Resistive switching properties and conduction mechanisms of LaSmOx thin film by RF sputtering for RRAM applications

[Display omitted] •Oxygen vacancies dominate the conduction mechanism of the LSO thin film.•The plasma gas influences the surface morphology, leading to change the RS stability.•The formation of AlOx interface has great effect on the RS performance. Polycrystalline LaSmOx (LSO) thin films were prepa...

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Published inMaterials science & engineering. B, Solid-state materials for advanced technology Vol. 271; p. 115313
Main Authors Chu, Yu-Tseng, Tsai, Meng-Hung, Huang, Cheng-Liang
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 01.09.2021
Elsevier BV
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Abstract [Display omitted] •Oxygen vacancies dominate the conduction mechanism of the LSO thin film.•The plasma gas influences the surface morphology, leading to change the RS stability.•The formation of AlOx interface has great effect on the RS performance. Polycrystalline LaSmOx (LSO) thin films were prepared by using RF sputtering and the bipolar resistive switching (BRS) properties in the Al/LSO/ITO structure were investigated. The impact of Ar/O2 ratio, film thickness and post metal annealing (PMA) condition on the resistive switching (RS) properties were also studied. The conductive mechanism is mainly dominated by the numbers of oxygen vacancies, which can be controlled through a different deposition atmosphere (Ar/O2) ratio and film thickness. In addition, the resistive switching characteristics can be improved by post metal annealing treatment due to film densification and the formation of AlOx interface layer in between the top electrode and the LaSmOx thin film. The optimized RRAM device revealed a profound improvement in the switching cycles, which can be as high as 4580.
AbstractList [Display omitted] •Oxygen vacancies dominate the conduction mechanism of the LSO thin film.•The plasma gas influences the surface morphology, leading to change the RS stability.•The formation of AlOx interface has great effect on the RS performance. Polycrystalline LaSmOx (LSO) thin films were prepared by using RF sputtering and the bipolar resistive switching (BRS) properties in the Al/LSO/ITO structure were investigated. The impact of Ar/O2 ratio, film thickness and post metal annealing (PMA) condition on the resistive switching (RS) properties were also studied. The conductive mechanism is mainly dominated by the numbers of oxygen vacancies, which can be controlled through a different deposition atmosphere (Ar/O2) ratio and film thickness. In addition, the resistive switching characteristics can be improved by post metal annealing treatment due to film densification and the formation of AlOx interface layer in between the top electrode and the LaSmOx thin film. The optimized RRAM device revealed a profound improvement in the switching cycles, which can be as high as 4580.
Polycrystalline LaSmOx (LSO) thin films were prepared by using RF sputtering and the bipolar resistive switching (BRS) properties in the Al/LSO/ITO structure were investigated. The impact of Ar/O2 ratio, film thickness and post metal annealing (PMA) condition on the resistive switching (RS) properties were also studied. The conductive mechanism is mainly dominated by the numbers of oxygen vacancies, which can be controlled through a different deposition atmosphere (Ar/O2) ratio and film thickness. In addition, the resistive switching characteristics can be improved by post metal annealing treatment due to film densification and the formation of AlOx interface layer in between the top electrode and the LaSmOx thin film. The optimized RRAM device revealed a profound improvement in the switching cycles, which can be as high as 4580.
ArticleNumber 115313
Author Chu, Yu-Tseng
Huang, Cheng-Liang
Tsai, Meng-Hung
Author_xml – sequence: 1
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  givenname: Cheng-Liang
  surname: Huang
  fullname: Huang, Cheng-Liang
  email: huangcl@mail.ncku.edu.tw
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RF sputtering
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LaSmOx
Post metal annealing
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Snippet [Display omitted] •Oxygen vacancies dominate the conduction mechanism of the LSO thin film.•The plasma gas influences the surface morphology, leading to change...
Polycrystalline LaSmOx (LSO) thin films were prepared by using RF sputtering and the bipolar resistive switching (BRS) properties in the Al/LSO/ITO structure...
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SubjectTerms Annealing
Densification
Film thickness
LaSmOx
Polycrystalline
Post metal annealing
RF sputtering
RRAM
Sputtering
Switching
Thin films
Title Resistive switching properties and conduction mechanisms of LaSmOx thin film by RF sputtering for RRAM applications
URI https://dx.doi.org/10.1016/j.mseb.2021.115313
https://www.proquest.com/docview/2572610479
Volume 271
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