Tuning the mechanical and thermal properties of (MgNiCoCuZn)O by intelligent control of cooling rates
The possibility of altering the phase equilibria of multicomponent oxide systems through precise control of configurational entropy has opened a platform with unlimited possibilities to fine-tune material properties. The current work is aimed at tailoring the mechanical and thermal properties of (Mg...
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Published in | Journal of the European Ceramic Society Vol. 43; no. 10; pp. 4517 - 4529 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
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Elsevier Ltd
01.08.2023
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Abstract | The possibility of altering the phase equilibria of multicomponent oxide systems through precise control of configurational entropy has opened a platform with unlimited possibilities to fine-tune material properties. The current work is aimed at tailoring the mechanical and thermal properties of (MgNiCoCuZn)O by an intelligent design of constituent phase structure resulting from controlled cooling from the stabilization temperature. Based on the cooling rates, the amount of CuO nucleation was found to vary between 5.4 and 12.3 wt%, along with a corresponding decrease in Cu2+ content in the matrix. It was observed that with the decrease in Cu2+ ion concentration in the matrix, the Young’s modulus and hardness increased by 33% and 26%, respectively, along with a corresponding decrease in the coefficient of thermal expansion by 15%. Similarly, an increased nucleation of CuO precipitates led to the improvement of fracture toughness of the material by 15%, while its thermal conductivity remained unaltered.
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AbstractList | The possibility of altering the phase equilibria of multicomponent oxide systems through precise control of configurational entropy has opened a platform with unlimited possibilities to fine-tune material properties. The current work is aimed at tailoring the mechanical and thermal properties of (MgNiCoCuZn)O by an intelligent design of constituent phase structure resulting from controlled cooling from the stabilization temperature. Based on the cooling rates, the amount of CuO nucleation was found to vary between 5.4 and 12.3 wt%, along with a corresponding decrease in Cu2+ content in the matrix. It was observed that with the decrease in Cu2+ ion concentration in the matrix, the Young’s modulus and hardness increased by 33% and 26%, respectively, along with a corresponding decrease in the coefficient of thermal expansion by 15%. Similarly, an increased nucleation of CuO precipitates led to the improvement of fracture toughness of the material by 15%, while its thermal conductivity remained unaltered.
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Author | Naberezhnov, Aleksandr A. Ionescu, Emanuel Kumar, Ravi Nallathambi, Varatharaja Bhaskar, Lalith Kumar Wang, Di Sumnikov, Sergey V. |
Author_xml | – sequence: 1 givenname: Varatharaja surname: Nallathambi fullname: Nallathambi, Varatharaja organization: Laboratory for High Performance Ceramics, Department of Metallurgical and Materials Engineering, Indian Institute of Technology Madras (IIT Madras), Chennai 600036, India – sequence: 2 givenname: Lalith Kumar surname: Bhaskar fullname: Bhaskar, Lalith Kumar organization: Laboratory for High Performance Ceramics, Department of Metallurgical and Materials Engineering, Indian Institute of Technology Madras (IIT Madras), Chennai 600036, India – sequence: 3 givenname: Di orcidid: 0000-0001-9817-7047 surname: Wang fullname: Wang, Di organization: Institute of Nanotechnology and Karlsruhe Nano Micro Facility (KNMFi), Karlsruhe Institute of Technology, Eggenstein-Leopoldshafen, Germany – sequence: 4 givenname: Aleksandr A. surname: Naberezhnov fullname: Naberezhnov, Aleksandr A. organization: Laboratory of Neutron Research, Ioffe Institute, St.-Petersburg, Russia – sequence: 5 givenname: Sergey V. surname: Sumnikov fullname: Sumnikov, Sergey V. organization: Frank Laboratory of Neutron Physics, Joint Institute for Nuclear Research, Dubna, Russia – sequence: 6 givenname: Emanuel orcidid: 0000-0002-3266-3031 surname: Ionescu fullname: Ionescu, Emanuel organization: Institute for Materials Sciences, Technical University of Darmstadt, Darmstadt 64287, Germany – sequence: 7 givenname: Ravi orcidid: 0000-0001-6856-6092 surname: Kumar fullname: Kumar, Ravi email: nvrk@iitm.ac.in organization: Laboratory for High Performance Ceramics, Department of Metallurgical and Materials Engineering, Indian Institute of Technology Madras (IIT Madras), Chennai 600036, India |
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