Highly Efficient Pure-White-Light-Emitting Diodes from a Single Polymer: Polyfluorene with Naphthalimide Moieties
Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer: polyfluorene derivatives with 1,8‐naphthalimide chromophores chemically doped onto the polyfluorene backbones. By adjusting the emission wavelength of the 1,8‐n...
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Published in | Advanced functional materials Vol. 16; no. 1; pp. 101 - 106 |
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Main Authors | , , , , , , , , |
Format | Journal Article |
Language | English |
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Weinheim
WILEY-VCH Verlag
05.01.2006
WILEY‐VCH Verlag |
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Abstract | Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer: polyfluorene derivatives with 1,8‐naphthalimide chromophores chemically doped onto the polyfluorene backbones. By adjusting the emission wavelength of the 1,8‐naphthalimide components and optimizing the relative content of 1,8‐naphthalimide derivatives in the resulting polymers, white‐light electroluminescence from a single polymer, as opposed to a polymer blend, has been obtained in a device with a configuration of indium tin oxide/poly(3,4‐ethylenedioxythiophene)(50 nm)/polymer(80 nm)/Ca(10 nm)/Al(100 nm). The device exhibits Commission Internationale de l'Eclairage coordinates of (0.32,0.36), a maximum brightness of 11 900 cd m–2, a current efficiency of 3.8 cd A–1, a power efficiency of 2.0 lm W–1, an external quantum efficiency of 1.50 %, and quite stable color coordinates at different driving voltages, even at high luminances of over 5000 cd m–2.
A highly efficient pure‐white‐light‐emitting polymer diode, exhibiting Commission Internationale de l'Eclairage (CIE) coordinates of (0.32,0.36), a current efficiency of 3.8 cd A–1, a power efficiency of 2.0 lm W–1, and an external quantum efficiency of 1.50 %, has been developed. The diode is based on a single polymer, polyfluorene, containing 1,8‐naphthalimide derivatives with different emission wavelengths (see Figure). |
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AbstractList | Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer: polyfluorene derivatives with 1,8‐naphthalimide chromophores chemically doped onto the polyfluorene backbones. By adjusting the emission wavelength of the 1,8‐naphthalimide components and optimizing the relative content of 1,8‐naphthalimide derivatives in the resulting polymers, white‐light electroluminescence from a single polymer, as opposed to a polymer blend, has been obtained in a device with a configuration of indium tin oxide/poly(3,4‐ethylenedioxythiophene)(50 nm)/polymer(80 nm)/Ca(10 nm)/Al(100 nm). The device exhibits Commission Internationale de l'Eclairage coordinates of (0.32,0.36), a maximum brightness of 11 900 cd m–2, a current efficiency of 3.8 cd A–1, a power efficiency of 2.0 lm W–1, an external quantum efficiency of 1.50 %, and quite stable color coordinates at different driving voltages, even at high luminances of over 5000 cd m–2.
A highly efficient pure‐white‐light‐emitting polymer diode, exhibiting Commission Internationale de l'Eclairage (CIE) coordinates of (0.32,0.36), a current efficiency of 3.8 cd A–1, a power efficiency of 2.0 lm W–1, and an external quantum efficiency of 1.50 %, has been developed. The diode is based on a single polymer, polyfluorene, containing 1,8‐naphthalimide derivatives with different emission wavelengths (see Figure). Abstract Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer: polyfluorene derivatives with 1,8‐naphthalimide chromophores chemically doped onto the polyfluorene backbones. By adjusting the emission wavelength of the 1,8‐naphthalimide components and optimizing the relative content of 1,8‐naphthalimide derivatives in the resulting polymers, white‐light electroluminescence from a single polymer, as opposed to a polymer blend, has been obtained in a device with a configuration of indium tin oxide/poly(3,4‐ethylenedioxythiophene)(50 nm)/polymer(80 nm)/Ca(10 nm)/Al(100 nm). The device exhibits Commission Internationale de l'Eclairage coordinates of (0.32,0.36), a maximum brightness of 11 900 cd m –2 , a current efficiency of 3.8 cd A –1 , a power efficiency of 2.0 lm W –1 , an external quantum efficiency of 1.50 %, and quite stable color coordinates at different driving voltages, even at high luminances of over 5000 cd m –2 . |
Author | Wang, L. X. Mei, C. Y. Geng, Y. H. Wang, F. S. Zhou, Q. G. Cheng, Y. X. Jing, X. B. Ma, D. G. Tu, G. L. |
Author_xml | – sequence: 1 givenname: G. L. surname: Tu fullname: Tu, G. L. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 2 givenname: C. Y. surname: Mei fullname: Mei, C. Y. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 3 givenname: Q. G. surname: Zhou fullname: Zhou, Q. G. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 4 givenname: Y. X. surname: Cheng fullname: Cheng, Y. X. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 5 givenname: Y. H. surname: Geng fullname: Geng, Y. H. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 6 givenname: L. X. surname: Wang fullname: Wang, L. X. email: lixiang@ciac.jl.cn organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 7 givenname: D. G. surname: Ma fullname: Ma, D. G. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 8 givenname: X. B. surname: Jing fullname: Jing, X. B. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China – sequence: 9 givenname: F. S. surname: Wang fullname: Wang, F. S. organization: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P.R. China |
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Copyright | Copyright © 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim |
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Notes | istex:CBA18416BBB16FE473C9CC1DDF7E193FC1E8D161 ark:/67375/WNG-1WV8MMX1-6 ArticleID:ADFM200500028 We acknowledge financial support from the National Natural Science Foundation of China (No. 20574067) and 973 Project (2002CB613402). |
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Snippet | Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer: polyfluorene... Abstract Light‐emitting diodes exhibiting efficient pure‐white‐light electroluminescence have been successfully developed by using a single polymer:... |
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SubjectTerms | Light-emitting diodes Light‐emitting diodes, organic organic Polyfluorenes White-light emitters |
Title | Highly Efficient Pure-White-Light-Emitting Diodes from a Single Polymer: Polyfluorene with Naphthalimide Moieties |
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