Numerical Simulation of Influence of Hydrogen Peroxide Photolysis on Water Chemistry in BWR Plant
As a novel technique to enhance the effect of H 2 addition for HWC (hydrogen water chemistry) in BWR coolant, UV light photolysis of H 2 O 2 was proposed. The effect of the H 2 O 2 photolysis on water radiolysis was simulated for a batch system at 288°C. It was demonstrated that this technique reduc...
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Published in | Journal of nuclear science and technology Vol. 38; no. 8; pp. 637 - 644 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
Published |
Tokyo
Taylor & Francis Group
01.08.2001
Atomic Energy Society of Japan |
Subjects | |
Online Access | Get full text |
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Abstract | As a novel technique to enhance the effect of H
2
addition for HWC (hydrogen water chemistry) in BWR coolant, UV light photolysis of H
2
O
2
was proposed. The effect of the H
2
O
2
photolysis on water radiolysis was simulated for a batch system at 288°C. It was demonstrated that this technique reduced the concentrations of H
2
O
2
and O
2
with less amount of H
2
than that under ordinary HWC condition. It was found that the technique can reduce the H
2
O
2
concentration even in the absence of H
2
addition although the OH concentration increases concomitantly. The radiation chemical mechanism under ordinary HWC condition is discussed briefly. The UV laser power required to reduce concentrations of the oxidizing species was estimated for a dose rate of †-ray 100Gy-s
-1
based on the simulated results. A potential role of the Cherenkov radiation in H
2
O
2
decomposition in coolant of a BWR plant was pointed out. |
---|---|
AbstractList | As a novel technique to enhance the effect of H
2
addition for HWC (hydrogen water chemistry) in BWR coolant, UV light photolysis of H
2
O
2
was proposed. The effect of the H
2
O
2
photolysis on water radiolysis was simulated for a batch system at 288°C. It was demonstrated that this technique reduced the concentrations of H
2
O
2
and O
2
with less amount of H
2
than that under ordinary HWC condition. It was found that the technique can reduce the H
2
O
2
concentration even in the absence of H
2
addition although the OH concentration increases concomitantly. The radiation chemical mechanism under ordinary HWC condition is discussed briefly. The UV laser power required to reduce concentrations of the oxidizing species was estimated for a dose rate of †-ray 100Gy-s
-1
based on the simulated results. A potential role of the Cherenkov radiation in H
2
O
2
decomposition in coolant of a BWR plant was pointed out. |
Author | HISHIDA, Mamoru ONO, Shoichi DOMAE, Masafumi |
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Keywords | Water chemistry Boiling water reactor Hydrogen peroxide Coolant Photolysis Laser Radiolysis Numerical simulation Corrosion protection Dose rate Nuclear reactor |
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References | Katsumura Y. (CIT0038) 1985; 24 Buxton B. V. (CIT0030) 1987 Ruiz C. P. (CIT0008) 1989; 5 Burns W. G. (CIT0007) 1976; 30 Takagi J. (CIT0036) 1984; 1 Uchida S. (CIT0037) 1995; 110 Christensen H. (CIT0010) 1995; 109 Bjergbakke E. (CIT0011) 1989; 48 Elliot A. J. (CIT0033) 1996; 100 Takagi J. (CIT0024) 1985; 87 Klaning U. K. (CIT0025) 1985; 89 Sunaryo G. R. (CIT0035) 1995; 45 Stefan M. I. (CIT0017) 1996; 30 Elliot A. J. (CIT0031) 1993; 89 Buxton G. V. (CIT0022) 1993; 89 Uchida S. (CIT0003) 1995; 110 CIT0014 Bjergbakke E. (CIT0012) 1989; 48 CIT0016 Christensen H. (CIT0023) 1983; 87 Schwarz H. A. (CIT0028) 1981; 58 Shiraishi H. (CIT0032) 1988; 92 Sunaryo G. R. (CIT0013) 1995; 45 Yeh T. K. (CIT0006) 2000; 8 Sunaryo G. R. (CIT0034) 1994; 44 (CIT0019) 1995 CIT0020 CIT0001 Cowan R. L. (CIT0002) 1996; 7 Curtis A. R. (CIT0018) 1987 Mcdonald D. D. (CIT0005) 1998 Hiroishi D. (CIT0029) 1989 Shiraishi H. (CIT0021) 1994; 98 Yeh T. K. (CIT0009) 1995; 121 CIT0004 Ichikawa N. (CIT0015) 1998 CIT0026 Han P. (CIT0027) 1990; 94 |
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Snippet | As a novel technique to enhance the effect of H
2
addition for HWC (hydrogen water chemistry) in BWR coolant, UV light photolysis of H
2
O
2
was proposed. The... |
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StartPage | 637 |
SubjectTerms | Applied sciences Boiling water reator coolant decomposition Energy Energy. Thermal use of fuels Exact sciences and technology Fission nuclear power plants hydrogen peroxide hydrogen water chemistry hydrogen addition Installations for energy generation and conversion: thermal and electrical energy photolysis simulation |
Title | Numerical Simulation of Influence of Hydrogen Peroxide Photolysis on Water Chemistry in BWR Plant |
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