Recent Advances of Oxidative Radical Cross‐Coupling Reactions: Direct α‐C(sp3)–H Bond Functionalization of Ethers and Alcohols
Oxygen‐containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct α‐C–H functionalization of inexpensive and abundant readily available ethers and alcohols by oxidative radical cross‐coupling with different nucleophilic partners (C–H, N–H,...
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| Published in | Advanced synthesis & catalysis Vol. 359; no. 1; pp. 2 - 25 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
04.01.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Oxygen‐containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct α‐C–H functionalization of inexpensive and abundant readily available ethers and alcohols by oxidative radical cross‐coupling with different nucleophilic partners (C–H, N–H, O–H and S–S), leading to the construction of C–C and C–X (X=C, N, O, S) bonds, has emerged as one of the vital strategies among oxidative cross‐coupling reactions. Owing to the features of being atom‐economic, environmentally benign, having a simple operation and biologically properties, a series of ether α‐C(sp3)–H bond activation reactions have been developed by metal or metal‐free systems via the radical oxidative coupling pathway, since the radical oxidative coupling reactions have wide range of applications. This review aims to highlight the recent advances in direct α‐C(sp3)–H bond functionalization of ethers and alcohols via radical oxidative process. |
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| AbstractList | Oxygen‐containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct α‐C–H functionalization of inexpensive and abundant readily available ethers and alcohols by oxidative radical cross‐coupling with different nucleophilic partners (C–H, N–H, O–H and S–S), leading to the construction of C–C and C–X (X=C, N, O, S) bonds, has emerged as one of the vital strategies among oxidative cross‐coupling reactions. Owing to the features of being atom‐economic, environmentally benign, having a simple operation and biologically properties, a series of ether α‐C(
sp
3
)–H bond activation reactions have been developed by metal or metal‐free systems
via
the radical oxidative coupling pathway, since the radical oxidative coupling reactions have wide range of applications. This review aims to highlight the recent advances in direct α‐C(
sp
3
)–H bond functionalization of ethers and alcohols
via
radical oxidative process.
magnified image Oxygen‐containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct α‐C–H functionalization of inexpensive and abundant readily available ethers and alcohols by oxidative radical cross‐coupling with different nucleophilic partners (C–H, N–H, O–H and S–S), leading to the construction of C–C and C–X (X=C, N, O, S) bonds, has emerged as one of the vital strategies among oxidative cross‐coupling reactions. Owing to the features of being atom‐economic, environmentally benign, having a simple operation and biologically properties, a series of ether α‐C(sp3)–H bond activation reactions have been developed by metal or metal‐free systems via the radical oxidative coupling pathway, since the radical oxidative coupling reactions have wide range of applications. This review aims to highlight the recent advances in direct α‐C(sp3)–H bond functionalization of ethers and alcohols via radical oxidative process. Oxygen-containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct alpha -C-H functionalization of inexpensive and abundant readily available ethers and alcohols by oxidative radical cross-coupling with different nucleophilic partners (C-H, N-H, O-H and S-S), leading to the construction of C-C and C-X (X=C, N, O, S) bonds, has emerged as one of the vital strategies among oxidative cross-coupling reactions. Owing to the features of being atom-economic, environmentally benign, having a simple operation and biologically properties, a series of ether alpha -C(sp super(3))-H bond activation reactions have been developed by metal or metal-free systems via the radical oxidative coupling pathway, since the radical oxidative coupling reactions have wide range of applications. This review aims to highlight the recent advances in direct alpha -C(sp super(3))-H bond functionalization of ethers and alcohols via radical oxidative process. |
| Author | Kumar, Pailla Santhosh Yang, Minghua Guo, Sheng‐rong |
| Author_xml | – sequence: 1 givenname: Sheng‐rong surname: Guo fullname: Guo, Sheng‐rong email: guosr9609@lsu.edu.cn organization: Lishui University – sequence: 2 givenname: Pailla Santhosh surname: Kumar fullname: Kumar, Pailla Santhosh organization: Lishui University – sequence: 3 givenname: Minghua surname: Yang fullname: Yang, Minghua email: mhyang@lsu.edu.cn organization: Lishui University |
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| PublicationTitle | Advanced synthesis & catalysis |
| PublicationYear | 2017 |
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| Snippet | Oxygen‐containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct α‐C–H functionalization of... Oxygen-containing heterocycles are an important class of compounds with diverse biological activities. In recent years, direct alpha -C-H functionalization of... |
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| SubjectTerms | Alcohols Bonding C(sp3)–H bond functionalization Carbon-carbon composites Chemical reactions Coupling Ethers radical oxidative coupling Radicals single eletron transfer (SET) Strategy |
| Title | Recent Advances of Oxidative Radical Cross‐Coupling Reactions: Direct α‐C(sp3)–H Bond Functionalization of Ethers and Alcohols |
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