Superior energy‐power performance of N‐doped carbon nano‐onions‐based asymmetric and symmetric supercapacitor devices

Summary Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we have synthesized N‐CNO by a simple flame pyrolysis method for symmetric and asymmetric (ASC) supercapacitor devices. The nitrogen doping is...

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Published inInternational journal of energy research Vol. 46; no. 2; pp. 1234 - 1249
Main Authors Pallavolu, Mohan Reddy, Gaddam, Neelima, Banerjee, Arghya Narayan, Nallapureddy, Ramesh Reddy, Joo, Sang Woo
Format Journal Article
LanguageEnglish
Published Chichester, UK John Wiley & Sons, Inc 01.02.2022
Hindawi Limited
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Abstract Summary Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we have synthesized N‐CNO by a simple flame pyrolysis method for symmetric and asymmetric (ASC) supercapacitor devices. The nitrogen doping is performed in‐situ during the pyrolysis of pyrrole. The synthesized N‐CNO has a high surface area of 49 m2 g−1 with 4 at% nitrogen content. The structural properties have confirmed the formation of graphitic N‐CNO with highly ordered concentric graphene layers with proper lattice spacing. The fabricated symmetric and asymmetric devices have shown high specific capacitance and excellent energy‐power performance. Especially, the ASC device shows a specific capacitance value 205 F g−1 with a high energy density (60 Wh kg−1) and power density (5.5 kW kg−1), leading to an increase in the power density by 260% for a mere 60% decrease in the energy density. In addition, both the novel symmetric and asymmetric devices have shown excellent capacity retention of 96% to 98% over 5000 cycles. The demonstrated results show the superior electrochemical performance of the active material, which indicates that the N‐rich‐CNOs can be used as a novel anode material in energy storage devices with high energy density and high power performance. Symmetric and Asymmetric supercapacitor devices of N‐CNOs.
AbstractList Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we have synthesized N‐CNO by a simple flame pyrolysis method for symmetric and asymmetric (ASC) supercapacitor devices. The nitrogen doping is performed in‐situ during the pyrolysis of pyrrole. The synthesized N‐CNO has a high surface area of 49 m2 g−1 with 4 at% nitrogen content. The structural properties have confirmed the formation of graphitic N‐CNO with highly ordered concentric graphene layers with proper lattice spacing. The fabricated symmetric and asymmetric devices have shown high specific capacitance and excellent energy‐power performance. Especially, the ASC device shows a specific capacitance value 205 F g−1 with a high energy density (60 Wh kg−1) and power density (5.5 kW kg−1), leading to an increase in the power density by 260% for a mere 60% decrease in the energy density. In addition, both the novel symmetric and asymmetric devices have shown excellent capacity retention of 96% to 98% over 5000 cycles. The demonstrated results show the superior electrochemical performance of the active material, which indicates that the N‐rich‐CNOs can be used as a novel anode material in energy storage devices with high energy density and high power performance.
Summary Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we have synthesized N‐CNO by a simple flame pyrolysis method for symmetric and asymmetric (ASC) supercapacitor devices. The nitrogen doping is performed in‐situ during the pyrolysis of pyrrole. The synthesized N‐CNO has a high surface area of 49 m2 g−1 with 4 at% nitrogen content. The structural properties have confirmed the formation of graphitic N‐CNO with highly ordered concentric graphene layers with proper lattice spacing. The fabricated symmetric and asymmetric devices have shown high specific capacitance and excellent energy‐power performance. Especially, the ASC device shows a specific capacitance value 205 F g−1 with a high energy density (60 Wh kg−1) and power density (5.5 kW kg−1), leading to an increase in the power density by 260% for a mere 60% decrease in the energy density. In addition, both the novel symmetric and asymmetric devices have shown excellent capacity retention of 96% to 98% over 5000 cycles. The demonstrated results show the superior electrochemical performance of the active material, which indicates that the N‐rich‐CNOs can be used as a novel anode material in energy storage devices with high energy density and high power performance. Symmetric and Asymmetric supercapacitor devices of N‐CNOs.
Author Nallapureddy, Ramesh Reddy
Gaddam, Neelima
Banerjee, Arghya Narayan
Pallavolu, Mohan Reddy
Joo, Sang Woo
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Snippet Summary Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we...
Highly graphitic nitrogen‐doped carbon nano‐onions (N‐CNO) have attracted much attention in the field of energy storage device applications. Herein, we have...
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SubjectTerms anode electrode
Anodes
asymmetric and symmetric supercapacitor devices
Asymmetry
Capacitance
Carbon
Density
Devices
Electrochemical analysis
Electrochemistry
Electrode materials
Energy
Energy storage
Flux density
Graphene
Nitrogen
N‐CNOs
Pyrolysis
pyrolysis method
Supercapacitors
Synthesis
Title Superior energy‐power performance of N‐doped carbon nano‐onions‐based asymmetric and symmetric supercapacitor devices
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fer.7242
https://www.proquest.com/docview/2622271802
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