Robust and Sustainable Indium Anode Leading to Efficient and Stable Organic Solar Cells
The fast degradation of the charge‐extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long‐term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non‐sustainable indium to construct efficient and stable OSCs and scale‐up modu...
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| Published in | Advanced materials (Weinheim) Vol. 35; no. 39; p. e2303729 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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01.09.2023
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| Abstract | The fast degradation of the charge‐extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long‐term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non‐sustainable indium to construct efficient and stable OSCs and scale‐up modules is developed. It is revealed that the recovered indium chloride (InCl
3
) from indium oxide waste can be applied as an effective hole‐selective interfacial layer for the ITO electrode (noted as InCl
3
–ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl
3
–ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm
2
), respectively. More importantly, the InCl
3
–ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T
80
lifetime of ≈10 000 h. |
|---|---|
| AbstractList | The fast degradation of the charge-extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long-term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non-sustainable indium to construct efficient and stable OSCs and scale-up modules is developed. It is revealed that the recovered indium chloride (InCl
) from indium oxide waste can be applied as an effective hole-selective interfacial layer for the ITO electrode (noted as InCl
-ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl
-ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm
), respectively. More importantly, the InCl
-ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T
lifetime of ≈10 000 h. The fast degradation of the charge‐extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long‐term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non‐sustainable indium to construct efficient and stable OSCs and scale‐up modules is developed. It is revealed that the recovered indium chloride (InCl 3 ) from indium oxide waste can be applied as an effective hole‐selective interfacial layer for the ITO electrode (noted as InCl 3 –ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl 3 –ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm 2 ), respectively. More importantly, the InCl 3 –ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T 80 lifetime of ≈10 000 h. The fast degradation of the charge-extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long-term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non-sustainable indium to construct efficient and stable OSCs and scale-up modules is developed. It is revealed that the recovered indium chloride (InCl3 ) from indium oxide waste can be applied as an effective hole-selective interfacial layer for the ITO electrode (noted as InCl3 -ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl3 -ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm2 ), respectively. More importantly, the InCl3 -ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T80 lifetime of ≈10 000 h.The fast degradation of the charge-extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long-term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non-sustainable indium to construct efficient and stable OSCs and scale-up modules is developed. It is revealed that the recovered indium chloride (InCl3 ) from indium oxide waste can be applied as an effective hole-selective interfacial layer for the ITO electrode (noted as InCl3 -ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl3 -ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm2 ), respectively. More importantly, the InCl3 -ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T80 lifetime of ≈10 000 h. The fast degradation of the charge‐extraction interface at indium tin oxide (ITO) poses a significant obstacle to achieving long‐term stability for organic solar cells (OSCs). Herein, a sustainable approach for recycling non‐sustainable indium to construct efficient and stable OSCs and scale‐up modules is developed. It is revealed that the recovered indium chloride (InCl3) from indium oxide waste can be applied as an effective hole‐selective interfacial layer for the ITO electrode (noted as InCl3–ITO anode) through simple aqueous fabrication, facilitating not only energy level alignment to photoactive blends but also mitigating parasitic absorption and charge recombination losses of the corresponding OSCs. As a result, OSCs and modules consisting of InCl3–ITO anodes achieve remarkable power conversion efficiencies (PCEs) of 18.92% and 15.20% (active area of 18.73 cm2), respectively. More importantly, the InCl3–ITO anode can significantly extend the thermal stability of derived OSCs, with an extrapolated T80 lifetime of ≈10 000 h. |
| Author | Xiang, Jiale Chen, Hongzheng Li, Chang‐Zhi Liu, Zhi‐Xi |
| Author_xml | – sequence: 1 givenname: Jiale surname: Xiang fullname: Xiang, Jiale organization: State Key Laboratory of Silicon and Advanced Semiconductor Materials Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China – sequence: 2 givenname: Zhi‐Xi orcidid: 0000-0002-6742-2465 surname: Liu fullname: Liu, Zhi‐Xi organization: State Key Laboratory of Silicon and Advanced Semiconductor Materials Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China – sequence: 3 givenname: Hongzheng surname: Chen fullname: Chen, Hongzheng organization: State Key Laboratory of Silicon and Advanced Semiconductor Materials Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China – sequence: 4 givenname: Chang‐Zhi orcidid: 0000-0003-1968-2032 surname: Li fullname: Li, Chang‐Zhi organization: State Key Laboratory of Silicon and Advanced Semiconductor Materials Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China |
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| Keywords | organic solar cells anode interfacial layers high stability indium recovery modules |
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| SubjectTerms | Anodes Energy conversion efficiency Energy levels Indium oxides Indium tin oxides Materials science Modules Photovoltaic cells Solar cells Thermal stability |
| Title | Robust and Sustainable Indium Anode Leading to Efficient and Stable Organic Solar Cells |
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