Low-loss contacts on textured substrates for inverted perovskite solar cells

Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts 1 – 3 . To improve efficiency further, it is crucial to combine effective light management with low interfacial losses 4 , 5 . Here we develop a conformal self-assembled monola...

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Published inNature (London) Vol. 624; no. 7991; pp. 289 - 294
Main Authors Park, So Min, Wei, Mingyang, Lempesis, Nikolaos, Yu, Wenjin, Hossain, Tareq, Agosta, Lorenzo, Carnevali, Virginia, Atapattu, Harindi R., Serles, Peter, Eickemeyer, Felix T., Shin, Heejong, Vafaie, Maral, Choi, Deokjae, Darabi, Kasra, Jung, Eui Dae, Yang, Yi, Kim, Da Bin, Zakeeruddin, Shaik M., Chen, Bin, Amassian, Aram, Filleter, Tobin, Kanatzidis, Mercouri G., Graham, Kenneth R., Xiao, Lixin, Rothlisberger, Ursula, Grätzel, Michael, Sargent, Edward H.
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 14.12.2023
Nature Publishing Group
Subjects
119/118
140/125
140/146
639/301/299/946
639/4077/909/4101/4096/946
Acids
Adsorbents
Adsorption
Chemical bonds
Efficiency
Energy conversion efficiency
Humanities and Social Sciences
Maximum power tracking
Molecular dynamics
multidisciplinary
Optoelectronic devices
Perovskites
Phosphonic acids
Photoelectric effect
Photovoltaic cells
Relative humidity
Room temperature
Science
Science (multidisciplinary)
Self-assembled monolayers
Self-assembly
Simulation
Solar cells
Spectrum analysis
Substrates
Online AccessGet full text

