The preparation and performance of visible-light-sensitized luminescent nanoparticles based on europium complex
Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by a co-precipitation-condensation method. The luminescent europium complex Eu（tta）3.bpt （tta = thenoyltrifluoroacetonate; bpt = 2-（N,N- di-ethy...
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| Published in | Chinese chemical letters Vol. 25; no. 2; pp. 247 - 252 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.02.2014
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| Abstract | Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by a co-precipitation-condensation method. The luminescent europium complex Eu（tta）3.bpt （tta = thenoyltrifluoroacetonate; bpt = 2-（N,N- di-ethylanilin-4-yl）-4,6-bis（pyrazol-l-yl）-l,3,5-triazine） was used as the active material, being encapsulated in the nanoparticles formed from 1H, 1H, 2H, 2H-perfluorooctyltrimethoxysilane （PFOTS） and poly（styrene-co-methyl methacrylate） [P（ST-co-MMA）]. The prepared nanoparticles not only can be well dispersed in water but also were of high photostability. Importantly, the nanoparticles displayed maximal excitation wavelength at 425 nm as well as an extended excitation wavelength up to 480 nm and a quantum yield for Eu3＋ luminescence of 0.22 （λex= 425 nm, room temperature）. |
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| AbstractList | A new kind of luminescent europium nanoparticles was prepared by the co-precipitation-condensation method. These nanoparticles exhibited excellent watersolubility, photostability and long-wavelength sensitized luminescence properties.
Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by a co-precipitation-condensation method. The luminescent europium complex Eu(tta)3·bpt (tta=thenoyltrifluoroacetonate; bpt=2-(N,N-di-ethylanilin-4-yl)-4,6-bis(pyrazol-1-yl)-1,3,5-triazine) was used as the active material, being encapsulated in the nanoparticles formed from 1H, 1H, 2H, 2H-perfluorooctyltrimethoxysilane (PFOTS) and poly(styrene-co-methyl methacrylate) [P(ST-co-MMA)]. The prepared nanoparticles not only can be well dispersed in water but also were of high photostability. Importantly, the nanoparticles displayed maximal excitation wavelength at 425nm as well as an extended excitation wavelength up to 480nm and a quantum yield for Eu3+ luminescence of 0.22 (λex=425nm, room temperature). Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by a co-precipitation-condensation method. The luminescent europium complex Eu（tta）3.bpt （tta = thenoyltrifluoroacetonate; bpt = 2-（N,N- di-ethylanilin-4-yl）-4,6-bis（pyrazol-l-yl）-l,3,5-triazine） was used as the active material, being encapsulated in the nanoparticles formed from 1H, 1H, 2H, 2H-perfluorooctyltrimethoxysilane （PFOTS） and poly（styrene-co-methyl methacrylate） [P（ST-co-MMA）]. The prepared nanoparticles not only can be well dispersed in water but also were of high photostability. Importantly, the nanoparticles displayed maximal excitation wavelength at 425 nm as well as an extended excitation wavelength up to 480 nm and a quantum yield for Eu3＋ luminescence of 0.22 （λex= 425 nm, room temperature）. |
| Author | Fu-Min Xue Ming-Hui Liang Zhen-Hua Wang Ling-Yu Luan Fu-Wei Li Yan Cheng Guang-Sheng Shao |
| AuthorAffiliation | Shandong Provincial Analysis and Test Center, ShanDong Academy of Science, Jinan 250014, China National Center for Nanosicence and Technology, Beijing 100190, China China Banknote Ink Company, Shanghai 201315, China |
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| CitedBy_id | crossref_primary_10_1002_cjoc_201400714 crossref_primary_10_1016_j_optmat_2014_09_036 crossref_primary_10_1134_S0965545X22700122 crossref_primary_10_1016_j_jphotochem_2019_111962 |
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| Keywords | Long-wavelength-sensitized luminescence Europium nanoparticles Bio-detection Co-precipitation-condensation |
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| Notes | Long-wavelength-sensitized luminescence;Europium nanoparticles;Co-precipitation-condensation;Bio-detection Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by a co-precipitation-condensation method. The luminescent europium complex Eu（tta）3.bpt （tta = thenoyltrifluoroacetonate; bpt = 2-（N,N- di-ethylanilin-4-yl）-4,6-bis（pyrazol-l-yl）-l,3,5-triazine） was used as the active material, being encapsulated in the nanoparticles formed from 1H, 1H, 2H, 2H-perfluorooctyltrimethoxysilane （PFOTS） and poly（styrene-co-methyl methacrylate） [P（ST-co-MMA）]. The prepared nanoparticles not only can be well dispersed in water but also were of high photostability. Importantly, the nanoparticles displayed maximal excitation wavelength at 425 nm as well as an extended excitation wavelength up to 480 nm and a quantum yield for Eu3＋ luminescence of 0.22 （λex= 425 nm, room temperature）. 11-2710/O6 |
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| PublicationDate | 2014-02-01 |
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| PublicationTitle | Chinese chemical letters |
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| PublicationYear | 2014 |
| Publisher | Elsevier B.V |
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| Snippet | Long-wavelength-sensitized luminescent materials are desired for bio-detection. In this paper, we prepared a new kind of luminescent europium nanoparticles by... A new kind of luminescent europium nanoparticles was prepared by the co-precipitation-condensation method. These nanoparticles exhibited excellent... |
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| SubjectTerms | Bio-detection Co-precipitation-condensation Europium nanoparticles Long-wavelength-sensitized luminescence 制备 可见光 基础 敏化发光 甲基丙烯酸甲酯 纳米粒子 纳米颗粒 铕配合物 |
| Title | The preparation and performance of visible-light-sensitized luminescent nanoparticles based on europium complex |
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