N. surname: Martyanov fullname: Martyanov, Igor N. – sequence: 5 givenname: K.J. surname: Klabunde fullname: Klabunde, K.J. email: kenjk@ksu.edu |
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Keywords | Trichloroethylene Visible light UV irradiation Mesoporous Cr–Al-MCM-41 Photocatalysis Aluminium Porous material Mesoporosity Ultraviolet irradiation Chlorocarbon Visible radiation Chromium Cr-Al-MCM-41 Photooxidation |
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Snippet | In the present study, the photooxidation of gaseous trichloroethylene (TCE) was performed on Cr–Al-MCM-41 (predominantly a SiO
2 framework) under visible light... |
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SubjectTerms | Catalysis Chemistry Colloidal state and disperse state Cr–Al-MCM-41 Exact sciences and technology General and physical chemistry Mesoporous Photocatalysis Photochemistry Physical chemistry of induced reactions (with radiations, particles and ultrasonics) Porous materials Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Trichloroethylene UV irradiation Visible light |
Title | Visible-light photooxidation of trichloroethylene by Cr–Al-MCM-41 |
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