Sensing temperature with Tb-Eu-based luminescent thermometer: A novel approach to increase the sensitivity
To obtain ratiometric temperature sensor with high sensitivity we have synthesized three rows of bimetallic Tb-Eu hydroxybenzoates, whose sensitivity was expected to exceed the theoretical limit due to the presence of the temperature-dependent OH-quenching. Single crystals of two new bimetallic comp...
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| Published in | Sensors and actuators. A. Physical. Vol. 345; p. 113787 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Lausanne
Elsevier B.V
01.10.2022
Elsevier BV |
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| Online Access | Get full text |
| ISSN | 0924-4247 1873-3069 |
| DOI | 10.1016/j.sna.2022.113787 |
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| Abstract | To obtain ratiometric temperature sensor with high sensitivity we have synthesized three rows of bimetallic Tb-Eu hydroxybenzoates, whose sensitivity was expected to exceed the theoretical limit due to the presence of the temperature-dependent OH-quenching. Single crystals of two new bimetallic complexes were obtained, and their crystal structures were determined. Despite europium complexes with the selected ligands do not emit light, bimetallic Tb-Eu complexes with 3- and 4-hydroxybenzoates demonstrate europium luminescence with the quantum yield up to 77 %. Selected 3- and 4-hydroxybenzoates demonstrated temperature-dependent luminescence in the range of 25–100 °C. For 3-hydroxybenzoate of Tb-Eu, thermometer sensitivity reached 4 %/°C at 100 °C, which exceeds the expected limit of 3.3 %/°C at this temperature and is the highest reported value at this temperature. Temperature resolution is about 3 °C.
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•Bimetallic Tb-Eu hydroxybenzoate formation increases europium luminescence efficiency from 0 % to up to 77 %.•Tb-Eu 3- and 4-hydroxybenzoates demonstrate temperature-dependent luminescence in the range of 25–100 °C.•The sensitivity reached 4 %/°C at 100 °C, which exceeds the theoretical limit.•Temperature resolution is about 3 °C. |
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| AbstractList | To obtain ratiometric temperature sensor with high sensitivity we have synthesized three rows of bimetallic Tb-Eu hydroxybenzoates, whose sensitivity was expected to exceed the theoretical limit due to the presence of the temperature-dependent OH-quenching. Single crystals of two new bimetallic complexes were obtained, and their crystal structures were determined. Despite europium complexes with the selected ligands do not emit light, bimetallic Tb-Eu complexes with 3- and 4-hydroxybenzoates demonstrate europium luminescence with the quantum yield up to 77 %. Selected 3- and 4-hydroxybenzoates demonstrated temperature-dependent luminescence in the range of 25–100 °C. For 3-hydroxybenzoate of Tb-Eu, thermometer sensitivity reached 4 %/°C at 100 °C, which exceeds the expected limit of 3.3 %/°C at this temperature and is the highest reported value at this temperature. Temperature resolution is about 3 °C.
[Display omitted]
•Bimetallic Tb-Eu hydroxybenzoate formation increases europium luminescence efficiency from 0 % to up to 77 %.•Tb-Eu 3- and 4-hydroxybenzoates demonstrate temperature-dependent luminescence in the range of 25–100 °C.•The sensitivity reached 4 %/°C at 100 °C, which exceeds the theoretical limit.•Temperature resolution is about 3 °C. To obtain ratiometric temperature sensor with high sensitivity we have synthesized three rows of bimetallic Tb-Eu hydroxybenzoates, whose sensitivity was expected to exceed the theoretical limit due to the presence of the temperature-dependent OH-quenching. Single crystals of two new bimetallic complexes were obtained, and their crystal structures were determined. Despite europium complexes with the selected ligands do not emit light, bimetallic Tb-Eu complexes with 3- and 4-hydroxybenzoates demonstrate europium luminescence with the quantum yield up to 77 %. Selected 3- and 4-hydroxybenzoates demonstrated temperature-dependent luminescence in the range of 25–100 °C. For 3-hydroxybenzoate of Tb-Eu, thermometer sensitivity reached 4 %/°C at 100 °C, which exceeds the expected limit of 3.3 %/°C at this temperature and is the highest reported value at this temperature. Temperature resolution is about 3 °C. |
| ArticleNumber | 113787 |
| Author | Goloveshkin, Alexander S. Gordeeva, Elena O. Yu. Kozhevnikova, Vladislava Utochnikova, Valentina V. Tcelykh, Liubov O. Latipov, Egor V. |
| Author_xml | – sequence: 1 givenname: Liubov O. surname: Tcelykh fullname: Tcelykh, Liubov O. email: lyuba.tselih@mail.ru organization: Department of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1, build.3, 119991 Moscow, Russian Federation – sequence: 2 givenname: Vladislava surname: Yu. Kozhevnikova fullname: Yu. Kozhevnikova, Vladislava organization: Department of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1, build.3, 119991 Moscow, Russian Federation – sequence: 3 givenname: Alexander S. surname: Goloveshkin fullname: Goloveshkin, Alexander S. organization: A.N. Nesmeyanov Institute of Organoelement Compounds, Vavilova St. 28, Moscow 119334, Russian Federation – sequence: 4 givenname: Egor V. surname: Latipov fullname: Latipov, Egor V. organization: Institute of Nanotechnology of Microelectronics of the Russian Academy of Sciences, Leninskiy Prospekt, 32 A, 119334 Moscow, Russian Federation – sequence: 5 givenname: Elena O. surname: Gordeeva fullname: Gordeeva, Elena O. organization: Department of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1, build.3, 119991 Moscow, Russian Federation – sequence: 6 givenname: Valentina V. surname: Utochnikova fullname: Utochnikova, Valentina V. email: valentina.utochnikova@gmail.com, valentina@inorg.chem.msu.ru organization: Department of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1, build.3, 119991 Moscow, Russian Federation |
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| Snippet | To obtain ratiometric temperature sensor with high sensitivity we have synthesized three rows of bimetallic Tb-Eu hydroxybenzoates, whose sensitivity was... |
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| SubjectTerms | Bimetals Chemical synthesis Crystal structure Europium Luminescence Luminescence thermometryelevated temperature hydroxobenzoates bimetallic complexeslanthanides Sensitivity Sensors Single crystals Temperature Temperature dependence Temperature sensors Thermometers Thermometry |
| Title | Sensing temperature with Tb-Eu-based luminescent thermometer: A novel approach to increase the sensitivity |
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