Tetraalkoxylated-PPV derivative: An efficient and pure green electroluminescent polymer with good solution processability
A new solution-processable tetraalkoxy-substituted poly(1,4-phenylenevinylene) derivative, poly{[2-(3′,7′-dimethyloctyloxy)-3,5,6-trimethoxy]-1,4-phenylenevinylene} (TALK-PPV), was synthesized through a dehydrohalogenation polymerization route, and its light-emitting properties were investigated. Th...
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| Published in | Current applied physics Vol. 9; no. 4; pp. 861 - 865 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.07.2009
한국물리학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1567-1739 1878-1675 1567-1739 |
| DOI | 10.1016/j.cap.2008.08.004 |
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| Abstract | A new solution-processable tetraalkoxy-substituted poly(1,4-phenylenevinylene) derivative, poly{[2-(3′,7′-dimethyloctyloxy)-3,5,6-trimethoxy]-1,4-phenylenevinylene} (TALK-PPV), was synthesized through a dehydrohalogenation polymerization route, and its light-emitting properties were investigated. The TALK-PPV showed highly blue-shifted UV–visible absorption and PL emission spectra compared to the dialkoxy-substituted PPV derivatives. This is because of the disturbance to the π-conjugation caused by a steric hindered structure. The TALK-PPV thin film exhibited an absorption peak at 446nm, with an onset at 515nm. Its PL emission maximum was at 554nm. Cyclic voltammetric analysis showed the HOMO and LUMO energy levels of the TALK-PPV to be 5.77 and 3.36eV, respectively. Light-emitting devices were fabricated with an ITO (indium-tin oxide)/PEDOT/polymer/Ca/Al configuration. The TALK-PPV component leads to pure green light emission with a CIE 1931 chromaticity of (0.20, 0.74) at 100cd/m2 brightness, which is very close to the standard green (0.21, 0.71) demanded by the NTSC (National Television System Committee). The maximum brightness of this device was 24,900cd/m2 with an efficiency of 1.45cd/A. |
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| AbstractList | A new solution-processable tetraalkoxy-substituted poly(1,4-phenylenevinylene) derivative, poly{[2-(3′,7′-dimethyloctyloxy)-3,5,6-trimethoxy]-1,4-phenylenevinylene} (TALK-PPV), was synthesized through a dehydrohalogenation polymerization route, and its light-emitting properties were investigated. The TALK-PPV showed highly blue-shifted UV–visible absorption and PL emission spectra compared to the dialkoxy-substituted PPV derivatives. This is because of the disturbance to the π-conjugation caused by a steric hindered structure. The TALK-PPV thin film exhibited an absorption peak at 446nm, with an onset at 515nm. Its PL emission maximum was at 554nm. Cyclic voltammetric analysis showed the HOMO and LUMO energy levels of the TALK-PPV to be 5.77 and 3.36eV, respectively. Light-emitting devices were fabricated with an ITO (indium-tin oxide)/PEDOT/polymer/Ca/Al configuration. The TALK-PPV component leads to pure green light emission with a CIE 1931 chromaticity of (0.20, 0.74) at 100cd/m2 brightness, which is very close to the standard green (0.21, 0.71) demanded by the NTSC (National Television System Committee). The maximum brightness of this device was 24,900cd/m2 with an efficiency of 1.45cd/A. A new solution-processable tetraalkoxy-substituted poly(1,4-phenylenevinylene) derivative, poly{[2- (3',7'-dimethyloctyloxy)-3,5,6-trimethoxy]-1,4-phenylenevinylene} (TALK-PPV), was synthesized through a dehydrohalogenation polymerization route, and its light-emitting properties were investigated. The TALK-PPV showed highly blue-shifted UV–visible absorption and PL emission spectra compared to the dialkoxy-substituted PPV derivatives. This is because of the disturbance to the p-conjugation caused by a steric hindered structure. The TALK-PPV thin film exhibited an absorption peak at 446 nm, with an onset at 515 nm. Its PL emission maximum was at 554 nm. Cyclic voltammetric analysis showed the HOMO and LUMO energy levels of the TALK-PPV to be 5.77 and 3.36 eV, respectively. Light-emitting devices were fabricated with an ITO (indium-tin oxide)/PEDOT/polymer/Ca/Al configuration. The TALK-PPV component leads to pure green light emission with a CIE 1931 chromaticity of (0.20, 0.74) at 100 cd/㎡ brightness, which is very close to the standard green (0.21, 0.71) demanded by the NTSC (National Television System Committee). The maximum brightness of this device was 24,900 cd/㎡ with an efficiency of 1.45 cd/A. A new solution-processable tetraalkoxy-substituted poly(1,4-phenylenevinylene) derivative, poly{[2- (3',7'-dimethyloctyloxy)-3,5,6-trimethoxy]-1,4-phenylenevinylene} (TALK-PPV), was synthesized through a dehydrohalogenation polymerization route, and its light-emitting properties were investigated. The TALK-PPV showed highly blue-shifted UV–visible absorption and PL emission spectra compared to the dialkoxy-substituted PPV derivatives. This is because of the disturbance to the p-conjugation caused by a steric hindered structure. The TALK-PPV thin film exhibited an absorption peak at 446 nm, with an onset at 515 nm. Its PL emission maximum was at 554 nm. Cyclic voltammetric analysis showed the HOMO and LUMO energy levels of the TALK-PPV to be 5.77 and 3.36 eV, respectively. Light-emitting devices were fabricated with an ITO (indium-tin oxide)/PEDOT/polymer/Ca/Al configuration. The TALK-PPV component leads to pure green light emission with a CIE 1931 chromaticity of (0.20, 0.74) at 100 cd/㎡ brightness, which is very close to the standard green (0.21, 0.71) demanded by the NTSC (National Television System Committee). The maximum brightness of this device was 24,900 cd/㎡ with an efficiency of 1.45 cd/A. KCI Citation Count: 4 |
| Author | Son, Jhun-Mo Lee, Ji-Hoon Kim, Kyu-Sik Hwang, Do-Hoon Kee, In-Seo Kang, In-Nam Park, Moo-Jin |
| Author_xml | – sequence: 1 givenname: Ji-Hoon surname: Lee fullname: Lee, Ji-Hoon email: jihoonli@cjnu.ac.kr, jihoonli@hanafos.com organization: Department of Polymer Science and Engineering, Chungju National University, Chungju 380-702, Republic of Korea – sequence: 2 givenname: In-Seo surname: Kee fullname: Kee, In-Seo organization: Samsung Advanced Institute of Technology, P.O. Box 111, Suwon 440-600, Republic of Korea – sequence: 3 givenname: In-Nam surname: Kang fullname: Kang, In-Nam organization: Department of Chemistry, The Catholic University of Korea, Bucheon 420-743, Republic of Korea – sequence: 4 givenname: Jhun-Mo surname: Son fullname: Son, Jhun-Mo organization: Samsung Advanced Institute of Technology, P.O. Box 111, Suwon 440-600, Republic of Korea – sequence: 5 givenname: Kyu-Sik surname: Kim fullname: Kim, Kyu-Sik organization: Samsung Advanced Institute of Technology, P.O. Box 111, Suwon 440-600, Republic of Korea – sequence: 6 givenname: Moo-Jin surname: Park fullname: Park, Moo-Jin organization: Department of Applied Chemistry, Kumoh National Institute of Technology, Kumi 730-701, Republic of Korea – sequence: 7 givenname: Do-Hoon surname: Hwang fullname: Hwang, Do-Hoon email: dhhwang@kumoh.ac.kr organization: Department of Applied Chemistry, Kumoh National Institute of Technology, Kumi 730-701, Republic of Korea |
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| CitedBy_id | crossref_primary_10_1088_1674_1056_22_11_117805 crossref_primary_10_1002_macp_201000236 crossref_primary_10_1016_j_synthmet_2012_01_027 crossref_primary_10_1016_j_jlumin_2011_03_021 |
| Cites_doi | 10.1038/347539a0 10.1080/10587259808044509 10.1002/(SICI)1521-4095(199910)11:15<1281::AID-ADMA1281>3.0.CO;2-6 10.1016/j.synthmet.2008.01.016 10.1021/ma00060a001 10.1021/jp048421g 10.1016/S0379-6779(98)00960-6 10.1016/S1567-1739(01)00027-X 10.1126/science.270.5243.1789 10.1039/cc9960002241 10.1021/ma010666t 10.1021/ma990347q 10.1021/ma020285v 10.1021/cm960455g 10.1063/1.469521 10.1021/ma00099a010 10.1021/jp9838285 10.1038/356047a0 10.1126/science.280.5370.1741 10.1016/j.cap.2003.11.092 10.1038/376498a0 10.1002/macp.1993.021940407 10.1021/ma00060a002 10.1021/cm010593s 10.1002/(SICI)1521-3773(19980302)37:4<402::AID-ANIE402>3.0.CO;2-9 10.1002/(SICI)1521-4095(200001)12:1<42::AID-ADMA42>3.0.CO;2-F 10.1016/0379-6779(94)02562-D 10.1038/357477a0 |
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| Keywords | 85.60.Pg 68.55.am Tetraalkoxylated PPV Green polymer light-emitting diodes 72.80.Le |
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| SubjectTerms | Green polymer light-emitting diodes Tetraalkoxylated PPV 물리학 |
| Title | Tetraalkoxylated-PPV derivative: An efficient and pure green electroluminescent polymer with good solution processability |
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