Performance improvement of perovskite solar cells by employing a CdSe quantum dot/PCBM composite as an electron transport layer
Organic–inorganic hybrid perovskites have recently attracted considerable interest for application in solar cells due to their low cost, high absorption coefficient and high power conversion efficiency (PCE). Herein, we utilize a CdSe quantum dot/PCBM composite as an electron transport layer (ETL) t...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 5; no. 33; pp. 17499 - 17505 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Organic–inorganic hybrid perovskites have recently attracted considerable interest for application in solar cells due to their low cost, high absorption coefficient and high power conversion efficiency (PCE). Herein, we utilize a CdSe quantum dot/PCBM composite as an electron transport layer (ETL) to investigate the structure, stability and PCE of CH 3 NH 3 PbI 3−x Cl x perovskite solar cells. It is found that adsorption of the CdSe/PCBM composite reduces the roughness of the perovskite, leading to a high-quality film with a compact morphology. Density functional theory (DFT) based first-principles calculations show that CdSe enhances the chemical stability of CH 3 NH 3 PbI 3−x Cl x involving strong atomic orbital hybridization. Interestingly, an inorganic-terminated perovskite surface has much stronger interaction with CdSe compared to the surface with organic CH 3 NH 3 termination, with noticeable interfacial charge redistribution. Experiments on solar cells incorporating the CdSe/PCBM composite as the ETL show enhanced photocurrent and fill factor, which is related to the in-built electric field between CH 3 NH 3 PbI 3−x Cl x and CdSe that greatly facilitates the separation of electron and hole pairs. We show an improved PCE of 13.7% with enhanced device stability in a highly humid atmosphere. These joint theoretical–experimental results may provide a new aspect for improving the structural stability and operating performance of optoelectronic devices based on perovskite structures. |
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| AbstractList | Organic–inorganic hybrid perovskites have recently attracted considerable interest for application in solar cells due to their low cost, high absorption coefficient and high power conversion efficiency (PCE). Herein, we utilize a CdSe quantum dot/PCBM composite as an electron transport layer (ETL) to investigate the structure, stability and PCE of CH 3 NH 3 PbI 3−x Cl x perovskite solar cells. It is found that adsorption of the CdSe/PCBM composite reduces the roughness of the perovskite, leading to a high-quality film with a compact morphology. Density functional theory (DFT) based first-principles calculations show that CdSe enhances the chemical stability of CH 3 NH 3 PbI 3−x Cl x involving strong atomic orbital hybridization. Interestingly, an inorganic-terminated perovskite surface has much stronger interaction with CdSe compared to the surface with organic CH 3 NH 3 termination, with noticeable interfacial charge redistribution. Experiments on solar cells incorporating the CdSe/PCBM composite as the ETL show enhanced photocurrent and fill factor, which is related to the in-built electric field between CH 3 NH 3 PbI 3−x Cl x and CdSe that greatly facilitates the separation of electron and hole pairs. We show an improved PCE of 13.7% with enhanced device stability in a highly humid atmosphere. These joint theoretical–experimental results may provide a new aspect for improving the structural stability and operating performance of optoelectronic devices based on perovskite structures. Organic–inorganic hybrid perovskites have recently attracted considerable interest for application in solar cells due to their low cost, high absorption coefficient and high power conversion efficiency (PCE). Herein, we utilize a CdSe quantum dot/PCBM composite as an electron transport layer (ETL) to investigate the structure, stability and PCE of CH₃NH₃PbI₃₋ₓClₓ perovskite solar cells. It is found that adsorption of the CdSe/PCBM composite reduces the roughness of the perovskite, leading to a high-quality film with a compact morphology. Density functional theory (DFT) based first-principles calculations show that CdSe enhances the chemical stability of CH₃NH₃PbI₃₋ₓClₓ involving strong atomic orbital hybridization. Interestingly, an inorganic-terminated perovskite surface has much stronger interaction with CdSe compared to the surface with organic CH₃NH₃ termination, with noticeable interfacial charge redistribution. Experiments on solar cells incorporating the CdSe/PCBM composite as the ETL show enhanced photocurrent and fill factor, which is related to the in-built electric field between CH₃NH₃PbI₃₋ₓClₓ and CdSe that greatly facilitates the separation of electron and hole pairs. We show an improved PCE of 13.7% with enhanced device stability in a highly humid atmosphere. These joint theoretical–experimental results may provide a new aspect for improving the structural stability and operating performance of optoelectronic devices based on perovskite structures. |
| Author | Zhou, Tingwei Zang, Zhigang Leng, Chongqian Lu, Shirong Zhou, Miao Zeng, Xiaofeng Tang, Xiaosheng Hu, Wei Wang, Ming Fang, Liang |
| Author_xml | – sequence: 1 givenname: Xiaofeng surname: Zeng fullname: Zeng, Xiaofeng organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 2 givenname: Tingwei surname: Zhou fullname: Zhou, Tingwei organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 3 givenname: Chongqian surname: Leng fullname: Leng, Chongqian organization: Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 401122, China – sequence: 4 givenname: Zhigang surname: Zang fullname: Zang, Zhigang organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 5 givenname: Ming surname: Wang fullname: Wang, Ming organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 6 givenname: Wei surname: Hu fullname: Hu, Wei organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 7 givenname: Xiaosheng surname: Tang fullname: Tang, Xiaosheng organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 – sequence: 8 givenname: Shirong surname: Lu fullname: Lu, Shirong organization: Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 401122, China – sequence: 9 givenname: Liang surname: Fang fullname: Fang, Liang organization: Department of Applied Physics, College of Physics, Chongqing University, Chongqing 401331, China – sequence: 10 givenname: Miao orcidid: 0000-0003-1390-372X surname: Zhou fullname: Zhou, Miao organization: Key Laboratory of Optoelectronic Technology & Systems, Ministry of Education, College of Optoelectronic Engineering, Chongqing University, Chongqing 400044 |
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