Anisotropic Fermi Surfaces, Electrical Transport, and Two-Dimensional Fermi Liquid Behavior in Layered Ternary Boride MoAlB

We report a study of fermiology, electrical anisotropy, and Fermi liquid properties in the layered ternary boride MoAlB, which could be peeled into two-dimensional (2D) metal borides (MBenes). By studying the quantum oscillations in comprehensive methods of magnetization, magnetothermoelectric power...

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Published inChinese physics letters Vol. 39; no. 5; pp. 57102 - 111
Main Authors Nie, Pan, Zuo, Huakun, Zhao, Lingxiao, Zhu, Zengwei
Format Journal Article
LanguageEnglish
Published Chinese Physical Society and IOP Publishing Ltd 01.05.2022
Wuhan National High Magnetic Field Center and School of Physics,Huazhong University of Science and Technology,Wuhan 430074,China%Department of Physics,Southern University of Science and Technology,Shenzhen 518055,China
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Abstract We report a study of fermiology, electrical anisotropy, and Fermi liquid properties in the layered ternary boride MoAlB, which could be peeled into two-dimensional (2D) metal borides (MBenes). By studying the quantum oscillations in comprehensive methods of magnetization, magnetothermoelectric power, and torque with the first-principle calculations, we reveal three types of bands in this system, including two 2D-like electronic bands and one complex three-dimensional-like hole band. Meanwhile, a large out-of-plane electrical anisotropy ( ρ bb / ρ aa ∼ 1100 and ρ bb / ρ cc ∼ 500, at 2 K) was observed, which is similar to those of the typical anisotropic semimetals but lower than those of some semiconductors (up to 10 5 ). After calculating the Kadowaki–Woods ratio (KWR = A / γ 2 ), we observed that the ratio of the in-plane A a , c / γ 2 is closer to the universal trend, whereas the out-of-plane A b / γ 2 severely deviates from the universality. This demonstrates a 2D Fermi liquid behavior. In addition, MoAlB cannot be unified using the modified KWR formula like other layered systems (Sr 2 RuO 4 and MoOCl 2 ). This unique feature necessitates further exploration of the Fermi liquid property of this layered molybdenum compound.
AbstractList We report a study of fermiology, electrical anisotropy, and Fermi liquid properties in the layered ternary boride MoAlB, which could be peeled into two-dimensional (2D) metal borides (MBenes). By studying the quantum oscillations in comprehensive methods of magnetization, magnetothermoelectric power, and torque with the first-principle calculations, we reveal three types of bands in this system, including two 2D-like electronic bands and one complex three-dimensional-like hole band. Meanwhile, a large out-of-plane electrical anisotropy ( ρ bb / ρ aa ∼ 1100 and ρ bb / ρ cc ∼ 500, at 2 K) was observed, which is similar to those of the typical anisotropic semimetals but lower than those of some semiconductors (up to 10 5 ). After calculating the Kadowaki–Woods ratio (KWR = A / γ 2 ), we observed that the ratio of the in-plane A a , c / γ 2 is closer to the universal trend, whereas the out-of-plane A b / γ 2 severely deviates from the universality. This demonstrates a 2D Fermi liquid behavior. In addition, MoAlB cannot be unified using the modified KWR formula like other layered systems (Sr 2 RuO 4 and MoOCl 2 ). This unique feature necessitates further exploration of the Fermi liquid property of this layered molybdenum compound.
We report a study of fermiology,electrical anisotropy,and Fermi liquid properties in the layered ternary boride MoAlB,which could be peeled into two-dimensional(2D)metal borides(MBenes).By studying the quantum oscillations in comprehensive methods of magnetization,magnetothermoelectric power,and torque with the first-principle calculations,we reveal three types of bands in this system,including two 2D-like electronic bands and one complex three-dimensional-like hole band.Meanwhile,a large out-of-plane electrical anisotropy(ρbb/ρaa~1100 and ρbb/ρcc~500,at 2 K)was observed,which is similar to those of the typical anisotropic semimetals but lower than those of some semiconductors(up to 105).After calculating the Kadowaki-Woods ratio(KWR=A/γ2),we observed that the ratio of the in-plane Aa,c/γ2 is closer to the universal trend,whereas the out-of-plane Ab/γ2 severely deviates from the universality.This demonstrates a 2D Fermi liquid behavior.In addition,MoAlB cannot be unified using the modified KWR formula like other layered systems(Sr2RuO4 and MoOCl2).This unique feature necessitates further exploration of the Fermi liquid property of this layered molybdenum compound.
Author Nie, Pan
Zuo, Huakun
Zhu, Zengwei
Zhao, Lingxiao
AuthorAffiliation Wuhan National High Magnetic Field Center and School of Physics,Huazhong University of Science and Technology,Wuhan 430074,China%Department of Physics,Southern University of Science and Technology,Shenzhen 518055,China
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CitedBy_id crossref_primary_10_1016_j_mtphys_2023_101060
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Snippet We report a study of fermiology, electrical anisotropy, and Fermi liquid properties in the layered ternary boride MoAlB, which could be peeled into...
We report a study of fermiology,electrical anisotropy,and Fermi liquid properties in the layered ternary boride MoAlB,which could be peeled into...
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StartPage 57102
Title Anisotropic Fermi Surfaces, Electrical Transport, and Two-Dimensional Fermi Liquid Behavior in Layered Ternary Boride MoAlB
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