Inverted Organic Solar Cells with Sol-Gel Processed High Work-Function Vanadium Oxide Hole-Extraction Layers
For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate inverted bulk‐heterojunction organic solar cells (OSCs) with a sol–gel derived V2O5 hole‐extraction‐layer on top of the active organic layer. The V2O5 l...
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Published in | Advanced functional materials Vol. 21; no. 24; pp. 4776 - 4783 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
Published |
Weinheim
WILEY-VCH Verlag
20.12.2011
WILEY‐VCH Verlag |
Subjects | |
Online Access | Get full text |
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Abstract | For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate inverted bulk‐heterojunction organic solar cells (OSCs) with a sol–gel derived V2O5 hole‐extraction‐layer on top of the active organic layer. The V2O5 layers are prepared in ambient air using Vanadium(V)‐oxitriisopropoxide as precursor. Without any post‐annealing or plasma treatment, a high work function of the V2O5 layers is confirmed by both Kelvin probe analysis and ultraviolet photoelectron spectroscopy (UPS). Using UPS and inverse photoelectron spectroscopy (IPES), we show that the electronic structure of the solution processed V2O5 layers is similar to that of thermally evaporated V2O5 layers which have been exposed to ambient air. Optimization of the sol gel process leads to inverted OSCs with solution based V2O5 layers that show power conversion efficiencies similar to that of control devices with V2O5 layers prepared in high‐vacuum.
Inverted organic solar cells employing a solution processed V2O5 (sV2O5) hole‐extraction‐layer on top of the active organic layer are demonstrated. Even without any post‐deposition treatment, the electronic structure of the sV2O5 layers is similar to that of thermally evaporated V2O5 (eV2O5) layers which have been exposed to ambient air. Optimized devices with sV2O5 layers show power conversion efficiencies similar to that of devices with eV2O5 layers. |
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AbstractList | Abstract
For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate inverted bulk‐heterojunction organic solar cells (OSCs) with a sol–gel derived V
2
O
5
hole‐extraction‐layer on top of the active organic layer. The V
2
O
5
layers are prepared in ambient air using Vanadium(V)‐oxitriisopropoxide as precursor. Without any post‐annealing or plasma treatment, a high work function of the V
2
O
5
layers is confirmed by both Kelvin probe analysis and ultraviolet photoelectron spectroscopy (UPS). Using UPS and inverse photoelectron spectroscopy (IPES), we show that the electronic structure of the solution processed V
2
O
5
layers is similar to that of thermally evaporated V
2
O
5
layers which have been exposed to ambient air. Optimization of the sol gel process leads to inverted OSCs with solution based V
2
O
5
layers that show power conversion efficiencies similar to that of control devices with V
2
O
5
layers prepared in high‐vacuum. For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate inverted bulk‐heterojunction organic solar cells (OSCs) with a sol–gel derived V2O5 hole‐extraction‐layer on top of the active organic layer. The V2O5 layers are prepared in ambient air using Vanadium(V)‐oxitriisopropoxide as precursor. Without any post‐annealing or plasma treatment, a high work function of the V2O5 layers is confirmed by both Kelvin probe analysis and ultraviolet photoelectron spectroscopy (UPS). Using UPS and inverse photoelectron spectroscopy (IPES), we show that the electronic structure of the solution processed V2O5 layers is similar to that of thermally evaporated V2O5 layers which have been exposed to ambient air. Optimization of the sol gel process leads to inverted OSCs with solution based V2O5 layers that show power conversion efficiencies similar to that of control devices with V2O5 layers prepared in high‐vacuum. Inverted organic solar cells employing a solution processed V2O5 (sV2O5) hole‐extraction‐layer on top of the active organic layer are demonstrated. Even without any post‐deposition treatment, the electronic structure of the sV2O5 layers is similar to that of thermally evaporated V2O5 (eV2O5) layers which have been exposed to ambient air. Optimized devices with sV2O5 layers show power conversion efficiencies similar to that of devices with eV2O5 layers. |
Author | Zilberberg, Kirill Riedl, Thomas Meyer, Jens Trost, Sara Behrendt, Andreas Kahn, Antoine Lützenkirchen-Hecht, Dirk Frahm, Ronald |
Author_xml | – sequence: 1 givenname: Kirill surname: Zilberberg fullname: Zilberberg, Kirill organization: Institute of Electronic Devices, University of Wuppertal, Rainer-Gruenter-Str. 21, 42119 Wuppertal, Germany – sequence: 2 givenname: Sara surname: Trost fullname: Trost, Sara organization: Institute of Electronic Devices, University of Wuppertal, Rainer-Gruenter-Str. 21, 42119 Wuppertal, Germany – sequence: 3 givenname: Jens surname: Meyer fullname: Meyer, Jens organization: Department of Electrical Engineering, Princeton University, Princeton, NJ, USA – sequence: 4 givenname: Antoine surname: Kahn fullname: Kahn, Antoine organization: Department of Electrical Engineering, Princeton University, Princeton, NJ, USA – sequence: 5 givenname: Andreas surname: Behrendt fullname: Behrendt, Andreas organization: Physics of Condensed Matter, University of Wuppertal, Germany – sequence: 6 givenname: Dirk surname: Lützenkirchen-Hecht fullname: Lützenkirchen-Hecht, Dirk organization: Physics of Condensed Matter, University of Wuppertal, Germany – sequence: 7 givenname: Ronald surname: Frahm fullname: Frahm, Ronald organization: Physics of Condensed Matter, University of Wuppertal, Germany – sequence: 8 givenname: Thomas surname: Riedl fullname: Riedl, Thomas email: t.riedl@uni-wuppertal.de organization: Institute of Electronic Devices, University of Wuppertal, Rainer-Gruenter-Str. 21, 42119 Wuppertal, Germany |
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Snippet | For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate inverted... Abstract For large‐scale and high‐throughput production of organic solar cells (OSCs), liquid processing of the functional layers is desired. We demonstrate... |
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SubjectTerms | high work-function materials inverted organic solar cells solution processed metal oxide vanadium oxide |
Title | Inverted Organic Solar Cells with Sol-Gel Processed High Work-Function Vanadium Oxide Hole-Extraction Layers |
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