Reddish-orange emission from Pr3+ doped zinc alumino bismuth borate glasses
Praseodymium doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission studies. The glassy nature of these glasses has been confirmed through XRD spectral measurements. From the absorption spectra, the Judd–Ofel...
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Published in | Physica. B, Condensed matter Vol. 428; pp. 36 - 42 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
01.11.2013
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Abstract | Praseodymium doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission studies. The glassy nature of these glasses has been confirmed through XRD spectral measurements. From the absorption spectra, the Judd–Ofelt intensity parameters Ωλ (λ=2, 4 and 6) and other radiative properties like transition probability (AR), radiative lifetimes (τR) and branching ratios (βR) have been evaluated. Emission spectra were measured for different concentrations of Pr3+ ions doped glasses by exciting the glasses at 445nm. The intensity of Pr3+ emission spectra increases from 0.1 to 1mol% and beyond 1mol% concentration quenching is observed. The suitable concentration of Pr3+ ions in ZnAlBiB glasses to act as a good lasing material at reddish-orange wavelength (604nm) region has been discussed by measuring the emission cross-sections for the intense emission transition 1D2→3H4. The CIE chromaticity co-ordinates were also evaluated from the emission spectra for all the glasses to understand the suitability of these materials for reddish-orange emission. From the measured emission cross-sections and CIE chromaticity co-ordinates, it was found that 1mol% of Pr3+ is aptly suitable for the development of visible reddish-orange lasers. |
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AbstractList | Praseodymium doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission studies. The glassy nature of these glasses has been confirmed through XRD spectral measurements. From the absorption spectra, the Judd-Ofelt intensity parameters ICOI> (I>=2, 4 and 6) and other radiative properties like transition probability (AR), radiative lifetimes (IR) and branching ratios (I2R) have been evaluated. Emission spectra were measured for different concentrations of Pr3+ ions doped glasses by exciting the glasses at 445 nm. The intensity of Pr3+ emission spectra increases from 0.1 to 1 mol% and beyond 1 mol% concentration quenching is observed. The suitable concentration of Pr3+ ions in ZnAlBiB glasses to act as a good lasing material at reddish-orange wavelength (604 nm) region has been discussed by measuring the emission cross-sections for the intense emission transition 1D2a3H4. The CIE chromaticity co-ordinates were also evaluated from the emission spectra for all the glasses to understand the suitability of these materials for reddish-orange emission. From the measured emission cross-sections and CIE chromaticity co-ordinates, it was found that 1 mol% of Pr3+ is aptly suitable for the development of visible reddish-orange lasers. Praseodymium doped Zinc Alumino Bismuth Borate (ZnAIBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission studies. The glassy nature of these glasses has been confirmed through XRD spectral measurements. From the absorption spectra, the Judd-Ofelt intensity parameters Phi ( lambda ) ( lambda = 2, 4 and 6) and other radiative properties like transition probability (A(R)), radiative lifetimes ( tau (R)) and branching ratios ( beta (R)) have been evaluated. Emission spectra were measured for different concentrations of Pr3+ ions doped glasses by exciting the glasses at 445 nm. The intensity of Pr3+ emission spectra increases from 0.1 to 1 mol% and beyond 1 mol% concentration quenching is observed. The suitable concentration of Pr3+ ions in ZnAIBiB glasses to act as a good lasing material at reddish-orange wavelength (604 nm) region has been discussed by measuring the emission cross-sections for the intense emission transition (1)D(2)->(3)H(4). The CIE chromaticity co-ordinates were also evaluated from the emission spectra for all the glasses to understand the suitability of these materials for reddish-orange emission. From the measured emission cross-sections and CIE chromaticity co-ordinates, it was found that 1 mol% of Pr3+ is aptly suitable for the development of visible reddish-orange lasers. Praseodymium doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission studies. The glassy nature of these glasses has been confirmed through XRD spectral measurements. From the absorption spectra, the Judd–Ofelt intensity parameters Ωλ (λ=2, 4 and 6) and other radiative properties like transition probability (AR), radiative lifetimes (τR) and branching ratios (βR) have been evaluated. Emission spectra were measured for different concentrations of Pr3+ ions doped glasses by exciting the glasses at 445nm. The intensity of Pr3+ emission spectra increases from 0.1 to 1mol% and beyond 1mol% concentration quenching is observed. The suitable concentration of Pr3+ ions in ZnAlBiB glasses to act as a good lasing material at reddish-orange wavelength (604nm) region has been discussed by measuring the emission cross-sections for the intense emission transition 1D2→3H4. The CIE chromaticity co-ordinates were also evaluated from the emission spectra for all the glasses to understand the suitability of these materials for reddish-orange emission. From the measured emission cross-sections and CIE chromaticity co-ordinates, it was found that 1mol% of Pr3+ is aptly suitable for the development of visible reddish-orange lasers. |
Author | Rama Moorthy, L. Mahamuda, Sk Sasikala, T. Swapna, K. Srinivasa Rao, A. |
Author_xml | – sequence: 1 givenname: Sk surname: Mahamuda fullname: Mahamuda, Sk email: mahamuda.ss@gmail.com organization: Department of Physics, KL University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 2 givenname: K. surname: Swapna fullname: Swapna, K. email: kswapna80@gmail.com organization: Department of Physics, KL University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 3 givenname: A. surname: Srinivasa Rao fullname: Srinivasa Rao, A. email: drsrallam@yahoo.co.in organization: Department of Physics, KL University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 4 givenname: T. surname: Sasikala fullname: Sasikala, T. organization: Department of Physics, SV University, Tirupathi 517502, AP, India – sequence: 5 givenname: L. surname: Rama Moorthy fullname: Rama Moorthy, L. organization: Department of Physics, SV University, Tirupathi 517502, AP, India |
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Keywords | Glasses Emission cross-section Radiative properties JO parameters Colour co-ordinates Praseodymium Radiative transition Doping Photoluminescence Judd-Ofelt theory Liquid state quenching XRD Radiative lifetimes Borate glasses Branching ratio Praseodymium additions Chromaticity Absorption spectra |
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Snippet | Praseodymium doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission... Praseodymium doped Zinc Alumino Bismuth Borate (ZnAIBiB) glasses were prepared by melt quenching technique and characterized by optical absorption and emission... |
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SubjectTerms | Amorphous materials, glasses and other disordered solids Bismuth Borates Chromaticity Colour co-ordinates Condensed matter: electronic structure, electrical, magnetic, and optical properties Emission Emission analysis Emission cross-section Emission spectra Exact sciences and technology Glass Glasses JO parameters Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Photoluminescence Physics Praseodymium Quenching Radiative properties Zinc |
Title | Reddish-orange emission from Pr3+ doped zinc alumino bismuth borate glasses |
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