The improved electrochemical performance of cross-linked 3D graphene nanoribbon monolith electrodes
Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GN...
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| Published in | Nanoscale Vol. 7; no. 15; pp. 6504 - 6509 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
England
21.04.2015
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| Abstract | Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes – [Ru(NH
3
)
6
]
3+/2+
, [Fe(CN)
6
]
3−/4−
and important bio-analytes – dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 μF cm
−2
) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices. |
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| AbstractList | Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes--[Ru(NH3)6](3+/2+), [Fe(CN)6](3-/4-) and important bio-analytes--dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 μF cm(-2)) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices.Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes--[Ru(NH3)6](3+/2+), [Fe(CN)6](3-/4-) and important bio-analytes--dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 μF cm(-2)) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices. Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes - [Ru(NH sub(3)) sub(6)] super(3+/2+), [Fe(CN) sub(6)] super(3-/4-) and important bio-analytes - dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 mu F cm super(-2)) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices. Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes – [Ru(NH 3 ) 6 ] 3+/2+ , [Fe(CN) 6 ] 3−/4− and important bio-analytes – dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 μF cm −2 ) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices. Technical advancement in the field of ultra-small sensors and devices demands the development of novel micro- or nano-based architectures. Here we report the design and assembly of cross-linked three dimensional graphene nanoribbons (3D GNRs) using solution based covalent binding of individual 2D GNRs and demonstrate its electrochemical application as a 3D electrode. The enhanced performance of 3D GNRs over individual 2D GNRs is established using standard redox probes--[Ru(NH3)6](3+/2+), [Fe(CN)6](3-/4-) and important bio-analytes--dopamine and ascorbic acid. 3D GNRs are found to have high double layer capacitance (2482 μF cm(-2)) and faster electron transfer kinetics; their exceptional electrocatalytic activity towards the oxygen reduction reaction is indicative of their potential over a wide range of electrochemical applications. Moreover, this study opens a new platform for the design of novel point-of-care devices and electrodes for energy devices. |
| Author | Alwarappan, Subbiah Narayanan, Tharangattu N. Vineesh, Thazhe Veettil |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25712510$$D View this record in MEDLINE/PubMed |
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| Title | The improved electrochemical performance of cross-linked 3D graphene nanoribbon monolith electrodes |
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