Rational design of the self-assembled BaCo1-xZrxO3-δ (x = 0.8–0.2) nanocomposites as the promising low/intermediate-temperature solid oxide fuel cell cathodes
Assembling multiple perovskites with complementary properties is a promising strategy to achieve high-performance cathodes for low/intermediate-temperature solid oxide fuel cell (LT/IT-SOFC). In this work, self-assembling perovskites of cubic BaZr0.82Co0.18O3-δ (cub-BZC) and hexagonal BaCo0.96Zr0.04...
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| Published in | Journal of the European Ceramic Society Vol. 42; no. 3; pp. 1042 - 1052 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.03.2022
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| Abstract | Assembling multiple perovskites with complementary properties is a promising strategy to achieve high-performance cathodes for low/intermediate-temperature solid oxide fuel cell (LT/IT-SOFC). In this work, self-assembling perovskites of cubic BaZr0.82Co0.18O3-δ (cub-BZC) and hexagonal BaCo0.96Zr0.04O2.6+δ (12H-BC) at the nanoscale can be realized in novel designed nanocomposites with nominal composition of BaCo1-xZrxO3-δ (x = 0.8–0.2), which can possess congenital compatibility, improved thermal expansion coefficients and electrical conductivity. The relative contents of cubic and hexagonal phases are significantly correlated with the zirconium content (x). Therein, BaCo1-xZrxO3-δ nanocomposites exhibit relatively low content differences among perovskite phases when x = 0.4 (cubic/hexagonal = 62:38) and x = 0.2 (hexagonal/cubic = 69:31) nanocomposites, which can form more extensive heterointerfaces for promoting oxygen adsorption, dissociation and reduction reaction. When further applied as cathode, the cell with BaCo1-xZrxO3-δ nanocomposites achieve 2265–598 mW cm−2 (800–600 °C) when x = 0.2 as a promising IT-SOFC cathode, and 315−148 mW cm−2 (550–500 °C) when x = 0.4 as a promising LT-SOFC cathode. |
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| AbstractList | Assembling multiple perovskites with complementary properties is a promising strategy to achieve high-performance cathodes for low/intermediate-temperature solid oxide fuel cell (LT/IT-SOFC). In this work, self-assembling perovskites of cubic BaZr0.82Co0.18O3-δ (cub-BZC) and hexagonal BaCo0.96Zr0.04O2.6+δ (12H-BC) at the nanoscale can be realized in novel designed nanocomposites with nominal composition of BaCo1-xZrxO3-δ (x = 0.8–0.2), which can possess congenital compatibility, improved thermal expansion coefficients and electrical conductivity. The relative contents of cubic and hexagonal phases are significantly correlated with the zirconium content (x). Therein, BaCo1-xZrxO3-δ nanocomposites exhibit relatively low content differences among perovskite phases when x = 0.4 (cubic/hexagonal = 62:38) and x = 0.2 (hexagonal/cubic = 69:31) nanocomposites, which can form more extensive heterointerfaces for promoting oxygen adsorption, dissociation and reduction reaction. When further applied as cathode, the cell with BaCo1-xZrxO3-δ nanocomposites achieve 2265–598 mW cm−2 (800–600 °C) when x = 0.2 as a promising IT-SOFC cathode, and 315−148 mW cm−2 (550–500 °C) when x = 0.4 as a promising LT-SOFC cathode. |
| Author | Cheng, Mojie Tu, Baofeng Liu, Di Qi, Huiying Zhang, Tonghuan |
| Author_xml | – sequence: 1 givenname: Huiying orcidid: 0000-0001-8643-4907 surname: Qi fullname: Qi, Huiying organization: Shandong University of Science and Technology, 579 Qianwangang Road, 266590, Qingdao, China – sequence: 2 givenname: Tonghuan surname: Zhang fullname: Zhang, Tonghuan organization: Shandong University of Science and Technology, 579 Qianwangang Road, 266590, Qingdao, China – sequence: 3 givenname: Mojie surname: Cheng fullname: Cheng, Mojie organization: Dalian Institute of Chemical Physics, 457 Zhongshan Road, 116023, Dalian, China – sequence: 4 givenname: Di surname: Liu fullname: Liu, Di organization: Shandong University of Science and Technology, 579 Qianwangang Road, 266590, Qingdao, China – sequence: 5 givenname: Baofeng surname: Tu fullname: Tu, Baofeng email: tubaofeng2019@163.com organization: Shandong University of Science and Technology, 579 Qianwangang Road, 266590, Qingdao, China |
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| Keywords | Solid oxide fuel cells Perovskites Nanocomposites Oxygen reduction reaction Heterointerface |
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| SubjectTerms | Heterointerface Nanocomposites Oxygen reduction reaction Perovskites Solid oxide fuel cells |
| Title | Rational design of the self-assembled BaCo1-xZrxO3-δ (x = 0.8–0.2) nanocomposites as the promising low/intermediate-temperature solid oxide fuel cell cathodes |
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