Defect dipole induced large recoverable strain and high energy-storage density in lead-free Na0.5Bi0.5TiO3-based systems
In this letter, we propose an effective route to obtain large recoverable strain, purely electrostrictive effects and high energy-storage density by inducing defect dipoles into Na0.5Bi0.5TiO3 (NBT)-based relaxor ferroelectrics. It has been found that pinched and double polarization hysteresis loops...
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| Published in | Applied physics letters Vol. 108; no. 20 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Melville
American Institute of Physics
16.05.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | In this letter, we propose an effective route to obtain large recoverable strain, purely electrostrictive effects and high energy-storage density by inducing defect dipoles into Na0.5Bi0.5TiO3 (NBT)-based relaxor ferroelectrics. It has been found that pinched and double polarization hysteresis loops with high maximum polarization (P
max) and negligible remanent polarization (P
r) can be observed due to the presence of acceptor-induced defect dipoles. A large recoverable strain of 0.24% with very little hysteresis and high electrostriction coefficient of 0.022 m4 C2 with purely electrostrictive characteristics were acquired when 11 mol. ‰ Mn-doped. Meanwhile, a high recoverable energy density of 1.06 J/cm3 with excellent temperature stability was obtained at the same composition owing to the enlarged value of P
max-P
r (36.8 μC/cm2) and relatively high electric field (95 kV/cm). Our achievement can open up the exciting opportunities for ferroelectric materials in high-precision positioning devices and high electric power pulse energy storage applications. |
|---|---|
| AbstractList | In this letter, we propose an effective route to obtain large recoverable strain, purely electrostrictive effects and high energy-storage density by inducing defect dipoles into Na0.5Bi0.5TiO3 (NBT)-based relaxor ferroelectrics. It has been found that pinched and double polarization hysteresis loops with high maximum polarization (Pmax) and negligible remanent polarization (Pr) can be observed due to the presence of acceptor-induced defect dipoles. A large recoverable strain of 0.24% with very little hysteresis and high electrostriction coefficient of 0.022 m4 C2 with purely electrostrictive characteristics were acquired when 11 mol. ‰ Mn-doped. Meanwhile, a high recoverable energy density of 1.06 J/cm3 with excellent temperature stability was obtained at the same composition owing to the enlarged value of Pmax-Pr (36.8 μC/cm2) and relatively high electric field (95 kV/cm). Our achievement can open up the exciting opportunities for ferroelectric materials in high-precision positioning devices and high electric power pulse energy storage applications. In this letter, we propose an effective route to obtain large recoverable strain, purely electrostrictive effects and high energy-storage density by inducing defect dipoles into Na0.5Bi0.5TiO3 (NBT)-based relaxor ferroelectrics. It has been found that pinched and double polarization hysteresis loops with high maximum polarization (P max) and negligible remanent polarization (P r) can be observed due to the presence of acceptor-induced defect dipoles. A large recoverable strain of 0.24% with very little hysteresis and high electrostriction coefficient of 0.022 m4 C2 with purely electrostrictive characteristics were acquired when 11 mol. ‰ Mn-doped. Meanwhile, a high recoverable energy density of 1.06 J/cm3 with excellent temperature stability was obtained at the same composition owing to the enlarged value of P max-P r (36.8 μC/cm2) and relatively high electric field (95 kV/cm). Our achievement can open up the exciting opportunities for ferroelectric materials in high-precision positioning devices and high electric power pulse energy storage applications. |
| Author | Qiao, Yulong Yu, Yang Li, Weili Feng, Yu Fei, Weidong Bai, Terigele Zhang, Tiandong Cao, Wenping Hou, Yafei |
| Author_xml | – sequence: 1 givenname: Wenping surname: Cao fullname: Cao, Wenping organization: Harbin Institute of Technology – sequence: 2 givenname: Weili surname: Li fullname: Li, Weili email: wlli@hit.edu.cn organization: 2National Key Laboratory of Science and Technology on Precision Heat Processing of Metals, Harbin Institute of Technology, Harbin 150001, People's Republic of China – sequence: 3 givenname: Yu surname: Feng fullname: Feng, Yu organization: Harbin Institute of Technology – sequence: 4 givenname: Terigele surname: Bai fullname: Bai, Terigele organization: Harbin Institute of Technology – sequence: 5 givenname: Yulong surname: Qiao fullname: Qiao, Yulong organization: Harbin Institute of Technology – sequence: 6 givenname: Yafei surname: Hou fullname: Hou, Yafei organization: Harbin Institute of Technology – sequence: 7 givenname: Tiandong surname: Zhang fullname: Zhang, Tiandong organization: Harbin Institute of Technology – sequence: 8 givenname: Yang surname: Yu fullname: Yu, Yang organization: Harbin Institute of Technology – sequence: 9 givenname: Weidong surname: Fei fullname: Fei, Weidong organization: Harbin Institute of Technology |
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| Snippet | In this letter, we propose an effective route to obtain large recoverable strain, purely electrostrictive effects and high energy-storage density by inducing... |
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| SubjectTerms | Applied physics Bismuth titanate Defects Dipoles Electrostriction Energy storage Ferroelectric materials Ferroelectricity Flux density Hysteresis loops Lead free Polarization Positioning devices (machinery) Recoverable strain Relaxors System effectiveness |
| Title | Defect dipole induced large recoverable strain and high energy-storage density in lead-free Na0.5Bi0.5TiO3-based systems |
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