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Abstract Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts 1 – 3 . To improve efficiency further, it is crucial to combine effective light management with low interfacial losses 4 , 5 . Here we develop a conformal self-assembled monolayer (SAM) as the hole-selective contact on light-managing textured substrates. Molecular dynamics simulations indicate that cluster formation during phosphonic acid adsorption leads to incomplete SAM coverage. We devise a co-adsorbent strategy that disassembles high-order clusters, thus homogenizing the distribution of phosphonic acid molecules, and thereby minimizing interfacial recombination and improving electronic structures. We report a laboratory-measured power conversion efficiency (PCE) of 25.3% and a certified quasi-steady-state PCE of 24.8% for inverted PSCs, with a photocurrent approaching 95% of the Shockley–Queisser maximum. An encapsulated device having a PCE of 24.6% at room temperature retains 95% of its peak performance when stressed at 65 °C and 50% relative humidity following more than 1,000 h of maximum power point tracking under 1 sun illumination. This represents one of the most stable PSCs subjected to accelerated ageing: achieved with a PCE surpassing 24%. The engineering of phosphonic acid adsorption on textured substrates offers a promising avenue for efficient and stable PSCs. It is also anticipated to benefit other optoelectronic devices that require light management. A co-adsorbent is used to achieve a uniform self-assembled phosphonic acid monolayer on a textured substrate, leading to more efficient inverted perovskite solar cells.
AbstractList Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts 1 – 3 . To improve efficiency further, it is crucial to combine effective light management with low interfacial losses 4 , 5 . Here we develop a conformal self-assembled monolayer (SAM) as the hole-selective contact on light-managing textured substrates. Molecular dynamics simulations indicate that cluster formation during phosphonic acid adsorption leads to incomplete SAM coverage. We devise a co-adsorbent strategy that disassembles high-order clusters, thus homogenizing the distribution of phosphonic acid molecules, and thereby minimizing interfacial recombination and improving electronic structures. We report a laboratory-measured power conversion efficiency (PCE) of 25.3% and a certified quasi-steady-state PCE of 24.8% for inverted PSCs, with a photocurrent approaching 95% of the Shockley–Queisser maximum. An encapsulated device having a PCE of 24.6% at room temperature retains 95% of its peak performance when stressed at 65 °C and 50% relative humidity following more than 1,000 h of maximum power point tracking under 1 sun illumination. This represents one of the most stable PSCs subjected to accelerated ageing: achieved with a PCE surpassing 24%. The engineering of phosphonic acid adsorption on textured substrates offers a promising avenue for efficient and stable PSCs. It is also anticipated to benefit other optoelectronic devices that require light management. A co-adsorbent is used to achieve a uniform self-assembled phosphonic acid monolayer on a textured substrate, leading to more efficient inverted perovskite solar cells.
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts1-3. To improve efficiency further, it is crucial to combine effective light management with low interfacial losses4,5. Here we develop a conformal self-assembled monolayer (SAM) as the hole-selective contact on light-managing textured substrates. Molecular dynamics simulations indicate that cluster formation during phosphonic acid adsorption leads to incomplete SAM coverage. We devise a co-adsorbent strategy that disassembles high-order clusters, thus homogenizing the distribution of phosphonic acid molecules, and thereby minimizing interfacial recombination and improving electronic structures. We report a laboratory-measured power conversion efficiency (PCE) of 25.3% and a certified quasi-steady-state PCE of 24.8% for inverted PSCs, with a photocurrent approaching 95% of the Shockley-Queisser maximum. An encapsulated device having a PCE of 24.6% at room temperature retains 95% of its peak performance when stressed at 65 °C and 50% relative humidity following more than 1,000 h of maximum power point tracking under 1 sun illumination. This represents one of the most stable PSCs subjected to accelerated ageing: achieved with a PCE surpassing 24%. The engineering of phosphonic acid adsorption on textured substrates offers a promising avenue for efficient and stable PSCs. It is also anticipated to benefit other optoelectronic devices that require light management.
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts13. To improve efficiency further, it is crucial to combine effective light management with low interfacial losses4 5. Here we develop a conformal self-assembled monolayer (SAM) as the hole-selective contact on lightmanaging textured substrates. Molecular dynamics simulations indicate that cluster formation during phosphonic acid adsorption leadsto incomplete SAM coverage. We devise a co-adsorbent strategy that disassembles high-order clusters, thus homogenizing the distribution of phosphonic acid molecules, and thereby minimizing interfacial recombination and improving electronic structures. We report a laboratorymeasured power conversion efficiency (PCE) of 25.3% and a certified quasi-steady-state PCE of 24.8% for inverted PSCs, with a photocurrent approaching 95% ofthe ShockleyQueisser maximum. An encapsulated device having a PCE of 24.6% at room temperature retains 95% of its peak performance when stressed at 65 °C and 50% relative humidity following more than 1,000 h of maximum power point tracking underl sun illumination. This represents one ofthe most stable PSCs subjected to accelerated ageing: achieved with a PCE surpassing 24%. The engineering of phosphonic acid adsorption on textured substrates offers a promising avenue for efficient and stable PSCs. It is also anticipated to benefit other optoelectronic devices that require light management.
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts . To improve efficiency further, it is crucial to combine effective light management with low interfacial losses . Here we develop a conformal self-assembled monolayer (SAM) as the hole-selective contact on light-managing textured substrates. Molecular dynamics simulations indicate that cluster formation during phosphonic acid adsorption leads to incomplete SAM coverage. We devise a co-adsorbent strategy that disassembles high-order clusters, thus homogenizing the distribution of phosphonic acid molecules, and thereby minimizing interfacial recombination and improving electronic structures. We report a laboratory-measured power conversion efficiency (PCE) of 25.3% and a certified quasi-steady-state PCE of 24.8% for inverted PSCs, with a photocurrent approaching 95% of the Shockley-Queisser maximum. An encapsulated device having a PCE of 24.6% at room temperature retains 95% of its peak performance when stressed at 65 °C and 50% relative humidity following more than 1,000 h of maximum power point tracking under 1 sun illumination. This represents one of the most stable PSCs subjected to accelerated ageing: achieved with a PCE surpassing 24%. The engineering of phosphonic acid adsorption on textured substrates offers a promising avenue for efficient and stable PSCs. It is also anticipated to benefit other optoelectronic devices that require light management.
Author Agosta, Lorenzo
Kanatzidis, Mercouri G.
Grätzel, Michael
Choi, Deokjae
Carnevali, Virginia
Filleter, Tobin
Park, So Min
Serles, Peter
Vafaie, Maral
Xiao, Lixin
Darabi, Kasra
Eickemeyer, Felix T.
Sargent, Edward H.
Graham, Kenneth R.
Shin, Heejong
Amassian, Aram
Lempesis, Nikolaos
Jung, Eui Dae
Hossain, Tareq
Atapattu, Harindi R.
Kim, Da Bin
Chen, Bin
Rothlisberger, Ursula
Zakeeruddin, Shaik M.
Wei, Mingyang
Yu, Wenjin
Yang, Yi
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/37871614$$D View this record in MEDLINE/PubMed
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Snippet Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts 1 – 3 . To improve efficiency...
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts . To improve efficiency further, it...
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts13. To improve efficiency further,...
Inverted perovskite solar cells (PSCs) promise enhanced operating stability compared to their normal-structure counterparts1-3. To improve efficiency further,...
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SubjectTerms 119/118
140/125
140/146
639/301/299/946
639/4077/909/4101/4096/946
Acids
Adsorbents
Adsorption
Chemical bonds
Efficiency
Energy conversion efficiency
Humanities and Social Sciences
Maximum power tracking
Molecular dynamics
multidisciplinary
Optoelectronic devices
Perovskites
Phosphonic acids
Photoelectric effect
Photovoltaic cells
Relative humidity
Room temperature
Science
Science (multidisciplinary)
Self-assembled monolayers
Self-assembly
Simulation
Solar cells
Spectrum analysis
Substrates
Title Low-loss contacts on textured substrates for inverted perovskite solar cells
URI https://link.springer.com/article/10.1038/s41586-023-06745-7
https://www.ncbi.nlm.nih.gov/pubmed/37871614
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