A p-type Ti(IV)-based metal-organic framework with visible-light photo-response
Here, we report a new Ti(IV)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72 eV. The electronic structure and bandgap were further investigated by DFT calculations. Photoelectrochemical studies indicated that NTU-9 is...
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| Published in | Chemical communications (Cambridge, England) Vol. 50; no. 29; pp. 3786 - 3788 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
14.04.2014
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Here, we report a new Ti(IV)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72 eV. The electronic structure and bandgap were further investigated by DFT calculations. Photoelectrochemical studies indicated that NTU-9 is photoactive under visible light illumination (λ > 400 nm) and acts as a p-type semiconductor. The results demonstrated that Ti(IV)-based MOFs could be promising visible-light photocatalysts for energy conversion and environmental remediation. |
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| AbstractList | Here, we report a new Ti(
iv
)-based porous metal–organic framework (MOF) (
NTU-9
), which displayed strong absorption in the visible region with a bandgap of 1.72 eV. The electronic structure and bandgap were further investigated by DFT calculations. Photoelectrochemical studies indicated that
NTU-9
is photoactive under visible light illumination (
λ
> 400 nm) and acts as a p-type semiconductor. The results demonstrated that Ti(
iv
)-based MOFs could be promising visible-light photocatalysts for energy conversion and environmental remediation. Here, we report a new Ti(IV)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72 eV. The electronic structure and bandgap were further investigated by DFT calculations. Photoelectrochemical studies indicated that NTU-9 is photoactive under visible light illumination (λ > 400 nm) and acts as a p-type semiconductor. The results demonstrated that Ti(IV)-based MOFs could be promising visible-light photocatalysts for energy conversion and environmental remediation. Here, we report a new Ti(iv)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72 eV. The electronic structure and bandgap were further investigated by DFT calculations. Photoelectrochemical studies indicated that NTU-9 is photoactive under visible light illumination ( lambda > 400 nm) and acts as a p-type semiconductor. The results demonstrated that Ti(iv)-based MOFs could be promising visible-light photocatalysts for energy conversion and environmental remediation. |
| Author | Liu, Bin Li, Pei-Zhou Zhang, Qichun Miao, Jianwei Gao, Junkuo Teng, Wen Yuan Zhao, Yanli Yang, Ling |
| Author_xml | – sequence: 1 givenname: Junkuo surname: Gao fullname: Gao, Junkuo email: qczhang@ntu.edu.sg organization: School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, Singapore. qczhang@ntu.edu.sg – sequence: 2 givenname: Jianwei surname: Miao fullname: Miao, Jianwei – sequence: 3 givenname: Pei-Zhou surname: Li fullname: Li, Pei-Zhou – sequence: 4 givenname: Wen Yuan surname: Teng fullname: Teng, Wen Yuan – sequence: 5 givenname: Ling surname: Yang fullname: Yang, Ling – sequence: 6 givenname: Yanli surname: Zhao fullname: Zhao, Yanli – sequence: 7 givenname: Bin surname: Liu fullname: Liu, Bin – sequence: 8 givenname: Qichun surname: Zhang fullname: Zhang, Qichun |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24522830$$D View this record in MEDLINE/PubMed |
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| Snippet | Here, we report a new Ti(IV)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72... Here, we report a new Ti( iv )-based porous metal–organic framework (MOF) ( NTU-9 ), which displayed strong absorption in the visible region with a bandgap of... Here, we report a new Ti(iv)-based porous metal-organic framework (MOF) (NTU-9), which displayed strong absorption in the visible region with a bandgap of 1.72... |
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| SubjectTerms | Absorption Catalysis Energy gaps (solid state) Illumination Light Mathematical analysis Metal-organic frameworks Organic Chemicals - chemistry P-type semiconductors Photocatalysts Porosity Remediation Semiconductors Titanium - chemistry |
| Title | A p-type Ti(IV)-based metal-organic framework with visible-light photo-response |
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