Hydrothermal Valorization of Biosugars with Heterogeneous Catalysts: Advances, Catalyst Deactivation, Mitigation Strategies and Perspectives
Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high‐performance catalysts. To assist the next‐stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent adva...
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| Published in | ChemSusChem Vol. 18; no. 2; pp. e202401405 - n/a |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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14.01.2025
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| Abstract | Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high‐performance catalysts. To assist the next‐stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent advances in biosugar hydrothermal valorization using heterogeneous catalysts, (2) the deactivation process of catalysts based on recycling tests of representative biosugar hydrothermal treatments, (3) state‐of‐the‐art understandings of the deactivation mechanisms of heterogeneous catalysts, and (4) strategies for preparing durable catalysts and the regeneration of deactivated catalysts. Based on the review, challenges and perspectives are proposed. Some remarkable achievements in heterogeneous catalysis of biosugars are highlighted. The understanding of catalyst durability needs to be further enhanced based on full examination of the catalytic performance based on the conversion of substrates, the yield, and selectivity of products. Further, a full examination of the physiochemical changes based on multiple characterization techniques is required to eclucidate the relationships between treatment variables and catalyst durability. Collectively, a clear understanding of the relationships between chemical reaction pathways, treatment variables, and the physiochemistry of catalysts is encouraged to be gained to advise the development of heterogeneous catalysts for long‐term and efficient hydrothermal upgrading of biosugars.
This graphic illustrates purposefully designing heterogeneous catalysts based on the relationships between reactions, catalysts, and deactivation mechanisms instead of adopting the conventional trial‐and‐error methodology for the hydrothermal valorization of biosugars. |
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| AbstractList | Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high‐performance catalysts. To assist the next‐stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent advances in biosugar hydrothermal valorization using heterogeneous catalysts, (2) the deactivation process of catalysts based on recycling tests of representative biosugar hydrothermal treatments, (3) state‐of‐the‐art understandings of the deactivation mechanisms of heterogeneous catalysts, and (4) strategies for preparing durable catalysts and the regeneration of deactivated catalysts. Based on the review, challenges and perspectives are proposed. Some remarkable achievements in heterogeneous catalysis of biosugars are highlighted. The understanding of catalyst durability needs to be further enhanced based on full examination of the catalytic performance based on the conversion of substrates, the yield, and selectivity of products. Further, a full examination of the physiochemical changes based on multiple characterization techniques is required to eclucidate the relationships between treatment variables and catalyst durability. Collectively, a clear understanding of the relationships between chemical reaction pathways, treatment variables, and the physiochemistry of catalysts is encouraged to be gained to advise the development of heterogeneous catalysts for long‐term and efficient hydrothermal upgrading of biosugars. Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high‐performance catalysts. To assist the next‐stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent advances in biosugar hydrothermal valorization using heterogeneous catalysts, (2) the deactivation process of catalysts based on recycling tests of representative biosugar hydrothermal treatments, (3) state‐of‐the‐art understandings of the deactivation mechanisms of heterogeneous catalysts, and (4) strategies for preparing durable catalysts and the regeneration of deactivated catalysts. Based on the review, challenges and perspectives are proposed. Some remarkable achievements in heterogeneous catalysis of biosugars are highlighted. The understanding of catalyst durability needs to be further enhanced based on full examination of the catalytic performance based on the conversion of substrates, the yield, and selectivity of products. Further, a full examination of the physiochemical changes based on multiple characterization techniques is required to eclucidate the relationships between treatment variables and catalyst durability. Collectively, a clear understanding of the relationships between chemical reaction pathways, treatment variables, and the physiochemistry of catalysts is encouraged to be gained to advise the development of heterogeneous catalysts for long‐term and efficient hydrothermal upgrading of biosugars. This graphic illustrates purposefully designing heterogeneous catalysts based on the relationships between reactions, catalysts, and deactivation mechanisms instead of adopting the conventional trial‐and‐error methodology for the hydrothermal valorization of biosugars. Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high-performance catalysts. To assist the next-stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent advances in biosugar hydrothermal valorization using heterogeneous catalysts, (2) the deactivation process of catalysts based on recycling tests of representative biosugar hydrothermal treatments, (3) state-of-the-art understandings of the deactivation mechanisms of heterogeneous catalysts, and (4) strategies for preparing durable catalysts and the regeneration of deactivated catalysts. Based on the review, challenges and perspectives are proposed. Some remarkable achievements in heterogeneous catalysis of biosugars are highlighted. The understanding of catalyst durability needs to be further enhanced based on full examination of the catalytic performance based on the conversion of substrates, the yield, and selectivity of products. Further, a full examination of the physiochemical changes based on multiple characterization techniques is required to eclucidate the relationships between treatment variables and catalyst durability. Collectively, a clear understanding of the relationships between chemical reaction pathways, treatment variables, and the physiochemistry of catalysts is encouraged to be gained to advise the development of heterogeneous catalysts for long-term and efficient hydrothermal upgrading of biosugars.Sustainable production of valuable biochemicals and biofuels from lignocellulosic biomass necessitates the development of durable and high-performance catalysts. To assist the next-stage catalyst design for hydrothermal treatment of biosugars, this paper provides a critical review of (1) recent advances in biosugar hydrothermal valorization using heterogeneous catalysts, (2) the deactivation process of catalysts based on recycling tests of representative biosugar hydrothermal treatments, (3) state-of-the-art understandings of the deactivation mechanisms of heterogeneous catalysts, and (4) strategies for preparing durable catalysts and the regeneration of deactivated catalysts. Based on the review, challenges and perspectives are proposed. Some remarkable achievements in heterogeneous catalysis of biosugars are highlighted. The understanding of catalyst durability needs to be further enhanced based on full examination of the catalytic performance based on the conversion of substrates, the yield, and selectivity of products. Further, a full examination of the physiochemical changes based on multiple characterization techniques is required to eclucidate the relationships between treatment variables and catalyst durability. Collectively, a clear understanding of the relationships between chemical reaction pathways, treatment variables, and the physiochemistry of catalysts is encouraged to be gained to advise the development of heterogeneous catalysts for long-term and efficient hydrothermal upgrading of biosugars. |
| Author | Lin, Richen Shen, Feng Xu, Siyu Liu, Juan Chun‐Ho Lam, Jason Jiang, Yujing Shuai, Li Zhu, Wenlei Song, Bing |
| Author_xml | – sequence: 1 givenname: Siyu orcidid: 0009-0003-1117-0558 surname: Xu fullname: Xu, Siyu organization: Nanjing University – sequence: 2 givenname: Yujing orcidid: 0000-0002-5420-7010 surname: Jiang fullname: Jiang, Yujing organization: Nanjing University – sequence: 3 givenname: Juan orcidid: 0000-0002-5221-2481 surname: Liu fullname: Liu, Juan organization: Nanjing University – sequence: 4 givenname: Jason orcidid: 0000-0003-3085-1634 surname: Chun‐Ho Lam fullname: Chun‐Ho Lam, Jason organization: Hong Kong Branch of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) – sequence: 5 givenname: Richen orcidid: 0000-0001-6861-8542 surname: Lin fullname: Lin, Richen organization: University College Cork – sequence: 6 givenname: Li orcidid: 0000-0002-7404-815X surname: Shuai fullname: Shuai, Li organization: Fujian Agriculture and Forestry University – sequence: 7 givenname: Feng orcidid: 0000-0002-6292-0094 surname: Shen fullname: Shen, Feng email: shenfeng@caas.cn organization: Ministry of Agriculture and Rural Affairs – sequence: 8 givenname: Wenlei orcidid: 0000-0001-6110-993X surname: Zhu fullname: Zhu, Wenlei email: wenleizhu@nju.edu.cn organization: Nanjing University – sequence: 9 givenname: Bing orcidid: 0000-0003-4791-083X surname: Song fullname: Song, Bing email: bing.song@scionresearch.com organization: University of New South Wales |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/39138129$$D View this record in MEDLINE/PubMed |
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| Keywords | Heterogeneous catalysis Hydrothermal treatment Catalyst deactivation Biomass valorization Biosugars |
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| SubjectTerms | Biofuels Biomass valorization Biosugars Catalyst deactivation Catalysts Catalytic converters Chemical reactions Deactivation Durability Heterogeneous catalysis Hydrothermal treatment Lignocellulose Physiochemistry |
| Title | Hydrothermal Valorization of Biosugars with Heterogeneous Catalysts: Advances, Catalyst Deactivation, Mitigation Strategies and Perspectives |
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